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Spontaneous Emergence of Persistent Spin Helix from Homogeneous Spin Polarization Valeriy A. Slipko,1,2 Ibrahim Savran,3 and Yuriy V. Pershin1,∗ 1Department of Physics and Astronomy and USC Nanocenter, University of South Carolina, Columbia, SC 29208, USA 2 Department of Physics and Technology, V. N. Karazin Kharkov National University, Kharkov 61077, Ukraine 3Department of Computer Science and Engineering, University of South Carolina, Columbia, SC 29208, USA We demonstrate that a homogeneous spin polarization in one-dimensional structures of finite lengthinthepresenceofBychkov-Rashbaspin-orbitcouplingdecaysspontaneouslytowardapersis- tent spin helix. The analysis of formation of spin helical state is presented within a novel approach 1 based on a mapping of spin drift-diffusion equations into a heat equation for a complex field. Such 1 a strikingly different and simple method allows generating robust spin structures whose properties 0 can be tuned by the strength of the spin orbit interaction and/or structure’s length. We generalize 2 ourresultsfortwo-dimensionalcasepredictingformationofpersistentspinhelixintwo-dimensional n channels from homogeneous spin polarization. a J PACSnumbers: 72.15.Lh,72.25.Dc,85.75.2d 1 3 The helical wave of rotating spin orientation is re- mation of homogeneous spin polarization into the per- ] ferred to as the spin helix. There is a significant interest sistent spin helix occurs when we introduce boundary l l to spin helix configurations in semiconductor materials conditions on electron space motion to describe finite- a h since the electron spin relaxation of such spin configura- length structures (in infinite systems the homogeneous - tionscanbepartially[1–3]orevencompletelysuppressed spin polarization decays exponentially as predicted by s e [4, 5]. While a partial suppression of spin relaxation in D’yakonov-Perel’ theory [18]). Using a novel approach m two-dimensional systems becomes possible in the pres- thatmapsspindrift-diffusionequationsintoaheattrans- . ence of only Bychkov-Rashba [6] spin-orbit coupling (see fer equation for a complex field we find the exact time- t a Refs. [1, 2]), the complete suppression of spin relaxation dependenceofthespinpolarizationdynamics. Itisinter- m requires a specific combination of Bychkov-Rashba and esting that the amplitude of the resulting spin helix has - Dresselhaus [7] interactions as it was demonstrated in anoscillatorydependenceonthesystem’slength. Below, d Ref. [4]. More generally, the relaxation of the spin he- we provide an intuitive explanation of this result based n lix is an example of situations [1–5, 8–17] when electron on properties of solution of heat equation. Moreover, it o c spin relaxation scenario deviates from the predictions of is necessary to emphasize that our theory is generalized [ D’yakonov-Perel’ theory [18]. for the case of two-dimensional (2D) channels and can 1 Experimentally, the spin grating technique [19] is typ- be straightforwardly verified experimentally. In partic- v ular, experimentally, the homogeneous spin polarization ically used [3, 5] to create spin helical configurations in 9 canbeeasilycreatedusingtheopticalorientationbycir- semiconductors. In this method, a sample is illuminated 3 cularly polarized light. Therefore, we believe that our 0 byapairofpumpbeamswithorthogonallinearpolariza- approach would simplify tremendously the generation of 0 tions. Theinterferenceofsuchbeamsresultsinaspacial long-living spin helical configurations in semiconductor . modulation of light helicity. Correspondingly, through 2 structures and advance the field of spin storage in semi- 0 theopticalorientationeffect,amodulationofspinpolar- conductors. 1 izationintheformofspinhelixisproduced. Moreover,a 1 spin injection from a ferromagnetic material into a semi- : v conductor can also be used to excite a spin helix [20]. t =0 i Inthisapproach, therotatingspinpolarizationiscaused X by coherent spin precession of electrons drifting in an r a applied electric field. However, the present authors are notawareaboutanyexperimentalstudiesofspin helixes excited by spin injection. t →∞ In this Letter, we propose an alternative approach to induce spin helical configurations. Specifically, we demonstrate that in one-dimensional (1D) systems of fi- FIG. 1: (Color online) Schematics of spontaneous transfor- nitelengthwithBychkov-Rashbaspin-orbitcouplingthe mationofhomogeneousspinpolarizationintopersistentspin spin helical configurations emerge in the process of re- helixinafinitelengthsystemwithBychkov-Rashbaspin-orbit laxation of homogeneous spin polarization (see Fig. 1). coupling. Mathematically, such a strikingly unexpected transfor- 2 1.0 1.0 1.000 1.000 (a) (b) 0.7500 0.7500 0.8 0.8 0.5000 0.5000 ) ) L L of 0.6 0.2500 of 0.6 0.2500 nits 0 nits 0 u0.4 -0.2500 u0.4 -0.2500 n n x (i x (i 0.2 S /S 0.2 S /S z 0 x 0 0.0 0.02 0.04 0.06 0.08 0.10 0.02 0.04 0.06 0.08 0.10 Time (in units of L2/D) Time (in un its of L2/D) FIG. 2: (Color online) Dynamics of formation of persistent spin helix from homogeneous spin polarization pointing in z direction at t = 0. These plots were obtained using Eq. (13) at ηL = 15.45. This value of the parameter ηL corresponds to the second local maximum of spin helix amplitude shown in Fig. 3. Let us consider dynamics of electron spin polariza- of time the spin polarization is homogeneous and points tion in a 1D system of a length L in x direction in the in z direction, that is presence of Bychkov-Rashba spin-orbit coupling. In one- S (x,t=0)=0, S (x,t=0)=S . (5) dimensional limit, spin drift-diffusion equations [2] can x z 0 be written as Let us introduce a complex polarization S =S +iS . x z It is straightforward to show that Eqs. (1,3) and bound- ∂S ∂S x = D∆S +C z −2γS , (1) ary conditions (4) can be rewritten in a more compact ∂t x ∂x x form using S: ∂S y = D∆S , (2) ∂t y ∂S ∂2S ∂S =D −iC −2γS, (6) ∂∂Stz = D∆Sz−C∂∂Sxx −2γSz, (3) ∂t (cid:18)∂x2∂S ∂x(cid:19) 2D −iCS =0. (7) ∂x where D = (cid:96)2/τ is the coefficient of diffusion, ∆ = Γ ∂2/∂x2, C = 2ηD is the constant describing spin rota- Defining a complex field u(x,t) by the relation tions, γ =η2D/2 is the coefficient describing spin relax- u(x,t)=e−iηxS(x,t), (8) ation, η = 2αm(cid:126)−1 is the spin precession angle per unit length, α isthespin-orbitcouplingconstant, mistheef- we find that Eq. (6) transforms into the heat equation fectiveelectronmass,(cid:96)isthemeanfreepathandτ isthe ∂u ∂2u momentum relaxation time. It follows from Eq. (2) that =D , (9) y component of spin polarization, S , is not coupled to ∂t ∂x2 y anyothercomponentofspinpolarization. Consequently, supplemented by Neumann (or second-type) boundary selecting Sy(x,t=0)=0 we can safely take out Sy from conditions our consideration. Eqs. (1,3) are complimented by stan- (cid:18) (cid:19) ∂u dard boundary conditions [21] =0. (10) ∂x Γ Moreover, it is worth noticing that the initial conditions (cid:18) (cid:19) (cid:18) (cid:19) ∂S ∂S 2D x +CS =0, 2D z −CS =0. (4) for u(x,t) are related to the initial conditions for S as ∂x z ∂x x Γ Γ u(x,t=0)=e−iηxS(x,t=0). (11) Here, Γ = [x = 0,x = L]. Mathematically, the bound- Consequently, the initially homogeneous spin polariza- aryconditions(4)areso-calledthird-typeboundarycon- tion in z direction (Eq. (5)) corresponds to a spatially ditions. This specific form of boundary conditions con- modulated complex field servesthespinpolarizationofelectronsthatscatterfrom the sample edges. We assume that at the initial moment u(x,t=0)=S sin(ηx)+iS cos(ηx). (12) 0 0 3 The solution of Eq. (9) with the boundary condi- 1.0 tions (10) and initial condition (12) was obtained by the methodofseparationofvariables. Itcanbepresentedin S the form 0.8 x de x S S(x,t) =isin(ηL/2)eiη(x−L/2)+ itu x z S0 ηL/2 pl 0.6 m 2ηLeiηx(cid:88)+∞ 1(η−L()−21−)n(eπ−ni)η2Le−π2Ln22Dt cos(cid:16)πLnx(cid:17). (13) ix A 0.4 x n=1 el H This is our main analytical result describing dynamics n x of spin polarization in 1D finite-length structures. Note pi 0.2 S thatS andS componentsofspinpolarizationaregiven x z by real and imaginary parts of Eq. (13), respectively. 0.0 The first term in the right-hand side of Eq. (13) de- 0 5 10 15 20 25 30 η L scribes the persistent profile of spin polarization (in the form of spin helix) emerging at long times. Concerning FIG.3: (Coloronline)Normalizedamplitudeofthepersistent the second term in the right-hand side of Eq. (13), it spin helix as a function of ηL. Insets show schematically governs the dynamics of transformation of the initially distributions of S and S at several specific values of ηL as homogeneous spin polarization into the persistent spin x z indicatedbyarrows. Positionsofminimaandmaximapoints helix. Fig. 2 demonstrates dynamics of Sz and Sx com- of the amplitude are discussed in the text. ponents of spin polarization given by Eq. (13). It is clearlyseenthattheinitiallyhomogeneousspinpolariza- tion in z directions transforms into the persistent spin helix with an (infinitely) long lifetime. these times τ = L2/(π2D) provides the time scale of 1 Explicitly, in the long time limit, the spin polarization thetransformationprocess. Thedependenceofspinpro- is given by cess on L is intuitively clear as electrons should "feel" the system’s length before the transformation ends. It’s sin(ηL/2) Sx(x,t=+∞)=−S0 ηL/2 sin(η(x−L/2)), (14) alsointerestingthatsuchatimecanbelongerorshorter then the relaxation time of homogeneous spin polariza- Sz(x,t=+∞)=S0sinη(LηL/2/2)cos(η(x−L/2)). (15) tiniogntτhhat=τ1/<(Dτη2)w. hInenpaηrLtic<ulaπr,,tτh1e/τthim=es(ηaLr/eπt)h2emseaamne- 1 h when ηL = π, and τ > τ when ηL > π (see also Fig. In these equations the factor sin(ηL/2)/(ηL/2) defines 1 h 3). reduction of the spin helix amplitude with the respect to the initial amplitude of homogeneous spin polarization In order to obtain an additional insight on spin re- S . We plot this function in Fig. 3. It is interesting laxation of the radial spin helix, we have performed ex- 0 thatthespinhelixamplitudeisanoscillatingfunctionof tensive Monte Carlo simulations employing an approach the parameter ηL and takes zero values when ηL=2πn described in Refs. [8] and [22]. This Monte Carlo sim- wherenisapositiveinteger. Thepositionsoflocalmax- ulation method uses a semiclassical description of elec- ima can be found numerically. In particular, positions tron space motion and quantum-mechanical description of four local maxima shown in Fig. 3 are 8.987, 15.450, of spin dynamics (the later is based on the Bychkov- 21.808, 28.132. Rashba coupling term). All specific details of the Monte The heat equation is the best starting point to under- Carlosimulationsprogramcanbefoundinthereferences stand the oscillatory dependence of spin helix amplitude cited above and will not be repeated here. A spin con- on ηL depicted in Fig. 3. Accordingly to Eq. (11), the servationconditionwasusedforelectronsscatteringfrom initially homogeneous initial condition (Eq. (5) for spin system boundaries. Generally, all obtained Monte Carlo diffusion equations transforms into a modulated initial simulation results are in perfect quantitative agreement condition for the heat equation. As the solution of heat withouranalyticalpredictionsthusconfirmingthemech- equation in the given context represents simply the pro- anismofformationofpersistentspinhelixfromhomoge- cess of temperature equilibration along the system, an neous spin polarization. A comparison of selected ana- integer number of modulation periods results in zero av- lytical and numerical curves is given in Fig. 4. erage "temperature" and, correspondingly in zero spin The results reported in this paper can be readily gen- helix amplitude. Moreover, we would like to mention eralized for the persistent spin helix in two dimensions that the spin helix formation process is described by a [4]. Indeed, it can be easily seen that in the case of series of exponentially decaying terms whose time con- equalstrengthofBychkov-RashbaandDresselhausspin- stants are given by τ = L2/(π2n2D). The longest of orbit interactions, α = β (where β is the Dresselhaus n 4 trol of spin helix characteristics is achievable via appro- 0.3 Monte Carlo result priate choice of the above mentioned parameters. This Analytical result suggested technique facilitates generation of spin helical 0.2 statesandcanbeusedinbothone-andtwo-dimensional geometries. 0.1 I. S. acknowledges PhD scholarship from the Repub- S0 lic of Turkey Ministry of National Education, Grant No: S/z 0.0 [010] MEB1416. -0.1 [100] -0.2 ∗ Electronic address: [email protected] -0.3 1 Y. V. Pershin, Phys. Rev. B 71, 155317 (2005). 0.0 0.2 0.4 0.6 0.8 1.0 2 Y. V. Pershin and V. A. Slipko, Phys. Rev. B 82, 125325 x/L (2010). 3 C. P. Weber, J. Orenstein, B. A. Bernevig, S.-C. Zhang, FIG. 4: (Color online) Long-time distribution of S at ηL= J. Stephens, and D. D. Awschalom, Phys. Rev. Lett. 98, z 8.987 found employing Monte Carlo simulation approach. 076604 (2007). The analytical curve is obtained using Eq. (15). The Monte 4 B.A.Bernevig,J.Orenstein,andS.-C.Zhang,Phys.Rev. Carlo simulation was performed for 105 electrons in GaAs Lett. 97, 236601 (2006). structure of 1.7µm length. This plot obtained using the pa- 5 J. D. Koralek, C. P. Weber, J. Orenstein, B. A. Bernevig, rametervaluesτ =0.1ps,l=10nm,α=3·10−12eVm. Inset: S.-C.Zhang,S.Mack,andD.D.Awschalom,Nature458, orientation of 2D channel for two-dimensional spin helix ex- 610 (2009). citation experiments. 6 Y. Bychkov and E. Rashba, JETP Lett. 39, 78 (1984). 7 G. Dresselhaus, Phys. Rev. 100, 580 (1955). 8 A. A. Kiselev and K. W. Kim, Phys. Rev. B 61, 13115 (2000). 9 E. Y. Sherman, Appl. Phys. lett 82, 209 (2003). spin-orbit coupling constant), the equations of spin dif- 10 M.Q.Weng,M.W.Wu,andQ.W.Shi,Phys.Rev.B69, fusion in 2D [4] take the general form of Eqs. (1-3). 125310 (2004). Therefore,introducingappropriateboundaryconditions, 11 Y. V. Pershin and V. Privman, Phys. Rev. B 69, 073310 namely, reducing the system into a 2D channel in [-110] (2004). direction (see the inset in Fig. 4), we obtain the situa- 12 L. Jiang, M. Weng, M. Wu, and J. Cheng, J. Appl. Phys. tion completely equivalent to that in 1D from the point 98, 113702 (2005). of view of spin dynamics. Taking into account recent ex- 13 P. Schwab, M. Dzierzawa, C. Gorini, and R. Raimondi, Phys. Rev. B 74, 155316 (2006). perimental demonstration of persistent spin helix [5] the 14 M. Q. Weng, M. W. Wu, and H. L. Cui, J. Appl. Phys. emergenceofpersistentspinhelixfromhomogeneousspin 103, 063714 (2008). polarization can be straightforwardly detected. Finally, 15 P. Kleinert and V. V. Bryksin, Phys. Rev. B 79, 045317 we would like to note that the amplitude of persistent (2009). spin helix can be increased by a repetitive excitation of 16 M. Duckheim, D. L. Maslov, and D. Loss, Phys. Rev. B homogeneous polarization by a train of laser pulses. 80, 235327 (2009). In summary, we have demonstrated that persistent 17 I. V. Tokatly and E. Y. Sherman, Ann. Phys. 325, 1104 (2010). spin helix forms in the process of relaxation of homo- 18 M.I.DyakonovandV.I.Perel’,Sov.Phys.SolidState13, geneous spin polarization in finite length systems. This 3023 (1972). observationcanbeusedasadifferenttechniqueforcreat- 19 A.R.Cameron,P.Riblet,andA.Miller,Phys.Rev.Lett. ing spin helical structures in semiconductors. The solu- 76, 4793 (1996). tionofspindrift-diffusionequationsdescribingformation 20 J. Schliemann, J. C. Egues, and D. Loss, Phys. Rev. Lett. of persistent helix was derived analytically and numeri- 90, 146801 (2003). cally using Monte Carlo simulation approach. The re- 21 V. M. Galitski, A. A. Burkov, and S. Das Sarma, Phys. Rev. B 74, 115331 (2006). sults obtained in both ways are in perfect agreement. It 22 S. Saikin, Y. Pershin, and V. Privman, IEE-Proc. Circ. is interesting that the persistent helix amplitude demon- Dev. Syst. 152, 366 (2005). strates an oscillatory dependence on the system length andstrengthofspinorbitinteraction. Therefore,thecon-

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