1 Simulation of arctic low-level clouds observed during the FIRE Arctic Cloud Experiment using a new bulk microphysics scheme. SHORT TITLE: Simulation of arctic low-level clouds Eric Girard *and Judith A. Curry Department of Aerospace Engineering Sciences CB 429, University of Colorado, Boulder, CO 80309-0429 * Corresponding author Submitted to J. Geophys. Res. on December 1, 1999, special section of the FIRE Arctic Cloud Experiment. In revised version on April 10, 2000. 2 Abstract. A new bulk cloud microphysics scheme that accounts for aerosol microphysi- cal properties and size distribution is implemented into the single-column version of the ARCSyM. This scheme is distinguished from other bulk microphysics schemes by its prognostic determination of cloud particle number concentration and saturation ratio. The new scheme is compared to a simpler bulk microphysics scheme and observations taken during the FIRE Arctic Cloud Experiment in May 1998. Qualitatively, the two micro- physics schemes are generally in agreement with the observed cloud formation and evo- lution. Comparison with aircraft measurements at three times shows that the new scheme better discriminates cloud phase and reproduces reasonably well the observed liquid and ice water content for two cases. The better performance of the new scheme is attributed to its more elaborated treatment of the freezing process which is made possi- ble by the prognostic determination of cloud particle number concentration and the assumption of a bimodal lognormal cloud size distribution. Sensitivity studies are per- formed to assess four aerosol microphysical properties on the evolution of cloud micro- physical processes. Results show that the IFN concentration, the aerosol number concentration, the slope of the aerosol size distribution and the aerosol solubility may impact substantially on cloud phase and total water content. The liquid water path and ice water path can vary by as much as 100 g m-2 locally as a result of the variation of these parameters related to aerosols. 3 1. Introduction The importance of arctic clouds and radiation to the regional and global climate is summarized by Curry etal. [1996]. The difficulty in simulating and remotely sensing these clouds motivated the FIRE Arctic Cloud Experiment [Curryetal., 2000], which was conducted in conjunction with the Surface Heat Budget of the Arctic Ocean (SHEBA) experiment [Perovichetal., 1999]. The difficulties in modelling arctic clouds have been hypothesized byCurryetal.[1996] to arise from the complex vertical structure of the sta- ble arctic atmosphere, the presence of mixed-phase clouds, and the susceptibility of the arctic clouds to modification by aerosols. Curryetal.[2000] describe an initial application of the SHEBA/FIRE dataset to evaluating cloud parameterizations in the context of single-column model simulations. Results of simulations for May 1998 showed that the models tend to underpredict low cloud amount and the column liquid water path. The underestimation of the column liquid water path was in part attributed to inaccurately representing mixed-phase clouds as entirely crystalline. Mixed-phase clouds occur at high frequency in the Arctic from November to June [Curryetal., 1990; Pinto, 1998; Perovichetal., 1999]. From observations obtained dur- ing autumn from the Beaufort Arctic Storms Experiment (BASE), Pinto[1998] hypothe- sized that mixed-phase clouds are maintained in the arctic boundary layer through a balance of condensation of liquid water through cooling and heterogeneous freezing of the cloud drops. Jiangetal. [2000] simulated the observed case study described by Pinto and found strong sensitivity of the phase of the cloud to the concentration of ice forming nuclei (IFN). Simulations by GirardandBlanchet(GB)[2000a] with an explicit 4 aerosol-cloud microphysics model have shown that low-level clouds may remain in a mixed-phase state as long as 10 hours in the Arctic during winter. Bulk microphysical parameterizations used in climate models [e.g.Fowleretal., 1996] typically distinguish the phase of cloud water by the cloud temperature. The dis- crimination between the liquid and ice phases may be specified in terms of a single cutoff temperature, or as a function of temperature with the ratio of ice water content to liquid water content varying from 0 at 0oC to 1 at -40oC.Curryetal.[1996] cite observations of liquid drops in arctic clouds at temperatures as low as -32oC, and clouds that are com- pletely glaciated at -14oC. Clearly, a simple temperature discriminator is not sufficient to diagnose the phase of supercooled clouds in the Arctic. The complexity of the interactions between arctic cloud microphysics and aerosol are discussed by GB[2000a, b]. Aerosol composition and concentration modify cloud microphysical properties through their ability to nucleate ice and water. Blanchetand Girard[1995] hypothesized that the microphysical properties associated to Arctic haze aerosols in the Arctic may alter the cloud particle mean diameter and consequently increase the precipitation efficiency. This would result in a larger dehydration rate of the air mass which in turn would lead to a decrease of the downward longwave radiation flux at the surface. Other indirect effects of aerosols such as the Twomey and the Albrecht effects [Twomey, 1991; Albrecht, 1989] may strongly affect cloud microphysical proper- ties. Current bulk microphysics schemes used in general circulation models generally describe cloud with four prognostic variables: liquid, ice, rain, and snow water content [e.g.Fowleretal., 1996]. In these schemes, the effective radius of cloud particles is 5 parameterized as a function of temperature [e.g.OuandLiou, 1995] or liquid or ice water content [e.g.McFarlaneetal., 1992]. Current moisture schemes are therefore of limited utility in studying cloud microphysical properties changes resulting from aerosol forcing. To account for the influence of aerosol on cloud microphysical properties, prognostic equations must be included for either particle concentration or size, in addition to con- densed water content. In this paper, we describe a new bulk microphysics scheme that is capable of accounting for the impact of aerosol on cloud nucleation. This scheme is developed by merging the cloud schemes from GB[2000b] for cloud liquid and cloud ice and the pro- duction of precipitation following Grelletal.[1995]. The new microphysics scheme pre- dicts the ice and liquid water content, rain and snow, number concentration of cloud droplets and ice crystals, and cloud saturation ratio. Aerosol concentration and composi- tion are prescribed. This scheme is tested against observations taken during the FIRE Arctic Cloud Experiment in May 1998. The new microphysics scheme is also compared to the original version of the microphysics scheme developed by Grelletal.[1995] that does not include prognostic equations for particle concentration or saturation ratio. Finally, a sensitivity experiment is carried out to assess the effect on cloud formation of changing the IFN and aerosol concentration, the slope of the aerosol size distribution and the aerosol solubility. 2. Model Description The single-column version of the Arctic Regional Climate System Model (ARC- SyM) [Lynchetal., 1995] was used in our study. The ARCSyM is based upon the NCAR 6 regional climate model Version 2 (RegCM) [Giorgietal., 1993a,b]. The model has 38 vertical levels with 13 levels between 900 hPa and the surface that allows for a high res- olution simulation of the vertical structure of the boundary layer. In this paper, a brief description of ARCSyM physics package is given. The bulk microphysics schemes used in this study are described in details thereafter. One is referred toLynchetal.[1995] for a more extensive description of the other components of the model. In the ARCSyM, the planetary boundary layer scheme of Holtslagetal.[1990] is used. The model uses the CCM2 solar radiation scheme [Briegleb, 1992a,b] and the RRTM infrared radiation scheme [Mlaweretal., 1997]. The cloud scheme ofGrellet al. [1995] is used for simulat- ing cumulus cloud processes. Two bulk microphysics schemes have been implemented in ARCSyM: (1) the NCAR/MM5 Penn State cloud scheme [Grelletal., 1995], hereafter referred to as the MM5 microphysics scheme, and (2) the new microphysics scheme developed in this research. The MM5 cloud scheme is based on the bulk microphysics scheme of Grellet al.[1995] and is an upgraded modified version of the microphysics scheme of Dudhia [1989].Prognosticvariablesare:the icemixingratio,liquidmixingratio,snowmixingratio and rain mixing ratio. Microphysical processes simulated include: nucleation of ice crys- tals, nucleation of water droplets, condensation, evaporation, deposition, sublimation, autoconversion of cloud droplet to rain, autoconversion of ice crystals to snow, melting/ freezing of snow/rain and of cloud droplets/ice crystals and collision processes. The new scheme is distinguished from the MM5 cloud scheme by the addition of three prognostic variables: the saturation ratio, the number concentration of cloud drop- lets and ice crystals. These prognostic variables added to the ice and liquid mixing ratios 7 allow for determining the mean diameter of ice crystals and water droplets diagnostically. Cloud particle size distribution is assumed to be a superposition of two lognormals with a standard deviation of 1.3, each lognormal representing one phase, followingGB[2000b]. This choice of cloud particle size distribution is based on simulation of arctic low cloud with an explicit microphysics model [GB, 2000a] and observations [Rogers and Yau, 1989]. Although observations indicate that the gamma size distribution can also be used to represent cloud spectra in models [RogersandYau, 1989], the lognormal distribution is preferred here since it is more representative of the cloud spectra obtained with the explicit microphysics model [GB, 2000a] which has been used to develop the bulk micro- physics scheme. The new scheme and the MM5 scheme are based upon eight and five prognostic equations respectively. The five common prognostic equations are: water vapor mixing ratioq: v ¶ q ¶ q ¶ q ¶ q v = –u v –v v –w v –PCC –PCI –PII–PID+ PREC + PRES + d (1) ¶ t ¶ x ¶ y ¶ z qv cloud liquid mixing ratioq: c ¶ q ¶ q ¶ q ¶ q c c c c = –u – v –w +PCI + PCC + PRM –PCA –PRG –PRH ¶ t ¶ x ¶ y ¶ z –PACCC –PRSC + d (2) qc cloud ice mixing ratioq: i 8 ¶ q ¶ q ¶ q ¶ q i i i i = –u – v –w +PII + PID+ PRG+ PRH – PRA– PACCI ¶ t ¶ x ¶ y ¶ z –PRSI –PRM + d (3) qi rain mixing ratioq: r ¶ q ¶ q ¶ q ¶ q r = –u r – v r – w r –PREC –PKR+ PCA+ PACCC +d ¶ t ¶ x ¶ y ¶ z qr (4) snow mixing ratioq: s ¶ q ¶ q ¶ q ¶ q s = –u s–v s–w s–PRES –PKS + PRA+ PACCI + d ¶ t ¶ x ¶ y ¶ z qs (5) The new scheme additionally includes the following prognostic equations: number concentration of cloud dropletsN: c ¶ N ¶ N ¶ N ¶ N c c c c = – u –v – w ¶ t ¶ x ¶ y ¶ z r – ----------------(PCA+ PRSC +PACCC–PRG–PRH – PCI + PRM)+d (6) m(D ) Nc c number concentration of ice crystalsN: i ¶ N ¶ N ¶ N ¶ N i i i i = –u –v –w ¶ t ¶ x ¶ y ¶ z r – ---------------(PRA+ PRSI +PACCI–PRG–PRH – PII +PRM)+d (7) m(D ) Ni i saturation ratioS: dS –L ¶ T ¶ T ¶ T ¶ T p ------ = ------------ + u +v + w + -------[PCC + PCI + PII + PID– PRES –PREC] (8) dt 2 ¶ t ¶ x ¶ y ¶ z e e R T s v 9 where u, v, w, p, T, r , L, e, R and d are respectively the zonal velocity, longitudinal s v velocity, vertical velocity, pressure, temperature, air density, latent heat of fusion, vapor partial pressure at water saturation, gas constant for water vapor and the turbulent verti- cal mixing. e =R/R where R is the gas constant for dry air. The terms m(D)represent v d d the mass of the ice crystal/cloud droplet of diameterD, which is the mean diameter of the size distribution. The variables related to moist processes (PRES,PREC,PRA,PCA, PRM,PID,PCC,PCI,PII,PACCI,PACCC,PRSC,PRSI,PKR,PKS,PRH,PRG) repre- sents the sources and sinks of the microphysics fields and they are defined in appendix A. Detailed formulation of these microphysical processes is given in Dudhia[1989] and Grelletal.[1995]. The saturation budget equation follows the formulation of Rogersand Yau[1989] (p.119). Srepresents the mean value or large scale value of the saturation ratio of the grid cell. Subscale variations ofSare not considered. The first term in (8) rep- resents the change of Sdue to air mass radiative and advective cooling and the change of S due to condensation and deposition. In our simulations with the single column model, the advective terms in equations (2) to (7) are neglected due to the absence of observations. Advective tendencies in the equations for water vapor and saturation are provided by the ECMWF reanalyses as described below. The vertical eddy diffusion (d ) is determined by the K-theory. The eddy diffusion coefficient is a function of the local Richardson number as described inGrell et al. [1995]. Cloud entrainment is neglected. Seven microphysical processes are treated differently in the new scheme relative to the MM5 scheme: the cloud water droplet nucleation (PCI), ice crystal nucleation (PII), the condensation/evaporation onto/of cloud water droplets (PCC), the deposition/subli- mation onto/of ice crystals (PID), the heterogeneous freezing of water droplets (PRH), 10 the homogeneous freezing of water droplets and interstitial aerosols (PRG) and the auto- conversion of ice crystals to snow (PRA). The treatment of these microphysical pro- cesses is described in GB[2000b] for the new scheme and in Grelletal.[1995] for the MM5 scheme. In this paper, due to their important role in the results in this research, the treatment of the heterogeneous freezing of cloud droplets and autoconversion of cloud ice to snow is described below. 2.1. Heterogeneous Freezing The freezing of cloud water droplets is an important process that determines the formation and longevity of mixed-phase clouds. Laboratory experiments [e.g. Prup- pacherandKlett, 1997] and measurements in the Arctic [Pinto, 1998] have shown that cloud glaciation varies as a function of the temperature and the cloud droplet size; the largest having more chances to freeze due to their higher probability to encounter an IFN in the atmosphere. In the new bulk microphysics scheme, the heterogeneous freezing of cloud water droplets depends on cloud droplet size, temperature and IFN concentration. The param- eterization ofMeyersetal.[1992] is used for the IFN concentration. The median freezing temperature (T ), which is defined as the temperature at which half of the cloud droplets m of a certain size freeze, is determined by the parameterization of Heverley [Pruppacher and Klett,1997, p. 351] as follows: 1 (cid:230) (cid:230) aln2(cid:246) (cid:230) ¶ T(cid:246) (cid:246) Tm = a--- lnŁ Ł --B----V----ł- + lnŁ ¶ tł ł (9)
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