Surface acoustic wave-induced electroluminescence intensity oscillation in planar light-emitting devices ∗ Marco Cecchini, Vincenzo Piazza, and Fabio Beltram NEST-INFM and Scuola Normale Superiore, I-56126 Pisa, Italy D. G. Gevaux, M. B. Ward, and A. J. Shields 5 Toshiba Research Europe Limited, Cambridge Research Laboratory, 0 260 Cambridge Science Park, Milton Road, Cambridge CB4 OWE, United Kingdom 0 2 H. E. Beere and D. A. Ritchie n Cavendish Laboratory, University of Cambridge, Cambridge CB3 0HE, United Kingdom a J Electroluminescenceemissionfromsurfaceacousticwave-drivenlight-emittingdiodes(SAWLEDs) 7 is studied by means of time-resolved techniques. We show that the intensity of the SAW-induced electroluminescenceismodulatedattheSAWfrequency(∼1GHz),demonstratingelectroninjection ] intothe p-typeregion synchronouswith the SAW wavefronts. r e h Surface-acoustic-wave(SAW) based devices are nowa- the acoustoelectric effects to planar systems where both t o days widely used for mobile and wireless applications, electron and holes are present and allow detailed studies . t as well as for satellite communications and military oftheeffectsoftheacousticmodulationinlight-emitting a applications[1]. The large-scale diffusion of sophisti- devices (LEDs). m cated communication systems stimulated a fast rise in In this Letter we report on time-resolved studies of - d the SAW-based device market, reaching a production theacoustoelectriceffectsinplanarLEDs. Wefabricated n volume of several million devices per day[2]. More re- devices containing lateral n-p junctions and interdigital o cently SAWs have attracted the interest of the semicon- transducersforSAWgeneration(SAWLEDs)andstudied c ductorcommunityinview ofthe exploitationoftheirin- theopticalpropertiesofthedevicesinducedbytheacous- [ teraction properties with two-dimensional-electron-gases tic perturbation. We monitored SAW-induced electro- 1 (2DEGs)embeddedinsemiconductorheterostructures[3, luminescence (EL) as a function of time and demon- v 4]. SAWs propagating through mesas containing high- strated the presence of oscillations with the same period 6 quality 2DEGs indeed drive modifications on the 2DEG of the SAW (∼1 ns). 3 equilibrium state. Acoustic waves propagating along Devices were fabricated starting with a p-type 1 1 piezo-electric substrates are accompanied by potential modulation-doped Al0.3Ga0.7As/GaAs heterostructure 0 waves which can trap electrons in their minima and in- grown by molecular beam epitaxy, containing a two- 5 duce dc currents or voltages[5, 6, 7]. The discovery of dimensionalholegas(2DHG)withina20-nm-wideGaAs 0 the so-called acoustoelectric effect was followed by the quantum well embedded 70nm below the surface. The / proposal of innovative device concepts. Among these measuredhole density and mobility after illumination at t a Talyanskiiet al. proposedthe implementationof a novel 1.5K were 2.0×1011 cm−2 and 35000cm2/Vs, respec- m current standard, demonstrating very precise acousto- tively. - electriccurrentquantizationduetochargedragbySAWs The heterostructurewas processedinto mesas with an d througha quantum pointcontact[8, 9, 10, 11, 12]. Con- annealed p-type Au/Zn/Au (5/50/150nm) Ohmic con- n trol over the constriction width allows very precise se- o tact. The fabrication of the n-type region of the junc- lection of the number of electrons packed in each SAW c tion followed Ref.[15]. The Be-doped layer was removed : minimum down to the single-electron-transport regime. from part of the mesa by means of wet etching (48s in v One of the most appealing applications proposed after i H3PO4:H2O2:H2O = 3:1:50) and the sample was loaded X the first report of the acoustoelectric quantized current into a thermal evaporator for the deposition of a self- r was to incorporate single-electron SAW pumps in pla- alignedNi/AuGe/Ni/Au(5/107/10/100nm)n-typecon- a nar 2D electron/2D hole gas (n-p) junctions to fabricate tact. After annealing, donors introduced by the n-type high-repetition-rate single-photon sources. contactprovideconductionelectronswithinthewellthus Very recently two different groups demonstrated one creatinganelectrongasbelowthemetalpad,adjacentto of the main building blocks of such source, that is the the 2DHG (inset of Fig1(a)). The n-contact was shaped possibilitytoswitchontheelectroluminescenceofplanar as a thin stripe placed perpendicular to the SAW propa- n-p junctions by applying SAWs[13, 14]. From a more gation direction, 250µm away from the p-contact. fundamental physics point of view these results extend SAWs propagating along the (0¯1¯1) crystal direction were generated by means of an interdigital transducer (IDT) composed of 100 pairs of 200µm-long Al fingers with 3µm periodicity (∼1GHz resonance frequency on ∗Electronicaddress: [email protected] GaAs). Transducers were fabricated at a distance of 2 EL measurements at low temperature (5K). Spectra as (a) 10-3 5 K a function of bias were collected by a cooled CCD af- ter spectral filtering by a single-grating monochromator. TheELspectrareportedinFig.1(b)showamainpeakat 10-5 818.7nm (full width half maximum (FWHM) of 1.8nm) RT originatingfromradiativerecombinationwithin the QW ) (A 10-7 p-type Be-doped layer andasecondarypeakat831.2nm(FWHM3.6nm)which I contact n-type originates from carbon impurities included in the het- contact erostructure material during growth[16]. The origin 10-9 (cid:0)(cid:0)(cid:0)(cid:0)(cid:0)(cid:0)(cid:0)(cid:0)(cid:0)(cid:0)(cid:0)(cid:0)(cid:0) (cid:1)(cid:1)(cid:1)(cid:1)(cid:1)(cid:1)(cid:1)(cid:1)(cid:1)(cid:1)(cid:1)(cid:1)(cid:1)(cid:1)(cid:1)(cid:1)(cid:1)(cid:1)(cid:1) of such peaks was also verified by photo-luminescence Holes Electrons measurements[17]. Light intensity, calculated by inte- GaAs QW gration over the main EL peak from 810nm to 826nm, as a function of the forwardbias applied to the junction 0 1 2 3 4 Forward Bias (V) reflects the rectifying behavior of the IV curves (inset of Fig.1(b)), showing a detection threshold of ∼1.65V. (b) 1.8 V TheSAWresonancefrequencywasdeterminedbymea- u.) 1.7 V suringthepowerreflectedbythetransducerasafunction b. u.) 1.6 V of excitation frequency. The transducer frequency re- ar b. sponse displayedat 5K a pronounceddip at 987.5MHz, ( ar y y ( whichisconsistentwiththeperiodicityofthetransducer, sit nsit and had a FWHM of 2.4MHz. Inten EL Inte T = 5 K driTvheeeltercatvreolnlisnginetloectthreic2fiDelHdGaswsohceinatethdewjiutnhcStiAoWn siscbain- L 1.6 1.7 ased just below threshold [13, 14]. Indeed, we observed E Forward Bias (V) the light versus voltage curve to shift to lower biases by ∼10meVinpresenceofSAWs(Fig.2(a)). Themaximum shiftwasobservedat-10dBmpowerlevel. Athigherlev- 800 810 820 830 els the increased electron extraction is counterbalanced Wavelength (nm) by the spatial separation of electrons and holes trapped respectively in SAW minima and maxima, leading to a FIG. 1: (a) Current-voltage characteristics from room tem- progressivesuppression of the EL signal.[14] perature down to 5K. Inset: fabrication scheme of the n-p The emission spectra were changed by the SAW only lateral junction. (b) Electro-luminescence spectra at differ- in intensity and no spectral shift of the main peaks was ent forward biases around the emission detecting threshold. observed (Fig.2(b)). Light-intensity data as a function Inset: Light-voltage characteristic of the planar LED at T = 5K. of IDT excitation frequency demonstrate that emission intensification occurs only within the transducer pass- band, as shown in the inset of Fig.2(b). 800µmfromthemesabyelectron-beamlithography. The We also studied the SAW-induced EL signal by time- width of the n-type contact stripe (2µm) was chosen of resolved measurements. To this end the EL signal was the same order of magnitude as the SAW wavelength spectrally filtered by a triple grating monochromator (3µm)inordertolimitSAWdampingduetothemassive and detected by a single-photon APD module (Perkin metalization and SAW diffusion originating from non- ElmerSPCM-AQR-16). Inordertoobtaintime-resolved uniform penetration of the Ohmic contact and inhomo- ELtracesweusedtime-correlatedphoton-countingtech- geneities in the etched region. niques. The signal from the SPCM was directed toward SeveralSAWLEDswerefabricatedandstudied,andall theSTARTinputofaBecker&HicklSPC-600computer of them showed qualitatively similar characteristics. All board,whiletheSTOPinputwasdrivenbyasignalsyn- the data shown in the following refer to one representa- chronous to that used to generate the SAW. A typical tivedevice,forwhichthetransportandopticalproperties data trace is shown in Fig.3(a). EL oscillations with ofthejunction,aswellastheefficiencyofthetransducer, period of about 1ns are present in the curve, reflecting will be systematically analyzed. the presenceofthe SAWmodulatingthe junctionpoten- The SAWLED was first electrically tested at low tem- tial. TheseoscillationsaremoreclearlyvisibleinFig.3(c) perature to verify the proper formation of the lateral where a magnified view of Fig.3(a) is displayed with a diode. Current-voltage curves (IVs) at different temper- smootheddatatrace. Thiseffectisfurtherhighlightedin atures(fromroomtemperaturedownto5K)showedrec- the frequency domain of the signal. Fig.3(b) reports the tifyingbehaviorandintersectedat∼1.5V(seeFig.1(a)). Fourier transform of the EL signal. A single peak at the This value corresponds to the diode conduction thresh- SAWfrequency clearlydominatesthe Fouriertransform. oldanditis consistentwiththe valueexpectedforGaAs Time-correlated measurements were made at different n-pjunctions. Emissionpropertieswerecharacterizedby biasesappliedtothejunction. Theoscillationamplitudes 3 ) Time (ns) . u (a) . NO SAW 10 15 20 25 30 35 40 b r SAW (-10 dBm) (a) a s sity ( Count800 ( b) n %)1.8 te 6 > (1.6 n C L I T = 5 K e C/<1.4 E 1.62 1.64 1.66 1.68 1.70 1.72 ud 4 D1.2 Forward bias (V) mplit 1.7 1.8 Forward bias (V) A 2 ) (b) Bias = 1.675 V u. T = 5 K b. u.) sity (ar ensity (arb. NSAOW SAW 0.5 F1.r0equen1.c 5y (GH2z.0) 2.5 (c) n nt 880 nte EL I 980 990 1000 860 I RF frequency (MHz) s L nt E u 840 o C 800 810 820 830 820 Wavelength (nm) 800 FIG. 2: (a) Light-voltage characteristic of the planar LED 42.0 42.5 43.0 43.5 44.0 44.5 without SAW (dashed line) and with SAW (solid line). Time (ns) SAW power and frequency were -10dBm and 987.5MHz re- spectively. (b) Electro-luminescence spectra without SAW FIG.3: (a)ELtimeevolutioninpresenceofSAW(987.5MHz, (dashedline)andinpresenceofaSAW(-10dBm,987.5MHz) -10dBm), at T = 5K and for a forward bias of 1.85V. (b) (solid line). Inset: electro-luminescence as a function of RF- Fouriertransform ofthetoppanelEL signal. Inset: Normal- frequency (-9 dBm) at T = 5K. The junction was forward izedoscillationintensityasafunctionoftheforwardbias. (c) biased with 1.8 V. ZoomofthetimeevolutionofSAW-inducedELshowedin(a) superimposed onto an FFT smoothing. werecalculatedfromtheFouriertransformsandnormal- ized by the corresponding mean EL intensities. In the recombining at different times depending on their posi- inset ofFig.3(b)we reportthe normalizedoscillationin- tion along the junction. The resulting oscillations are tensity as a function of the forwardbias. The oscillation therefore averaged out, while the EL mean-intensity in- amplitude is around 1.5% of the signal and remains al- creasestillremainspresent. Webelievethatfurtheropti- most unchanged at different bias voltages, as expected mizationofthedevicegeometrywillleadtohighcontrast for an exponential increase of the EL close to the con- oscillations and is currently being investigated. duction threshold. Since the recombination time in our In conclusion, we fabricated n-p lateral junctions with system is much less than 1 ns, determined by means of interdigital transducers and studied the effect of SAWs photoexcited-carrier lifetime measurements, the reason on the device time-resolved emission properties. SAW- for the observed small oscillation amplitude originates inducedemissionwasfirstcharacterizedbyspectralmea- from other limiting factors. Ideally the SAW wavefronts surements andlight-voltagemeasurements. Electrolumi- would get to the thin n-type contactwithout any distor- nescencewasobservedtoincreaseinintensityinthepres- tion and perfectly parallel to the contact itself. But real ence of SAWs when the diode was biased near the con- devices introduce deviations from the picture described duction threshold. Time-resolved measurements of the above. The presence of the mesa edges and of defects electroluminescence in the presence of SAWs were car- alongthe SAW pathintroducedduring the mesa etching ried out at severalbias voltages,demonstrating modula- process constitute scattering centers which lead to mod- tion of the light intensity at the frequency of the SAW ification of the acoustic wave-fronts. In addiction, an- (∼1GHz). Theamplitudeoftheoscillationwasfoundto nealed Ohmic contacts have a strong corrugation. 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