XA9949996 IAEA-TECDOC-1083 Status of liquid metal cooled fast reactor technology ^yi^p INTERNATIONAL ATOMIC ENERGY AGENCY ft 3 0 - 22 April 1999 V The originating Sectiof noth is publicae tIihAot nEnsia Aw Nuclear Power Technology Development Section International Atomic Energy Agency Wagramer Stras5se 001 xoB OP A-1400 Vienna, Austna e hTIAEA doest on normally maintain stocksf o reportsn i this series However, copies of these reports on microfiche or in electronic form can be obtained from INIS Clearinghouse International Atomic Energy Agency Wagramer Strasse5 PO Box 100 A-1400 Vienna, Austria E-mail: CHOUSE® IAEA.ORG URL http://www taea org/programmes/inis/mis htm Orders should be accompanied by prepayment of Austrian Schillings 100,- m the form of a cheque or in the form of IAEA microfiche service coupons e orbde ryeda swmehpicah ratele yIN hfIrSotm Clearinghouse STATF ULOSIQ UID METAL COOLED FAST REACTOR TECHNOLOGY IAEA, VIENNA, 1999 IAEA-TECDCC-1083 ISSN 1011-4289 ©IAEA, 1999 Pre inIhAtt eyEbd nA Ai ustna April 1999 FOREWORD In 1985 the International Atomic Energy Agency published a report entitled "Status of Liquid Metal Cooled Fast Breeder Reactors" (Technical Reports Series No. 246). It was a general reviee whts fot atusf o fast reactor development ta that time, covering some aspectsfo designd na operationd na reviewing experience frome ht earliest days.t I summarizedeht programmes and plans in all countries which were pursuing the development of fast reactors. Durin eghtp eriod 1985-1998, there have been substantial advancen si fast reactor technology development. Chief among these has been the demonstration of reliable operation by several prototypes dna experimental reactors,e ht reliable operationf o fuela ta high bumup (BN- 600, BN-350, Phenix, PFR BOR-60, FFTF). Some additional countries, such as China, India and the Repubf lKoic orea have launw cfhaesentd reactor prograe mIhAtmE teAAs .meetinnogs liquid metal cooled fast reactor (LMFR) technology,t i became evident that there have been significant technological advances as well as changes in the economic and regulatory environment since 1985. Therefore, the International Working Group on Fast Reactors (IWGFR) has recommended the preparation of a new status report on fast reactor technology. The present status report inte onpdtrso vide comprehed dnnesitavaie led informnatoion LMFR technoloe nhgfopToyrc . sauics tical issues te hruaast eo futel ngineers, scientists, managers, university students and professors, on the following topics: experience in construction and operation, reactor phd ysnsaaifcest y, core structural mad tfenuraeial ltechnology, fast reactor engineering and activities in progress on LMFR plants. This report has been prepared with contributions from China, France, Germany, India, Japan, the Russian Federation, the United Kingdom and the United States of America. The responsible IAEA officer was A. Rinejski of the Division of Nuclear Power. The IAEA expresses its appreciation to all those who have participated in the preparation of this reference compilation and also to the Member States that have made available experts to asd spnisaatr ticipan tteih is work. EDITORIAL NOTE In preparing this publication for press, staff of the IAEA have made up the pages from the original manuscripts). The views expressed do not necessarily reflect those of the IAEA, the governments of the nominating Member States or the nominating organizations. Through eohtutetx t namf oeMs ember Stae rtreaes tains eatdh ey were whe shetatenw xt compiled. The seuo f particular designations of countrier sot erritories doet onsi mpy jlnayu dgemeehtn ybt e lhegta pl ousbttf ale osi tsuIsuhAhcs ateEhrA ,c ,ounr ttroeierrs itof roitehse ,ir authdonritaies instie tduhetir ltooiom nfs itation of their boundaries. The mention of names of specific companies or products (whether or not indicated as registered) doet osni mpy lniyan tention oti nfringe proprietary rightr sosn, houe lbcd tio nstrun eae dsan dorsement r roecommende pahatt irnoe toInh A otfE A. CONTENTS CHAPT. 1ER BACKGD ROOVNUEANRDV IEW..........................................................................................1... . 1.1. Progress within the period 1985-1998................................................................................................................ 1 1.1.1. Demonstration reactor operation.............................................................................................................1 1.1.2. Prototype reactor operation....................................................................................................................1.. 1.1.3. Technical achievements...........................................................................................................................2 1.1.4. Design advances....................................................................................................................................... 3 1.2. Contenf ttosh is report.........................................................................................................................................4. CHAPTER 2. OPERATION EXPERIENCE WITH PROTOTYPE AND DEMONSTRATION LMFRs........................................................................................................... 5 2.1. BN-350 operating experience.............................................................................................................................. 5 2.1.1. Design features......................................................................................................................................... 5 2.1.2. Operating experience...............................................................................................................................7 2.1.3. Safety enhancement and equipment life extension................................................................................ 21 2.1.4. Review of experimental programme...................................................................................................... 22 2.2. Phenix operating experience..............................................................................................................................23 2.2.1. Design features.......................................................................................................................................23 2.2.2. Operating experience.............................................................................................................................25 2.2.3. Statutory inspection - Spring 1989........................................................................................................ 26 2.2.4. Inspections and maintenance during the test period (1991-1993)........................................................ 28 2.2.5. Negative reactivity shutdown.................................................................................................................29 2.2.6. Plant statistics........................................................................................................................................92. 2.2.7. Radiological safety................................................................................................................................. 30 2.3. PFR operational experience............................................................................................................................... 30 2.3.1. Design features.......................................................................................................................................30 2.3.2. Review of operating history................................................................................................................... 34 2.3.3. Advanced technology developments..................................................................................................... 52 2.3.4. PFR safety and licensing........................................................................................................................ 53 2.3.5. PFR and the fuel cycle........................................................................................................................... 55 2.3.6. The future............................................................................^ 2.3.7. PFR in perspective.................................................................................................................................58 2.4. Super Phen1 oipx erating experience...........................................................................................................9...5.. . 2.4.1. Design features..................................................................................................................................9..5.. . 2.4.2. Operating experience............................................................................................................................. 62 2.4.3. The present situation.............................................................................................................................. 71 2.5. BN-600 operation experience...........................................................................................................................2.7 2.5.1. Design features.......................................................................................................................................72 2.5.2. Operating experience.............................................................................................................................78 2.5.3. Radiological safety................................................................................................................................. 87 2.5.4. Fire safety, sodium leaks......................................................................................................................8.8. 2.5.5. BN-600 operating safety enhancement..............................................................................................9..8.. 2.5.6. Experimental programmes..................................................................................................................... 91 Bibliography....................................................................................................................................................... 92 CHAPTER 3. EXPERIENCE IN CONSTRUCTION AND PRE-OPERATION AL TESTING OF THE PROTOTYPE LMFRs.................................................................................... 95 3.1. Construction and pre-operational testing of the LMFR SNR-300.................................................................... 95 3.1.1. Introduction............................................................................................................................................95 3.1.2. Description.............................................................................................................................................95 3.1.3. Constructiond nap re-operational testing...............................................................................................99 3.1.4. Unexpected occurrences and their remedy.......................................................................................... 106 3.1.5. Achievements................................................................................................................................9..0..1... 3.1.6. Epilogue..........................................................................................................................................5.1..1.. 3.2. Construction and pre-operational testing of the prototype LMFBR "Monju"................................................ 117 3.2.1. Overviewf o project.............................................................................................................................711 3.2.2. Research and development.................................................................................................................. 118 3.2.3. Design and construction of monju....................................................................................................... 120 3.2.4. Pre-operational tests........................................................................................................................8.2..1.. References...............................................................................................................................................3...3..1... . CHAPT. 4ER LMFR PHYSICS ..............................................................................................................5...3....1..... . 4.1. Production of nuclear data for reactor neutronics calculations....................................................................... 137 4.1.1. Measurement fo esu eht dna nuclear theory........................................................................................731 4.1.2. Analysis................................................................................................................................................138 4.1.3. Compilation.......................................................................................................................................... 138 4.1.4. Evaluation............................................................................................................................................ 138 4.1.5. Nuclear data uncertainty information.................................................................................................9.31 4.1.6. Integral measurements....................................................................................................................0.4..1.. 4.1.7. Fission spectrum average....................................................................................................................04.1 4.1.8. Dosimetrycross-sections..................................................................................................................... 140 4.1.9. Nuclear data processing codes and group cross section data sets....................................................... 141 4.1.10. Validation............................................................................................................................................. 143 4.1.11. Uncertainties in reactor parameters caused by nuclear data uncertainties.......................................... 143 4.2. Energy production, radiation emission, induced radioactivity and irradiation damage.................................. 144 4.2.1. Heating................................................................................................................................................. 145 4.2.2. The radioactivity of irradiated fuel...................................................................................................... 147 4.2.3. Activatiof sont ructud crnoaalo lant materials................................................................................7.4..1.. 4.2.4. Irradiation damage effects and dosimetry............................................................................................ 148 4.3. Neutronics calculation methods....................................................................................................................... 149 4.3.1. Forms of heterogeneity........................................................................................................................ 150 4.3.2. Metr htoroedfas ting heterogeneity.............................................................................................1..5...1... . 4.3.3. Control rod homogenisation................................................................................................................ 152 4.3.4. Derivation of broad group cross-sections............................................................................................ 152 4.3.5. Whole reactor calculation methods...............................................................................................2..5..1.. 4.3.6. The sub-group treatment of resonance shielding................................................................................. 153 4.3.7. Perturbation theory methods......................................................................................................5...5...1... . 4.3.8. Methof daods justmf econrt oss-sect itinifo toengts ral measurements........................................5...5..1.. 4.3.9. Kinetics calculations...........................................................................................................................6.51 4.4. Computer codes used in fast reactor neutronics.............................................................................................. 157 4.4.1. Codes basedn o diffusion theory.........................................................................................................7.51 4.4.2. Transport theory and codes.................................................................................................................. 158 4.4.3. Codes based on the Monte Carlo method............................................................................................ 159 4.4.4. Application of code systems to fast reactor calculations..................................................................... 161 4.5. Validaf tmiooend tdhnaotada.s .............................................................................................................4..6...1... . 4.5.1. Effective multiplication of a core at start-up....................................................................................... 165 4.5.2. Variation of reactivity with bum-up.................................................................................................... 166 4.5.3. Incinerati ffooins sion products ..................................................................................................6..6...1... . 4.5.4. Power distributions........................................................................................................................7..6..1.. 4.5.5. Control rod reactivity worths............................................................................................................... 168 4.6. Reactivity coefficients...................................................................................................................................... 169 4.6.1. Doppler effects....................................................................................................................................07.1 4.6.2. Sodium voiding dnas odium density coefficients...............................................................................37.1 4.7. Shielding studies..............................................................................................................................................471 References...........................................................................................................................................5....7....1.... . Bibliography..................................................................................................................................................... 180 CHAPTER 5. LMFR SAFETY: NEW TRENDS AND FINDINGS................................................................... 185 w treeNndn 5si.sa1 f .ety principd glneoas als...................................................................................................5.8..1.. 5.1.1. LMFRs and main recent nuclear safety trends.................................................................................... 185 5.1.2. Safety fundamentals....................................................................................................................5..8...1... . 5.1.3. Risk minimization and accident analysis approaches consequences for LMFRs............................... 186 5.1.4. Localsubassemblyfaults...................................................................................................................4.9.1 5.1.5. Sodium fires......................................................................................................................................... 200 5.2. Emergency heat removal by natural and forced convection............................................................................ 205 5.2.1. Safety objectif veoems ergency heat removal systems (EHRS)..................................................5...0..2.. . 5.2.2. Main design concepts...........................................................................................................................205 5.2.3. Status of international R&D activities and future needs...................................................................... 219 5.2.4. General conclusions.............................................................................................................................220 References........................................................................................................................................................221 CHAPTER 6. SOME ASPECTS OF INSTRUMENTATION AND INSPECTION OF MAIN LMFR COMPONENTS.............................................................................................. 225 6.1. Steam generator: designs, instrumentd apntriooatne ction..............................................................................225 6.1.1. Configuration...................................................................................................................................5..2.2. 6.1.2. Construction.........................................................................................................................................232 6.1.3. Design details.......................................................................................................................................235 6.1.4. Protection.............................................................................................................................................237 6.1.5. Sodium-water reactionn ssi team generators....................................................................................9.3.2. 6.2. Reactor core with other components: acoustic instrumentation...................................................................... 249 6.2.1. Detection of boiling.............................................................................................................................249 6.2.2. Plant monitoring...................................................................................................................................252 6.3. Ultrasonic instrumentation............................................................................................................................... 255 6.3.1. Ultrasonic imaging...............................................................................................................................256 6.3.2. Ultrasonic monitoring..........................................................................................................................256 6.3.3. Ultrasonic measurement of temperature.............................................................................................. 259 6.3.4. Ultrasonic systems...............................................................................................................................259 6.4. In-service inspection and repair.......................................................................................................................259 6.4.1. Background..........................................................................................................................................262 6.4.2. Operational in-service inspection components.................................................................................... 262 6.4.3. Rd desenevaearlcoh pn mFreiann tce..................................................................................................264 References........................................................................................................................................................270 CHAPTE. 7R CORE STRUCTURAL MATED RFUNIAEALL TECHNOLOGY FOR HIGH BURN-UP..................................................................................... 273 7.1. Introduction......................................................................................................................................................273 7.2. Behaviour of materials for fuel pin cladding and subassembly duct (wrapper).............................................. 273 n c7il.aP2d.1d .ing materials..........................................................................................................................273 7.2.2. Wrapper-tube (duct) materials.............................................................................................................279 7.3. Irradiation performanf oocxe ide fuel elements........................................................................................0..8...2. . 7.3.1. Fuel and fission product behaviour......................................................................................................283 7.3.2. Mechanical interaction between fuel and cladding (FCMI)................................................................ 286 7.3.3. Chemical interaction between fuel and cladding (FCCI).................................................................... 286 7.3.4. Behaviour under off-normal conditions........................................................................................8..8...2. . 7.3.5. Fain lbeiped haviour............................................................................................................................290 7.3.6. Modellif noogx ide fuel performances ................................................................................................291 7.3.7. Achievable bum-up..............................................................................................................................291 7.4. Irradiation performaf mnocee tallic fuel elements..................................................................................2...9...2.. . 7.5. Irradiation performancf oae dvanced fuel elements....................................................................................4..9.2. 7.5.1. Carbide fuel elements...........................................................................................................................295 7.5.2. Nitride fuel elements............................................................................................................................299 7.5.3. Fr huoiefgl h plutonium burning....................................................................................................0..0..3.. 7.6. Irradiation performance of absorber elements................................................................................................. 307 References........................................................................................................................................................313 CHAPTERS. LMFR ENGINEERING.................................................................................................................317 8.1. Sodium pumps.................................................................................................................................................. 317 8.1.1. Design basis......................................................................................................................................... 317 8.1.2. Sodium pump design features..........................................................................................................9.1.3.. 8.1.3. Pump testing techniques....................................................................................................................... 336 8.1.4. Pump operating experience.................................................................................................................. 337 8.1.5. Cavitation snio dium pump impellers.............................................................................................0..4.3.. 8.1.6. Structural improvements in new sodium pump designs......................................................................343 8.2. Thermal-hydraulics of the primary circuit....................................................................................................... 351 8.2.1. Introduction..........................................................................................................................................351 8.2.2. Objectives of the thermal-hydraulic studies........................................................................................ 351 8.2.3. Steady state studiet ohp ehst foo olsf o pool-type reactors.................................................................2.53 8.2.4. Transient studiet oph sfoo ols.............................................................................................................26.3 8.2.5. Studies of the cold pool of a pool-type reactor.................................................................................... 363 8.2.6. Strongback..................................................................................................................................4...6...3.. . 8.2.7. Diagrid.................................................................................................................................................364 8.2.8. Gas entrainment at the free surface...................................................................................................... 365 8.2.9. Cover gas thermal-hydraulics.............................................................................................................. 366 8.2.10. Thermal stripping studies.....................................................................................................................366 8.2.11. Conclusions..........................................................................................................................................369 8.3. Decommissioning of the experimental liquid-metal fast reactor Rapsodie..................................................... 370 8.3.1. Introduction..........................................................................................................................................370 8.3.2. Main features of the installation........................................................................................................... 370 8.3.3. Pre-decommissioningoperations (1983-1985)...................................................................................372 8.3.4. Decommissioning operations (1986-1994).........................................................................................373 8.3.5. Conclusions..........................................................................................................................................378 References........................................................................................................................................................ 381 CHAPTER 9. ACTIVITIES IN PROGRESS ON LMFR PLANTS.................................................................... 385 9.1. European fast reactor.......................................................................................................................................385 Introduction..........................................................................................................................................385 Organizational e sEthruurtco ftpuoerae n fast reactor cooperation............................................5...8...3.. . .3. EFR programme status.........................................................................................................................386 .4. Main design features............................................................................................................................ 388 Ds&u.Rp5e pdh. toe frost ign..............................................................................................................6..0.4. Concept validation phase achievements...........................................................................8......0......4..... .. R pFroEe jse heucThct.tc. .ef.os..s ...............................................................................................5..1..4.. 9.2. BN-1600M.......................................................................................................................................................415 9.2.1. Stages of development and design concept evolution.........................................................................415 9.2.2. Basic paramd denetesairgs n optimization..........................................................................................416 9.2.3. Reactor unit design...............................................................................................................................420 9.2.4. Reactor plant safety..............................................................................................................................429 9.3. BN-800 reactor plant........................................................................................................................................431 9.3.1. Design status........................................................................................................................................ 431 9.3.2. Reactor design basis...................................................................................................................1...3...4... . 9.3.3. Reactor design concept........................................................................................................................431 9.3.4. Main design improvements and reactor plant features........................................................................ 433 9.4. BN-600M advanced LMFR............................................................................................................................. 445 9.4.1. Design status........................................................................................................................................445 9.4.2. Design basis.........................................................................................................................................449 9.4.3. Reactor design concept and main data.................................................................................................449 9.4.4. Safety features......................................................................................................................................451 9.4.5. Improvement of economic performance.............................................................................................. 452 9.5. The demonstration fast breeder reactor...........................................................................................................453 9.5.1. Introduction..........................................................................................................................................453 9.5.2. DFBR plant design...............................................................................................................................453 9.5.3. Techd necnicoaan lomic evaluation.....................................................................................................463 9.5.4. ProspectsR BF rof commercialization.................................................................................................468 9.5.5. Conclusion.......................................................................................................................................9.6..4. 9.6. Prototype fast breeder reactor-design description........................................................................................... 469 9.6.1. Introduction.......................................................................................................................................... 469 9.6.2. Reactor assembly................................................................................................................................. 469 9.6.3. Primary sodium system................................................................................................................5...7..4.. . 9.6.4. Secondary sodium systems............................................................................................................6..7..4.. 9.6.5. Fuel handling...................................................................................................................................6..7..4. 9.6.6. Decay heat removal..............................................................................................................................476 9.6.7. Materials..............................................................................................................................................67.4 9.6.8. Instrumentatiod ncna ontrol.................................................................................................................478 9.6.9. Fire protection......................................................................................................................................478 9.6.10. Containment.........................................................................................................................................479 9.6.11. Emergency control room .....................................................................................................................479 9.6.12. Balancf ope lant (BOP)........................................................................................................................479 9.6.13. Present status........................................................................................................................................479 9.7. ALMR technology development......................................................................................................................479 9.7.1. Introduction..........................................................................................................................................479 9.7.2. ALMR plant design..............................................................................................................................484 9.7.3. Integral fast reactor concept development........................................................................................... 501 9.8. BMN-170 modular fast nuclear reactor........................................................................................................... 510 9.8.1. Design goals and status........................................................................................................................510 9.8.2. Design basis...................................................................................................................................2..1..5.. 9.8.3. Reactor safety features......................................................................................................................... 515 9.8.4. Radiological safety......................................................................................................................7...1...5.. . 9.8.5. Economics............................................................................................................................................517 9.9. Experimental fast reactor CEFR-25.................................................................................................................518 9.9.1. Introduction.........................................................................................................................................^^ 9.9.2. Histod arncya hievements....................................................................................................................518 9.9.3. Trends of experimental reactors .......................................................................................................... 522 9.9.4. CEFR-25 design...................................................................................................................................522 9.9.5. Site work..............................................................................................................................................528 9.9.6. Nuclear licensing systen Cmi hina.................................................................................................9..2..5.. 9.9.7. Safety features......................................................................................................................................529 Bibliography.....................................................................................................................................................531 CHAP. T0E1SR UMD FMUNATRAUYR E TRENDS..............................................................................3...3...5.. . 10.1. Introduction......................................................................................................................................................533 10.2. Technology trends............................................................................................................................................533 10.2.1. Fast reactorss ab urnersf op lutonium................................................................................................533 10.2.2. Fast reac stionarcs ineraf tnoours clear waste....................................................................................536 10.2.3. Design styles......................................................................................................................................538 10.2.4. Safety.................................................................................................................................................. 539 e phroTgr1a0m.3 .me.......................................................................................................................................0...4...5.. . 10.4. Conclusion........................................................................................................................................................541 Contributors to drafting and review.............................................................................................................................543 Cha1pte r BACKGROUND AND OVERVIEW 1.1. PROGRESS WITE PHHEITNR IOD 198- 51 998 1.1.1. Demonstration reactor operation The outstanding success of the decade has undoubtedly been the reliable operation of the BN-600 pt lBs aabn enaoen ltpiooehn evjna Rare ariur sttasisk Iloslaina h.sin cde n19a80 , lifetime lon Ia1d9 .% 9t f2i aa2 7cc thfooire vea dl oad face htsf Toou8r c 3.c%.s5ea sws achieved in spite of a number of incidents including sodium fires. The effectiveness of the protective and remedial measures clearly demonstrates that a sodium-cooled fast reactor is capable of sustained reliable contribution to an electricity supply system. In Frane cShetu per Phenix plan taCt reys-Malvs isalwluec cessfully commissiondenad operated, but not without difficulty. Three incidents marked the commissioning procedure and caused lengthy delayn s1I. 987 ta hs seoarwde ium leak froe uhmts ed fuel storage drumn 1i, 990 there was an air leak into an auxiliary circuit which caused extensive pollution of the primary sodium,d na alson i 1990n a exceptional snow fall causede ht collapsee ht fo roofe ht fo turbine hall with extensive damage to the steam plant. Partly as a result of this experience the safety of the s ptalhawonr toughly revied wmneaodd ificatioo intms pre orhevtse pono sstee condary sodium fires were made. A public enquiry on renewal of the operating license was held and reported s prn e r apeor1oheial9swas di9fttntdy4ia tvrnets .al fyau T,rwhthise r dae lyaybed small leak of argon from the sealing bell surrounding one of the intermediate heat exchangers. Corrective action was taken and in the latter part of 1995 and through 1996 power was gradually raisee dht fot ull-power level. Later political changes called future operation into questiondna in February 1998 the French Government finally confirmed to discontinue its operation. 1.1.2. Prototype reactor operation In Germany construction foS NR-30s a0cw ompleted dcna ommissionins agsw uccessfully taken to an advanced stage. A small leak in a ferritic steel sodium dump tank was found, and ths easworem e poll euphttri oifmon ary sodiu ymmb oisture released from shielding material. Effective technical provisions to meet the extensive criticism of the safety of the plant were successfully put into place, but the project was eventually terminated for political reasons. The earlier problem fsos team lea ekhet snvi aporaR ptFPo lehart fsno ntiS cotland were successfully solved, but in 1987 there was a large leak in one of the superheaters. This gave rise to a major review of the protection against large sodium-water reactions. In 1991 the primary sodium was polluted by oil from one of the sodium pumps. These technical problems were overcome successfully, and in addition in 1990 an operating license (which hitherto had not been a legal necessity) was obtained from the safety authority after a review against the same criteria appliedo t commercial thermal reactors. Whes awfn tii nally shut downn i 19saw9 RF4P operating with good reliability. ehBTN-350 plann Kit azakhsts aaonhp erate roodfv 0ey2r ea ac dransa rs,o fefu ture operation has been made. Means of improving the protection of the plant against the effects of