Research and Development on a Salt Processing Alternative for High-Level Waste at the Savannah River Site PDF
Preview Research and Development on a Salt Processing Alternative for High-Level Waste at the Savannah River Site
ee us i s are trd. Plea ke eaert ge bry ins EVALUATION OF CRITERIA FOR Paall s. ent ed ting filesetbeen acci PROCSEELSESCINTGIN AGL TAE SRANLATTIVE al typhave ginay FOR HIGH-LEVEL WASTE AT orim he ors m terr THE SAVANNAH RIVER SITE: k, not froographic INTERIM REPORT op oy er bme t p ao ps original ed, and he ain m tret Committee on Radionuclide Separation Processes for High-Level Waste at the Savannah oe ed frat bnnot Board on RadioaRcitviveer SWitaeste Management ea es crer, c Board on Chemical Sciences and Technology L filwev Division on Earth and Life Studies Mo Xh National Research Council m g, ed fromattin en recomposg-specific forn. eno the original work has bation of and other typesettiding styles, for attributiauthoritative version epresentaks, hean as the digital rord breblicatio PDF file: This new nal; line lengths, wnt version of this pu NATIONWAaLsh AinCgtAoDn,E DM.CY. PRESS About this to the origiuse the pri ee us ii s are trd. Plea eakerte NATIONAL ACADEMY PRESS 2101 Constitution Avenue, N.W. Washington, D.C. 20418 ge bry ins NbeOrsT aIrCeE d:r Tawhen pfrroomjec tth teh acto uisn tchiles soufb tjheec tN oaf ttihoinsa rle Apocratd wemasy aopfp Srocvieendc besy, tthhee GNoavtieornnailn gA cBaodaermd yo fo tfh Ee nNgaintieoenrainl gR, easneda rtchhe CInosutintcuitle, owfh Moseed miceinme-. Paall The members of the committee responsible for the report were chosen for their special competences and with regard for appropriate balance. s. ent This study was supported by Contract/Grant No. DEFC0199EW59049 between the National Academy of Sciences and the Department of ed ting filesetbeen acci EiLolrynib errregafylre.y c Ato ntfh yCe oovpniiegnwrioessn oss f,C tfhainetda oilnrogggasinn, igczo-aintnico-lPnuuss iboolrni csaa,g toeirno crnei ecDso amthtamat epnrdoavtiidoends seuxpppreosrst efdo ri nth teh ipsr poujebclti.cation are those of the author(s) and do not necessar- al typhave ILnitberranrayt ioofn Calo Sntgarnedsas rCd aBtaolookg NCuarmdb Neru m0-b3e0r9 9-07X-XXXXXXX-XX ginay Additional copies of this report are available from National Academy Press, 2101 Constitution Avenue, N.W., Lockbox 285, Washington, orim D.C. 20055; (800) 624-6242 or (202) 334-3313 (in the Washington metropolitan area); Internet, http://www.nap.edu he ors Printed in the United States of America m terr k, not froographic Copyright 2001 by the National Academy of Sciences . All rights reserved. op oy er bme t p ao ps original ed, and he ain m tret oe ed frat bnnot ea es crer, c L filwev Mo Xh m g, ed fromattin en recomposg-specific forn. eno the original work has bation of and other typesettiding styles, for attributiauthoritative version epresentaks, hean as the digital rord breblicatio e: This new e lengths, won of this pu PDF filnal; linnt versi About this to the origiuse the pri ee us iii s are trd. Plea ke eaert ge bry ins Paall s. ent ed ting filesetbeen acci al typhave ginay orim he ors m terr The National Academy of Sciences is a private, nonprofit, self-perpetuating society of distinguished k, not froographic stCecochhnongloarelrossg se yin nag na1dg8 e6tod3 ,ti hnthe sierc Aiuescneat idffoeirc m tahyne d gh eeannsge ari anmle waenreidlnfagatr ere e.t shUeaapt rorcneh qt,hu deier aedusi ctihato tteroid tay td oov fti hstheee ft hucehrt ahfreetderrae nrgacrlae ng otoefv dse ctroine mint cebeny ta tonhnde op er bome ty scientific and technical matters. Dr. Bruce M. Alberts is president of the National Academy of Sciences. p ao ps The National Academy of Engineering was established in 1964, under the charter of the National Academy original ed, and othfe S sceileenccteiosn, aosf a i tpsa mraelmlelb oerrgs,a snhizaaritniogn w oift ho uthtset aNnadtiinogn aeln Agicnaedeersm. yIt oisf Sauctioennocemso tuhse irne siptso andsmibiinliitsyt rfaotrio and vanisdi nign he ain the federal government. The National Academy of Engineering also sponsors engineering programs aimed at m tret meeting national needs, encourages education and research, and recognizes the superior achievements of oe ed frat bnnot engineers. Dr. William A. Wulf is president of the National Academy of Engineering. ea The Institute of Medicine was established in 1970 by the National Academy of Sciences to secure the es crer, c services of eminent members of appropriate professions in the examination of policy matters pertaining to L filwev the health of the public. The Institute acts under the responsibility given to the National Academy of XMho Sciences by its congressional charter to be an adviser to the federal government and, upon its own initiative, m g, to identify issues of medical care, research, and education. Dr. Kenneth I. Shine is president of the Institute ed fromattin of Medicine. een recomposng-specific foron. TtaAhdhceve abi dNsreioanmatgdiyo tc,nh otaehml ef mRe Cdeueosneruiaatnylr c cgoihofl vshCceaoirsenu nbmnceceeci nlao tnwm.d aFe stu e tonchrhcegnt aipoonrlinoiznigencydgi pw biaynilt htaoh ctpehc eeNor rAaadttciiaonandngcea eaml gAwyeci’nstah cdp yegu mreopnfyo e bsoreoafs tlS h opc ftoi heflnueiccr Ntiehesaes ti rdniion e1gnt9e ak1rlnm 6Ao itwcnoa leaeddsde sgbmoeyc y aita nhotdeef the original work has bation of and other typesettiding styles, for attributiauthoritative version StIrwhencwsesip etwsienct.ccuinteetianvest t eiaoiolfnyfind c,M a oatlfh-ne aetddh c iNeeac ndaiNngteiaeimont.ni eioDaeenlsrr aA.i.on lB crgRagr ceudosecemmea mryMc uho. n fAC iEtloinbeugesn.irc ntTiselh .ea erni Cndg oD uinrn. c pWirlo iivlsl iiadadimnmg iA nse.i srWtveiruceeldfs ajtoorei nt hctlehy ag bioryvm ebaronntmh a Aenndct a,v dtiheceme piceuhsba laiinrcmd, aatnhnde, epresentaks, hean as the digital rord breblicatio e: This new e lengths, won of this pu PDF filnal; linnt versi About this to the origiuse the pri ee us iv s are trd. Plea ke eaert ge bry ins COMMITTEE ON RADIONULIDE SEPARATION PROCESSES FOR HIGH-LEVEL Paall WASTE AT THE SAVANNAH RIVER SITE s. ent ed ting filesetbeen acci GJMORIHLETNGO OEN.R BYLEE RRV.C ECANHWSOO,P NCPa,I lNCif,ho Varniirci,ae B -ICnehscthaittiuer,lt eI notfe Trneacthionnoalol g(rye,t iPreadsa),d Meneanlo Park, California al typhave DJAAMREYSL HE .H E.S BPUESNCSHO,N U, nIoivwears Sittya toef UKnainvsearss,i tLya, wArmenecse originmay GEORGE E. KELLER II, Union Carbide Corporation (retired), South Charleston, West Virginia he ors THEODORE A. KOCH, E.I. du Pont de Nemours and Company (retired), Wilmington, Delaware m terr ALFRED P. SATTELBERGER, Los Alamos National Laboratory, Los Alamos, New Mexico k, not froographic MARTIN J. STEINDLER, Argonne National Laboratory (retired), Downers Grove, Illinois op Staff oy er bme t ROBERT S. ANDREWS, Senior Staff Officer, Board on Radioactive Waste Management p ao ps CHRISTOPHER K. MURPHY, Program Officer, Board on Chemical Sciences and Technology original ed, and LTOANUIR GAR LELEANNLOESA, FS,e Anidomr iPnriosjteractti vAes sAisstsaoncti,a Bteo, aBrdo aornd Ronad Rioaadciotiavcet iWvea Wstea sMtea nMaagneamgeenmtent he ain m tret oe ed frat bnnot ea es crer, c L filwev Mo Xh m g, ed fromattin en recomposg-specific forn. eno the original work has bation of and other typesettiding styles, for attributiauthoritative version epresentaks, hean as the digital rord breblicatio e: This new e lengths, won of this pu PDF filnal; linnt versi About this to the origiuse the pri ee us v s are trd. Plea ke eaert ge bry ins BOARD ON RADIOACTIVE WASTE MANAGEMENT Paall s. ent JOHN F. AHEARNE, Chair, Sigma Xi and Duke University, Research Triangle Park, North Carolina ed ting filesetbeen acci CRROHOBABEERRRLTTE SMJ .M .B BCUECDRONNMIETBRZI,OE F,, uCVtuiocrnees- uRClehtasanoitru,,r BcCeeostn hAseusslsdtoaacn, iMta, tGaersiy,p lIfan-nOcd.b, eBrefrrikcekl,e Sy,w Citazleifrolarnndia al typhave GROREDGNOERYY C R. E. WCHINOGP,P UINn,i vFelorsriitdya o Sf tMateic Uhingiavne,r sAitnyn, TAarlblaohrassee ginay JAMES H. JOHNSON, JR., Howard University, Washington, D.C. m the orierrors m RNOIKGOELRA EY. KP.A LSAPVEERRSOONV,, CRluasrski aUnn Aivceardseitmy,y W ofo Srcceisetnecre, sM, Masosascchouwsetts k, not froographic JAWALINLEELX IACA.NMSD. LAEO.R MN MGILA, LMCSLa, AcOkCaakHy RLScAidhNgoeo, lEA o.sIfs. oMdcuii naPteeosdn, tUU dnneii vvNeeerrsmsiittoyiue osrs f( r&Nete iCvreoaddm)a,p, OaRnleynn e(oyre, tMireadry),l aWndilmington, Delaware ooyp MARTIN J. STEINDLER, Argonne National Laboratories (retired), Argonne, Illinois er bme t ATSUYUKI SUZUKI, University of Tokyo, Japan p ao JOHN J. TAYLOR, Electric Power Research Institute (retired), Palo Alto, California VICTORIA J. ps original ed, and TSCHINKEL, Landers and Parsons, Tallahassee, Florida he ain Staff m tret oe KEVIN D. CROWLEY, Director ed frat bnnot RBAORBBERATR AS. PAANSDTRINEAW, SS,t aSfefn Oiofrf iScetarff Officer ea es crer, c GREGORY H. SYMMES, Senior Staff Officer ML filowev JSOUHSNAN R .B W. MILOECYK, SLeEnRio, rR Setsaefafr Ochf fAicsesrociate Xh m g, TONI GREENLEAF, Administrative Associate ed fromattin LLAAUTRRIAC IDA. CLL. BAANIOLSE,Y S,e Sneionri oPrr Pojreocjte cAt sAsissstiasntatnt en recomposg-specific forn. SAJAUNMZGAEENSL NAYE AR TS. TETASA,CY JKRLO.H, ROO,Uf fSiSceEen ,iA oPrsr soPijrseotcajten cAtt sAsissstiasntatnt eno the original work has bation of and other typesettiding styles, for attributiauthoritative version epresentaks, hean as the digital rord breblicatio e: This new e lengths, won of this pu PDF filnal; linnt versi About this to the origiuse the pri ee us vi s are trd. Plea ke eaert ge bry ins BOARD ON CHEMICAL SCIENCES AND TECHNOLOGY Paall s. ent KENNETH N. RAYMOND, Co-Chair, University of California, Berkeley ed ting filesetbeen acci JJCOOASHTENHP ELHR. MAINN. EDD CEES.R FISMEONONSN,E ECL,o AU-CUnhi,v aUeirrns,i iCvtyea rrosnfiet Nyg iooerf t MhM eCalralyorlonal nUindna, i Cavneodrlsl eiNtgyoe,r PtPhia tCrtskabruorlginha, PSetantnes Uylnviavneirasity, Raleigh al typhave ARILCICHEA RP.D G MA.S GT,R SOtaSnSf,o Drdo Uwn Civheermsiitcya, lS Ctaonmfopradn, yC, aMlifidolranniad, Michigan ginay NANCY B. JACKSON, Sandia National Laboratory, Albuquerque, New Mexico m the orierrors m GSAENOGRTGAEE E K. KIMEL, ELlEi RL iIlIl,y U annido nC oCmarpbaindye, CInodmiapnaanpyo (lrise,t iIrneddi)a, nSaouth Charleston, West Virginia k, not froographic WTPAHILUOLLMI AJA. MSR E JK.I DMLEEEMRY,PE MERRe, rLEckoR s,R AHeslaaermvaraocrshd NLUaantbiivooernarastloi tLryiae, bsC,o aRrmaatobhrrwyida, gyLe, o,N sM eAwals asJmaecroshseu,y sNetetws Mexico ooyp LYNN F. SCHNEEMEYER, Bell Laboratories, Murray Hill, New Jersey er bme t MARTIN B. SHERWIN, Chem Ven Group, Inc., Boca Raton, Florida p ao JEFFREY J. SIIROLA, Chemical Process Research Laboratory, Kingsport, Tennessee ps he original ained, and CAPEHRTNREIOSRLT JDI.N SFET. ASS.TN SAGLN,O UCAnENiLvELer,, s GGiteyen ooerfgr aUial tMIanhos,tt Siotrauslt,te TL orafok Tye,e CcMhitinycohlioggayn, Atlanta m tret JOHN C. TULLY, Yale University, New Haven, Connecticutt oe CHI-HUEY WONG, Scripps Research Institute, La Jolla, California ed frat bnnot STEVEN W. YATES, University of Kentucky, Lexington ea es crer, c Staff ML filowev DOUGLAS J. RABER, Director Xh m g, RUTH MCDIARMID, Program Officer ed fromattin CSYHBRIILS TAO. PPHAEIGRE K, A. MdmUiRniPsHtraYti, vPer oAgsrsaomci Oatfeficer en recomposg-specific forn. eno the original work has bation of and other typesettiding styles, for attributiauthoritative version epresentaks, hean as the digital rord breblicatio e: This new e lengths, won of this pu PDF filnal; linnt versi About this to the origiuse the pri ee us ACKNOWLEDGEMENT OF REVIEWERS vii s are trd. Plea ke eaert ge bry ins Acknowledgement of Reviewers Paall s. ent ed ting filesetbeen acci original typmay have technTichails erxeppeorrtti seh,a si nb aececno rrdeavniecwe ewdi tihn pdroracfetd uforerms abpyp roinvdeidv ibdyu atlhse cNhoatsieonn aflo rR ethseeairr cdhi vCeorsuen cpile r(sNpRecCti)v eRse paonrdt he ors Review Committee. The purpose of this independent review is to provide candid and critical comments that will m terr assist the institution in making the published report as sound as possible and to ensure that the report meets k, not froographic iafnonsldlto idtwurtaiinfotgn m ainla dnsituvasindcdruaiaprldts sr f eofmor rat hioneb icrjeo pcnatfirivtdiicetyinp,t aieatvilo itdnoe ipnnrc oteht,ee ca rtne tdvh ieree wisnp tooefgn trshiitivyse ronefep stosh rett o:d ethlieb esrtautdivye cphraorcgees.s .T Whee rwevisiehw to c tohmanmke tnhtes op er bome ty RJ. oBbreernt tM H.i Bskeeryn,e Uron, iUve.Srs. iNtyu ocfl eAarr iRzoengaulatory Commission (retired) p ao ps Lawrence Kershner, Dow Chemical Company original ed, and JKaemnense tWh .N M. Ritacyhmelol,n Bde, lUl Lniavbesr/sLituyc eonf tC Taelicfhonrnoilao,g Bieesrkeley he ain Edwin L. Zebroski, Elgis Consulting m tret Although the reviewers listed above have provided many constructive comments and suggestions, they were oe ed frat bnnot nreolte aassek.e Td hteo reenvdieowrs eo ft hteh icso rnecploursti ownass oorv reercseoemnm beyn Rdaotyiocne sW n.o Mr duirdr atyh,e yU nseivee trhseit yfi noaf lN dorratfht Cofa rthoeli nreap, oaprtp boeinfoterde bitys ea the NRC's Report Review Committee, who was responsible for making certain that an independent examination es crer, c of this report was carried out in accordance with institutional procedures and that all review comments were L filwev carefully considered. Responsibility for the final content of this report rests entirely with the authoring Mo committee and the institution. Xh m g, ed fromattin en recomposg-specific forn. eno the original work has bation of and other typesettiding styles, for attributiauthoritative version epresentaks, hean as the digital rord breblicatio e: This new e lengths, won of this pu PDF filnal; linnt versi About this to the origiuse the pri ee us ACKNOWLEDGEMENT OF REVIEWERS viii s are trd. Plea ke eaert ge bry ins Paall s. ent ed ting filesetbeen acci al typhave ginay orim he ors m terr k, not froographic op oy er bme t p ao ps original ed, and he ain m tret oe ed frat bnnot ea es crer, c L filwev Mo Xh m g, ed fromattin en recomposg-specific forn. eno the original work has bation of and other typesettiding styles, for attributiauthoritative version epresentaks, hean as the digital rord breblicatio e: This new e lengths, won of this pu PDF filnal; linnt versi About this to the origiuse the pri ee us CONTENTS ix s are trd. Plea ke eaert ge bry ins Contents Paall s. ent ed ting filesetbeen acci al typhave originmay SUMMARY 1 he ors m terr INTRODUCTION 1 k, not froographic BACKGROUND 2 op er bome ty DOE SELECTION CRITERIA AND GOALS 3 p ao ps COMMENTS ON CRITERIA 6 original ed, and FINDINGS AND RECOMMENDATIONS 7 he ain m tret REFERENCES CITED 8 oe ed frat bnnot APPENDIX A. BIOGRAPHICAL SKETCHES OF COMMITTEE MEMBERS 10 ea es crer, c APPENDIX B. LETTERS OF REQUEST FOR THIS STUDY 13 L filwev XMho APPENDIX C. HIGH-LEVEL WASTE TANKS AT THE SAVANNAH RIVER SITE 18 m g, ed fromattin en recomposg-specific forn. eno the original work has bation of and other typesettiding styles, for attributiauthoritative version epresentaks, hean as the digital rord breblicatio e: This new e lengths, won of this pu PDF filnal; linnt versi About this to the origiuse the pri
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