Super-radiance Multiatomic Coherent Emission Optics and Optoelectronics Series Series Editors: E R Pike frs, B E A Saleh and S Lowenthal Other books in the series Aberrations of Optical Systems W T Welford Cutting and Polishing Optical and Electronic Materials G W Fynn and W J A Powell Ferroelectric Crystals for Laser Radiation Control A M Prokhorov and Yu S Kuz’minov The Fabry-Perot Interferometer J M Vaughan Infrared Optical Fibers T Katsuyama and H Matsumura Interferometry of Fibrous Materials N Barakat and A A Hamza KDP-Family Single Crystals L N Rashkovich Laser Analytical Spectrochemistry edited by V S Letokhov Laser Heating of Metals A M Prokhorov, V I Konov, I Ursu and I N Mihailescu Laser Picosecond Spectroscopy and Photochemistry of Biomolecules edited by V S Letokhov Laser Resonators and the Beam Divergence Problem Y A Anan’ev The Optical Constants of Bulk Materials and Films - 2nd Edition L Ward Physics and Chemistry of Crystalline Lithium Niobate A M Prokhorov and Yu S Kuz’minov Prism and Lens Making F Twyman Waves in Focal Regions J J Stamnes Optics and Optoelectronics Series Super-radiance Multiatomic Coherent Emission M G Benedict Attila Jozsef University, Szeged, Hungary A M Ermolaev University of Durham, UK Université Libre de Bruxelles, Belgium V A Malyshev Vavilov State Optical Institute, St Petersburg, Russia I V Sokolov St Petersburg State University, St Petersburg, Russia E D Trifonov Russian Herzen University, St Petersburg, Russia Published in 1996 by Published in Greai Bniain by Taylor & Francis Group Taylor & Francis Group 270 Madison Avenue 2 Park Square New York. NY 10016 Milion Park. Abingdon Oxon OX14 4RN © 1996 by Taylor & Francis Group. LLC No claim lo origmai U.S. Government works 1 0 9 8 7 6 5 4 3 Inieraational Standard Book Number-10; 0-7503-0283-6 (Hardcover) Internationa] Standard Book Number-13: 978-0-7503-0283-8 (Hardcover) Library of Congress catalog number 96-3 I 132 Thi^ book contain^ information obtained from authentic and highly regarded sources. Repnnted materiai ib quoted with permission, and sources are indicated. A wide vanety of references are listed. Reasonable efforts have been uiade to publish reliable data and information, but the author and the publisher cannot assume responsibility foi the validity of all maienals or for the consequences of their use. No part of this book may be repnnted. reproduced, transmitted, or utilized in any form by any electronic, mechanical, or other means, now known or hereafter invented, including photocopying, microfilming, and recording, or in any mlormation storage or retrieval system, without written permission from the publishers. Trademark Notice: Product or corporate names may be trademarks or registered trademarks, and are used only for identification and explanation without intent to infringe. Library of Congress Cataloging-in-Publication Data Catalog record is available from the Library of Congress Visit the Taylor & Francis Web site at informa http://www.tayiorandfrancis.com Taylor & Francis Group is the Academic Division of Informa pic To the memory of Maria Ivanovna Petrashen an outstanding scientist, teacher and personality Contents Preface xi Introduction 1 The elementary theory of super-radiance 5 1.1 Cooperative spontaneous emission of two two-level atoms separated by a distance less than the wavelength 5 1.2 Super-radiance of a system of N two-level atoms in a small volume: the Dicke model 10 1.3 Photon statistics of super-radiance in the Dicke model 18 1-4 Semiclassical theory of super-radiance of an extendeds ystem 24 1.5 Solution of the Maxwell-Bloch equations for super-radiance 32 1.6 Concluding remarks 37 The observation of super-radiance 38 2.1 Super-radiance in gases 38 2.2 Observation of super-radiance in solid-state materials 59 2.3 Concluding remarks 70 Quantum electrodynamical approach 72 3.1 Formulation of the problem 73 3.2 Diagram method of non-stationary perturbation theory 74 3.3 The spontaneous decay of a single two-level atom 78 3.4 The interaction of two-level atoms via the transverse electromagnetic field 84 3.5 Super-radiance of two two-level atoms 91 3.6 Super-radiance by extended polyatomic systems 99 3.7 Angular correlation of photons in super-radiance 110 Quantum fluctuations and self-organization in super-radiance 114 4.1 Quantum Maxwell-Bloch equations, Heisenberg picture 114 4.2 The initial conditions for the quantum Maxwell-Bloche quations 118 4.3 Averaging over semiclassical solutions 120 4.4 Statistical characteristics of super-radiance 122 4.5 Self-organization in super-radiance 128 Vll vili Contents The semiclassical theory 131 5.1 The equations of the model 131 5.2 Transition to amplified spontaneous emission 134 5.3 Area theorem and self-induced transparency 137 5.4 Linear régime of coherent amplification 140 5.5 Linear régime of super-radiance 146 5.6 Threshold condition and induced super-radiance 151 5.7 Solution of the nonlinear problem 153 5.8 Cooperative Raman scattering 157 5.9 Lasing without inversion 162 5.10 Concluding remarks 165 The influence of dipole-dipole inter-atomic coupling upon super-radiance 166 6.1 Preliminary remarks 166 6.2 Dipole-dipole interaction in the semiclassical theory 168 6.3 Quantum theory of super-radiance from a regular short linear chain of two-level atoms 182 6.4 Concluding remarks 189 7 Super-radiance of multi-spin systems 190 7.1 Preliminary remarks 190 7.2 Experimental observations of super-radiance of multi-spin systems in a cavity 191 7.3 Theory of super-radiance of proton multi-spin systems in a cavity 194 7.4 Comparison with NMR super-radiance experiments 203 7.5 Concluding remarks 206 8 Effects of diffraction upon super-radiance 207 8.1 Two-dimensional super-radiance 207 8.2 Super-radiance of a ‘sheet of paper’ volume 219 8.3 Concluding remarks 223 9 Reflection and transmission on the boundary of a resonant medium 225 9.1 Integral equation for the propagation problem without SVEAS 226 9.2 The linear and stationary régime: Fresnel’s formulae 229 9.3 Cooperative transient properties of a resonant thin layer 231 9.4 Nonlinear transient reflection from the boundary of an extended medium 241 9.5 Internal reflection in an inverted medium: correlation of forward-backward super-radiance pulses 246 10 Resonant boundary value problem with local field effects 250 10.1 The modified Maxwell-Bloch equations with the local field correction 251 Contents IX 10.2 Local field correction and the linear resonant refractive index 253 10.3 Nonlinear transmissiona nd mirror-less bistability 254 10.4 The local field correction for a thin layer: microscopic derivation 263 10.5 Concluding remarks 266 11 New sources and applications of super-radiance 268 11.1 High-gain super-radiant régimes in FEL 268 11.2 Gamma-ray super-radiance 273 11.3 Recombination super-radiance in semiconductors 275 11.4 Sub-radiance 277 11.5 Experimental observation of super-radiance and SBR of two trapped ions 279 11.6 Super-radiance and non-classical light 282 Super-radiance references and further reading 285 Other references 319 Index 323