STRONG INTERACTIONS IN LOW DIMENSIONS Physics and Chemistry of Materials with Low-Dimensional Structures VOLUME 25 Editor-in-Chief F. LÉVY, Institut de Physique Appliquée, EPFL, Département de Physique, PHB-Ecublens, CH-1015 Lausanne, Switzerland Honorary Editor E. MOOSER, EPFL, Lausanne, Switzerland International Advisory Board J. V. ACRIVOS, San José State University, San José, Calif., U.S.A. R. GIRLANDA, Università di Messina, Messina, Italy H. KAMIMURA, Dept. of Physics, University of Tokyo, Japan W. Y. LIANG, Cavendish Laboratory, Cambridge, U.K. P. MONCEAU, CNRS, Grenoble, France G. A. WIEGERS, University of Groningen, The Netherlands The titles published in this series are listed at the end of this volume. STRONG INTERACTIONS IN LOW DIMENSIONS Edited by D. Baeriswyl Department of Physics, University of Fribourg, Fribourg, Switzerland and L. Degiorgi Solid State Physics Laboratory, ETH Zürich, Switzerland KLUWER ACADEMIC PUBLISHERS DORDRECHT / BOSTON/ LONDON A C.I.P. Catalogue record for this book is available from the Library of Congress. ISBN 1-4020-1798-7 (HB) ISBN 1-4020-3463-6 (e-book) Published by Kluwer Academic Publishers, P.O. Box 17, 3300 AADordrecht, The Netherlands. Sold and distributed in North, Central and South America by Kluwer Academic Publishers, 101 Philip Drive, Norwell, MA02061, U.S.A. In all other countries, sold and distributed by Kluwer Academic Publishers, P.O. Box 322, 3300 AHDordrecht, The Netherlands. Printed on acid-free paper All Rights Reserved ©2004 Kluwer Academic Publishers No part of this work may be reproduced, stored in a retrieval system, or transmitted in any form or by any means, electronic, mechanical, photocopying, microfilming, recording or otherwise, without written permission from the Publisher, with the exception of any material supplied specifically for the purpose of being entered and executed on a computer system, for exclusive use by the purchaser of the work. Printed in the Netherlands. TABLE OF CONTENTS Chapter 1 – Introduction Strong interactions in low dimensions: introductory remarks 1 D. Baeriswyl and L. Degiorgi [email protected], [email protected] Chapter 2 Dynamic correlations in quantum magnets 21 C. Broholm and G. Aeppli [email protected], [email protected] Chapter 3 Angle resolved photoemission in the high temperature superconductors 63 J.C. Campuzano [email protected] Chapter 4 Luttinger liquids: the basic concepts 93 K. Scho¨nhammer [email protected] Chapter 5 Photoemission in quasi-one-dimensional materials 137 M. Grioni marco.grioni@epfl.ch Chapter 6 Electrodynamic response in “one-dimensional” chains 165 L. Degiorgi [email protected] v vi Strong interactions in low dimensions Chapter 7 Optical conductivity and correlated electron physics 195 A.J. Millis [email protected] Chapter 8 Optical signatures of electron correlations in the cuprates 237 D. van der Marel [email protected] Chapter 9 Charge inhomogeneities in strongly correlated systems 277 A.H. Castro Neto and C. Morais Smith [email protected], [email protected] Chapter 10 Transport in quantum wires 321 A. Yacoby [email protected] Chapter 11 Transport in one dimensional quantum systems 347 X. Zotos and P. Prelovˇsek xenophon.zotos@epfl.ch Chapter 12 Energy transport in one-dimensional spin systems 383 A.V. Sologubenko and H.R. Ott [email protected], [email protected] Chapter 13 Duality in low dimensional quantum field theories 419 M.P.A. Fisher [email protected] Subject Index 439 Materials Index 441 Chapter 1 STRONG INTERACTIONS IN LOW DIMENSIONS: INTRODUCTORY REMARKS D. Baeriswyl D´epartement de Physique, Universit´e de Fribourg, P´erolles, CH-1700 Fribourg, Switzerland. [email protected] L. Degiorgi Laboratorium fu¨r Festko¨rperphysik, ETH Zu¨rich, CH-8093 Zu¨rich, Switzerland. [email protected] The physical properties of low–dimensional systems have fascinated researchersforagreatpartof thelastcentury, andhaverecently become one of the primary centers of interest in condensed matter research. At the beginning, this field appeared much more like a playground for cre- ative theorists than a serious domain of solid–state physics. In fact, the exact treatment of the one–dimensional Lenz–Ising model and Bethe’s ingeniousdiagonalization oftheantiferromagneticHeisenbergchainwere considered at most as firststeps towards a theory of electronic and mag- neticpropertiesofreal,three–dimensionalcrystals. Similarly,Tomonaga presented his study of sound waves in a one–dimensional system of in- teracting fermions as mathematically interesting but physically not very useful. Acollection ofimportantearlydevelopments hasbeenassembled andcommenteduponbyLiebandMattis[1], whoemphasizedthatwhile exact solutions of one–dimensional models provide useful tests for ap- proximate methods, “in almost every case the one–dimensional physics is devoid of much structure, and describes a colorless universe much less interesting than our own”. This point of view was based on the observation that “in one dimension bosons do not condense, electrons do not superconduct, ferromagnets do not magnetize, and liquids do not freeze”. Fortunately, it has since been demonstrated that the one– 1 D. Baeriswyl and L. Degiorgi (eds.), Strong Interactions in Low Dimensions, 1–19. © 2004 by Kluwer Academic Publishers, Printed in the Netherlands. 2 Strong interactions in low dimensions dimensionalworld has its own richness, and thatthere arereal materials which to a good approximation may be considered as consisting of un- coupled chains, at least for temperatures or frequencies which are not too low. Some of the specific features predicted for interacting one– dimensional electron systems, such as charge– and spin–density waves, haveindeedbeenobserved inmanyquasi–one–dimensional materials [2], and under particular circumstances, such as Fermi–surfacenesting,can also be found in higher dimensions. In this book we attempt to convey the colorful facets of condensed matter systems with reduced dimensionality. We are of course aware of the fact that many important aspects must be left aside in such a collection of specific subjects; some of the most regretful omissions will be mentioned later. The following introductory remarks are intended as an aid to identifying some of the essential concepts which will reappear at several places in the subsequent chapters. At the same time this introductionmayhelptoconnectthedifferenttopicstreatedinthebook, some of which might at first sight appear rather disparate. 1. Ordering in low dimensions Inourthree–dimensionalworldweareaccustomedtothespontaneous appearance of order at sufficiently low temperatures. Liquids condense to form periodic solids, magnetic moments are aligned in ferromagnetic orantiferromagneticconfigurations,andFermiliquidsturnintosuperflu- ids. Atzerotemperaturethestateoflowestenergydeterminesthestable configuration of a system, but at finite temperatures it is the minimum of the free energy which determines whether the order parameter – the magnetization in a ferromagnet, the condensate fraction in a superfluid or the intensity of Bragg peaks in a periodic solid – remains finite or is completely suppressed due to thermal fluctuations. The destabilizing effects of temperature are particularly strong in one dimension. While in two or higher dimensions the Ising model exhibits long–range order below a finite critical temperature, this is no longer true in one dimen- sion, where thermal fluctuations destroy the spin correlations beyond a finite correlation length. These fluctuations are even more effective in the case of a continuous order parameter. Thus, according to the Mermin–Wagner theorem, the classical two–dimensional XY model has no true long–range order at finite temperatures [3]. Nevertheless this model – which can be used for representing the phase fluctuations of a complex order parameter or the spin configurations in an easy–plane Heisenberg ferromagnet – shows a transition from a disordered high– temperature phase with exponentially decaying correlations to a phase Strong interactions in low dimensions: introductory remarks 3 withquasi–long–range order below theKosterlitz–Thouless temperature T . The appropriate quantity describing this transition is the phase KT stiffness or superfluid density, which is finite below T and shows a KT universal discontinuity at T [4]. KT At zero temperature classical spin models on a bipartite lattice have long–range order, but this is not necessarily true for the corresponding quantummodels. Thusforboththespin–1 quantumXYandHeisenberg 2 modelsthespincorrelationsdecayalgebraically, andeventheIsingchain becomes disordered under a sufficiently strong transverse field. The latter case is very illuminating [5, 6] as the external field allows one to drivethesystemthroughaquantumcritical point,asecond–orderphase transition at T = 0 where quantum fluctuations are relevant [7]. For dimensions higher than 1 the quantum XY model has long–range order for all values of the spin, at least on a hypercubic lattice [8]. This result has also been proven for the quantum Heisenberg antiferromagnet for 3 or higher dimensions (and any spin) [9]. For dimension D=2 a rigorous proof still seems not to be available for S = 1, but both numerical 2 simulations and analytical calculations indicate that long–range order does exist, albeit with a reduced moment [10]. Low–dimensional systems not only experience strong quantum and thermal fluctuations, but also admit ordering tendencies which are diffi- cult to realize in three–dimensional materials. Prominent examples are spin– and charge–density waves in quasi–one–dimensional organic com- pounds and spontaneous circulating currents (leading to “orbital anti- ferromagnetism”) in two dimensions. The competition among several possibleorder parameters leads to rich phase diagrams and an enhanced sensitivity to disorder or applied external fields. Some of these order parameters are very difficult to observe directly. As an example, while phases with spontaneous spin or charge currents around the plaquettes of a square lattice occur naturally in models of interacting fermions in twodimensions[11], theirunambiguousdetection appearstobeverydif- ficult. Thus it is at present not clear whether the so–called “pseudogap phase” in the layered cuprates is related to such a hidden order para- meter [12]. 2. Dimensional crossover A real material is not truly one–dimensional (1D), butat most quasi– one–dimensional, i.e. a collection of weakly coupled chains. (Notable exceptions include quantum wires and nanotubes.) Thus one of the important questions will be the extent to which the coupling between chains is relevant. Anillustrative exampleis theIsingmodelon asquare