Uranium in the Aquatic Environment: Proceedings of the International Conference Uranium Mining and Hydrogeology III and the International Mine Water Association Symposium Freiberg, Germany, 15-21 September 2002 PDF
Preview Uranium in the Aquatic Environment: Proceedings of the International Conference Uranium Mining and Hydrogeology III and the International Mine Water Association Symposium Freiberg, Germany, 15-21 September 2002
B. J. Merkel• B. Planer-Friedrich • C. Wolkersdorfer (Eds.) Uranium in the Aquatic Environment Springer-Verlag Berlin Heidelberg GmbH B. J. Merkel B. Planer-Friedrich C. Wolkersdorfer (Editors) Uranium in the Aquatic Environment Proceedings of the International Conference Uranium Mining and Hydrogeology 111 and the International Mine Water Association Symposium Freiberg, Germany, 15-21 September 2002 With 453 Figures, 151 Tables and a CD-ROM i Springer Prof. Dr. Broder J. Merkel Dipl-Geol. Britta Planer-Friedrich Dr. Christian Wolkersdorfer Technical University Bergakademie Freiberg Department of Geology Gustav-Zeuner-Str. 12 09596 Freiberg, Germany http://www.geo. tu -freiberg. de!umh! Cataloging-in-Publication Data Applied for Die Deutsche Bibliothek -CIP-Einheitsaufnahme Uranium in the aquatic environment: proceedings of the International Conference Uranium Mirring and Hydrogeology III and the International Mine Water Association Symposium Freiberg, Germany, 15-21 September 2002; with CD-ROM I ed.: Broder Merkel .... - Berlin; Heidelberg; New York; Barcelona; Hongkong; London; Mailand; Paris; Tokio: Springer 2002 ISBN 978-3-642-62877-1 ISBN 978-3-642-55668-5 (eBook) DOI 10.1007/978-3-642-55668-5 This work is subject to copyright. All rights are reserved, whether the whole or part of the material is concerned, specifically of translation, reprinting, reuse of illustrations, recitati on, broadcasting, reproduction on microfllm or in any other way, and storage in data banks. Duplication of this publication or parts thereof is permitted only under the provi sions of the German Copyright Law of September 9, 1965, in its current version, and per mission for use must always be obtained from Springer-Verlag. Violations are liable for prosecution under the German Copyright Law. http://www.springer.de © Springer-Verlag Berlin Heidelberg 2002 Originally published by Springer-Verlag Berlin Heidelberg New York in 2002 Softcover reprint of the hardcover 1st edition 2002 The use of general descriptive names, registered names, trademarks, etc. in this publicati on does not imply, even in the absence of a specific statement, that such names are exempt from relevant protective laws and regulations and therefore free for general use. Production: PRO EDIT GmbH, 69126 Heidelberg, Germany Cover Design: Erich Kirchner, Heidelberg, Germany Typesetting: Camera-ready by the editors Printedon acid-free paper SPIN: 10866911 30/3130S0-5 4 3 2 1 0 - Contents Michael Kinze Dose Limitsand Maximum Concentration Limits (MCL's) for Radionuclides Implication on Remediation ofUranium Mining and Milling Facilities in Saxony, Germany .................................................................................................................. l Alexander T. Jakubick, Rene Kahnt Remediation oriented use of conceptual site models at WISMUT GmbH: Rehabilitation of the Trünzig tailings management area ......................................... 9 Paul L Y ounger Deep mine hydrogeology after closure: insights from the UK ............................. 25 Heinrich Reincke, Stephanie Hurst, Petra Schneider Strategy Concept Elbe ........................................................................................... 41 Gavin M. Mudd Environmental hydrogeology of in situ leach uranium mining in Australia ......... .49 Henk Coetzee, Peter Wade & Frank Winde Reliance on existing wetlands for pollution control around the Witwatersrand gold/uranium mines of South Africa -Are they sufficient? .................................. 59 Gavin K. Gillmore, John Grattan, F. Brian Pyatt, Paul S. Phillips, Gillian Pearce Radon, water and abandoned metalliferous mines in the UK: Environmental and Human Health implications ................................................................................... 65 Peter L. Neitzel, Petra Schneider, Helmut Schlumprecht Physico-chemical surface water conditions of catchments with metallogenic origin: A contribution to the establishment ofthe EC Water Framework Directive 2000/60/EG in Germany ........................................................................................ 77 Polona Vrecek, Ljudmila Benedik, Urska Repinc, Peter Stegnar, Ivan Gantar Radionuclides in underground water in an area contaminated with uranium mill waste ...................................................................................................................... 85 LA. Torgoev, U.G. Aleshyn, H. B. Havenit Impact ofUranium Mining and Processing on the Environment ofMountainous areas of Kyrgyzstan ............................................................................................... 93 Zoran Nikic, Jovan Kovacevic, Branislav Radosevic Uranium content in ground water in Stara Planina Triassie Sediments ................. 99 VI Contents C.R. Dudgeon, F.R.P.Kalf Contaminant transport from proposed Jabiluka mine uranium tailings paste repositories - 10 000 year dispersion and dilution analysis ................................ 10 7 David Read, Karl-Heinz Hellmuth, Juha Kaija, Lasse Ahonen Natural Uranium Fluxes and their Use in Repository Safety Assessment... ........ ll5 Guido Bracke, Bemd Förster, Herbert Meyer, Gerd Hensel, Götz-Wolfram Thauer, Thornas Taylor Long Term Safety ofthe Asse Salt Mine ............................................................ 127 Regina Dashko; Alexey Korotkov Risk Assessment for Underground Disposal ofRadioactive Wastes in Clay Strata ................................................................................................................... 133 Thornas Brasser, Ulrich Noseck, Dagmar Schönwiese Uranium Migration in Argillaceous Sediments as Analogue for Transport Processes in the Far Field ofRepositories (Heselbach Site, Germany) ............... 139 Francisco Lemos, Terry Sullivan, Kurt Friese, Timothy Ross, Maria Barbosa Translating natural concentrations and fluxes into safety indicators for radioactive waste repositories ................................................................................................ 14 7 Stephan Kistinger, Guido Deissmann, Martin Goldsworthy, RalfH. Stollenwerk Evaluation of the long-term durability of engineered dry covers for mining wastes, and consideration ofassociated design constraints ............................................. 155 Petra Schneider; Schaffrath, M.; Nindel, K. Hydrology ofEngineered Covers ofWaste Rock Dumps towards Heavy Rainfall Phenomena: A Case Study in Uranium Mill Tailings Mitigation ....................... 165 Dieter Rammlmair Hard pan forrnation on mining residuals ............................................................. 17 3 Zenko Yoshida, Yoshihiro Meguro, Shuichi lso, Jin Ougiyanagi, Osamu Tomioka, Y ouichi Enokida, Ichiro Yamamoto Supercritical Carbon Dioxide Fluid Leaching (SFL) ofUranium from Solid Wastes Using HN0 -tributylphosphate (TBP) Complex as a Reactant .............. 183 3 Guido Deissmann, Stefan Thierfeldt, Adrian Bath, Stephan Jefferis Release behaviour ofradionuclides from contaminated concrete materials ........ l89 Gregory Delecaut, PierreDe Canniere, Lian Wang and Norbert Maes Solubility of an uranium(IV) amorphous phase under geochemical conditions representative for the direct disposal of spent nuclear fuel in Boom Clay .......... 197 Contents VII Ulrich Noseck, Thomas Brasser, Ales Laciok, Mirek Hercik, Frantisek WoHer Uranium rnigration in argillaceous sediments as analogue for transport processes in the far field of repositories (Ruprechtov site, Czech Republic) ...................... 207 Klaus-Peter Seiler, Wolfgang Graf, Hans Lang, Reinhard Zapata Groundwater flow systems and the export of uranium from nuclear waste repositories to the biosphere ................................................................................ 217 Urho J. Suksi, Kari Rasilainen, Timo Ruskeeniemi, Nuria Marcos, Karl-Heinz Hellmuth NaturalU occurrences as a palaeo-hydrogeological indicator-observations from the Palmottu natural analogue site, Finland ......................................................... 227 Xueshi Lu, Yanxin Wang, Pingan Luo, Xiaobin Li and Xiaoqi Zhang Calculation of radioactive field in nuclear accident contaminated area from data acquired in aerial survey ...................................................................................... 23 7 Konstantin Yefimov, V.N. Chemonozhkin, Sergey Dmitriev, Lev Prozorov, Aleksey Tkachenko Experimentallarge diameter well in the clays for radioactive waste Repository 247 Jordi Bruno, Lara Duro, Esther Cera and Mireia Grive Redox processes in uranium deposits-Lessons from Natural Analogue Studies255 Broder Merkel Flooding of the Königstein uranium mine -Aquifer reactivity versus dilution ... 263 Sabine M. Spiessl, Henning Prommer, Martin Sauter, Chunmiao Zheng Numerical simulation ofuranium transport in flooded underground mines ........ 273 FrankWinde Stream pollution by adjacent tailing deposits and fluvial transport of dissolved uranium -dynamics and mechanisms investigated in rnining areas of Germany, Southem Africa and Australia ............................................................................. 283 Robert A. Fjeld, John T. Coates, Alan W. Elzerman, and James D. Navratil Mobilities ofuranium species in sedimentary interbed from the Snake River Plain ..................................................................................................................... 293 Yanxin Wang, Teng Ma, Leehang Xu A 3-D numerical modeling ofreactive transport ofU(VI) in shallow groundwaters: a case study at a uranium mill tailing site in southem China ....... 303 Jan Novak, Jii'i M11Zak Flooding of the deep uranium mine Hamr I by free water from tailings pond .... 311 VIII Contents Hana Cermäkova, Jan Novak, Jii'i Ml1Zäk Application of numerical simulation system on Turonian aquifer remediation control ................................................................................................................. 319 Andre Grigoriev, Alexei Marchenko Factors controlling migration and concentration of natural and technogerne radionuclides in bottom sediments ofthe Bastern Gulf ofFinland, Baltic Sea ... 327 P. G6mez, A. Garral6n, B. Buil and L. Sanchez Geochemical processes related to uranium mobilisation on groundwaters in a restored uranium mine ......................................................................................... 333 Christian Ekberg Uncertainties in Chemical Calculations .............................................................. 343 G. Meinrath, B. Merkel, P. Schneider, B. Delakowitz The Role ofMetrology and Statistics in Making Geochemical Modeling Defensible ........................................................................................................... 351 Leopold Vrankar, Goran Turk, Franc Runovc The Influence of Geostatistical Data on the ReHability of the Meshless Method in Transport Modeling ............................................................................................. 359 G. Geipel, G. Bernhard, V. Brendler Complex Formation ofUranium(IV) with Phosphate and Arsenate ................... 369 Maria Betti, Laura Aldave de las Heras, Lorenzo Pema, Fabio Bocci, Tania Huber Hyphenated techniques for speciation ofUranium and other actinides .............. 377 MarcusAmme Raman microspectrometric investigations ofU0 alteration products: Natural 2 analogues to alpha radiolysis effects ................................................................... 385 Marcus Walter, Thuro Amold, Harald Funke, Tobias Reich, Gert Bernhard Sorption ofUranium(VI) onto Schwertmannite-EXAFS investigations ........... 395 Harald Zänker, Wolfgang Richter, Gudrun Hüttig, Henry Moll Colloid-bome Uranium in Mine Waters .............................................................. 399 Silvia Jahn, Michael Paul, DelfBaacke Contaminant Release and Carbonate Availability ofSulphide-Bearing Waste Rock derived from Long-term Column Tests ............................................................... 407 Contents IX Katja Schmeide, Gerhard Geipel, Dietmar Keil, Klaus Jansen, Dirk Praschak, Karl Heinz Reise, Gert Bernhard Separation ofuranium from aqueous solution by textile bound calixarenes 000000.417 Evelyn Krawczyk-Bärsch, Thuro Arnold, Nils Schmeißer, Felix Brandt, Dirk Bosbach and Gert Bernhard The effect of chlorite dissolution on the sorption behavior ofU(VI) Ooooooooooooooooo.425 Vadim Shakhverdov Major factors of processes forming uranium ore in exogenetic epigenetic deposits ofthe Chu-Sarysu Province (Southern Kazakhstan) oooooooooooooooooooooooooooooooooooooooooo.431 Wemer Lutze, Weiliang Gong, and Ho Eric NuttaU Microbially mediated reduction and immobilization ofuranium in groundwater437 Arokiasamy Jo Francis Microbial Transformations ofUranium Complexed with Organic and Inorganic Ligands ooooooooooooooo 0000000000000 000000000 00 ooooooooooooooooooooooooooooooooooooooooo ooooooooooooooooooooooooo 00 ooooo 44 7 Sonja Selenska-Pobell, Katrin Flemming, Tzvetelina Tzvetkova, Johannes Raff, Michaela Schnorpfeil, Andrea Geißler Bacterial communities in uranium mining waste piles and their interaction with heavy metals 0000000000000 00 000000000000000 00 0000000000000000000000 00 0000000000000 00000000000000000 oo 00 00 ooooooooooo 04 55 Ho Vandenhove, Mo V an Hees Phytoextraction for clean-up oflow-level uranium contaminated soil evaluated465 Carsten Brackhage, Eo Gert Dudel Long-term differences in transfer and accumulation ofpotentially toxic trace elements and radionuclides in trees on uranium rnining dumps (Erzgebirge, Germany)ooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooooo471 Alexandru Cecal, Karin Popa, Ioan Caraus, lftimie Craciun Uranium and thorium uptake on hydrophilic plants ooooooooooooooooooooooooooooooooooooooooooo.479 Holger Dienemann, Carsten Brackhage, Anja Dannecker, Eo Gert Dudel, Joachim Rotsehe Soil formation and quality on uranium mining dumps depending on different tree species under special consideration of selected radionuclide contarnination 0000 0.489 Margarete Kalin, Martin P 0S rnith and Mark Bo Wittrup Ecosystem restoration incorporating rninerotrophic ecology and Stoneworts that accumulate 22~ 000 0000000 00000000000 ooooooooooooooooooooooooooooooooooooooooooooooooo ooooooooooooo 000000 00000000 495 X Contents M. Merroun, C. Hennig, A. Rossberg, T. Reich, R. Nicolai, K-H. Heise, S. Selenska-Pobell Characterization ofuranium (VI) complexes formed by different bacteria relevant to uranium mining waste piles ............................................................................. 505 Alix Günther, Gert Bernhard, Gerhard Geipel, Andre Rossberg, Tobias Reich Uranium speciation in plants ............................................................................... 513 Gerhard Gramss, Klaus-Dieter Voigt, Hans Bergmann Mobilization ofhazardous metals by plants growing in soils from uranium mining ................................................................................................................. 521 Heiko Schönbuchner, Mattbias Leiterer, Bemd Machelett, Hans Bergmann Mobility and plant availability ofheavy metals in soils ofuranium mining dumps529 Astrid Koban, Gerhard Geipel, Gert Bernhard, Thomas Fanghänel Complex Formation ofUranium(VI) with Glucose I-Phosphate ........................ 537 Donald R. Metzler, Kenneth E. Karp Performance report on the operations of a pilot plant for the treatment of vanadium in ground water-New Rifle UMTRA Site, Rifle, Colorado, USA ... 541 Henk Coetzee, Stephane Chevrel & Francis Cottard Inter-disciplinary sturlies ofthe impact of gold and uranium mining in the Witwatersrand Goldfield ..................................................................................... 553 Dirk Mallants, Ludo Diels, Leen Bastiaens, Johan Vos, Hugo Moors, Lian Wang, N orbert Maes, and Bildegarde Vandenhove Removal of uranium and arsenic from groundwater using six different reactive materials: assessment ofremoval efficiency ....................................................... 561 Christoph Klinger, Ulf Jenk, Jochen Schreyer Processes in passive mine water remediation with zero-valent iron and Iignite as reactive materials ................................................................................................. 569 C. Noubactep, G. Meinrath, P. Volke, H.-J. Peter, P. Dietrich, B. Merkel Mechanism ofUranium Fixation by Zero Valent Iron: The Importance ofCo- precipitation ......................................................................................................... 577 Margarete Kalin, Gunter Kießig, Annette Küchler Ecological water treatment processes for underground uranium mine water: Progressafter three years of operating a constructed wetland ............................. 587
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