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Principles of Lasers FIFTHEDITION Principles of Lasers FIFTHEDITION Orazio Svelto PolytechnicInstituteofMilan andNationalResearchCouncil Milan,Italy TranslatedfromItalianandeditedby David C. Hanna SouthamptonUniversity Southampton,England 123 OrazioSvelto PolitecnicodiMilano Dipto.Fisica PiazzaLeonardodaVinci,32 20133Milano Italy ISBN978-1-4419-1301-2 e-ISBN978-1-4419-1302-9 DOI10.1007/978-1-4419-1302-9 SpringerNewYorkDordrechtHeidelbergLondon LibraryofCongressControlNumber:2009940423 1stedition:(cid:2)c PlenumPress,1976 2ndedition:(cid:2)c PlenumPublishingCorporation,1982 3rdedition:(cid:2)c PlenumPublishingCorporation,1989 4thedition:(cid:2)c PlenumPublishingCorporation,1998 (cid:2)c SpringerScience+BusinessMedia,LLC2010 Allrightsreserved.Thisworkmaynotbetranslatedorcopiedinwholeorinpartwithoutthewrittenpermission ofthepublisher(SpringerScience+Business Media,LLC,233SpringStreet,NewYork,NY10013,USA),except forbriefexcerptsinconnectionwithreviewsorscholarlyanalysis.Useinconnectionwithanyformofinformation storageandretrieval,electronicadaptation,computersoftware,orbysimilarordissimilarmethodologynowknown orhereafterdevelopedisforbidden. Ifthereiscoverart,insertcoverillustrationline.Givethenameofthecoverdesignerifrequestedbypublishing. Theuseinthispublicationoftradenames,trademarks,servicemarks,andsimilarterms,eveniftheyarenotidentified assuch,isnottobetakenasanexpressionofopinionastowhetherornottheyaresubjecttoproprietaryrights. Printedonacid-freepaper SpringerispartofSpringerScience+BusinessMedia(www.springer.com) To my wife Rosanna and to my sons Cesare and Giuseppe Preface Thisbookismotivatedbytheveryfavorablereceptiongiventothepreviouseditionsaswell as bythe considerablerangeof new developmentsin the laser field since thepublicationof thethirdeditionin1989.Thesenewdevelopmentsinclude,amongothers,Quantum-Welland Multiple-QuantumWelllasers,diode-pumpedsolid-statelasers,newconceptsforbothstable and unstable resonators, femtosecondlasers, ultra-high-brightnesslasers etc. The basic aim ofthebookhasremainedthesame,namelytoprovideabroadandunifieddescriptionoflaser behavioratthesimplestlevelwhichiscompatiblewithacorrectphysicalunderstanding.The bookisthereforeintendedasatext-bookforasenior-levelorfirst-yeargraduatecourseand/or asareferencebook. Thiseditioncorrectsseveralerrorsintroducedinthepreviousedition.Themostrelevant additionsorchangestosincethethirdeditioncanbesummarizedasfollows: 1. A much-more detailed description of Amplified Spontaneous Emission has been given [Chapt. 2] and a novel simplified treatment of this phenomenon both for homogeneousorinhomogeneouslineshasbeenintroduced[AppendixC]. 2. A major fraction of a chapter [Chapt. 3] is dedicated to the interaction of radiation withsemiconductormedia,eitherinabulkformorina quantum-confinedstructure (quantum-well,quantum-wireandquantumdot). 3. Amoderntheoryofstableandunstableresonatorsisintroduced,whereamoreexten- sive use is made of the ABCD matrix formalism and where the most recent topics ofdynamicallystableresonatorsaswellasunstableresonators,withmirrorshaving Gaussianorsuper-Gaussiantransversereflectivityprofiles,areconsidered[Chapt.5]. 4. Diode-pumping of solid-state lasers, both in longitudinal and transverse pumping configurations, are introduced in a unified way and a comparison is made with correspondinglamp-pumpingconfigurations[Chapt.6]. 5. Spatially-dependentrateequationsareintroducedforbothfour-levelandquasi-three- levellasersandtheirimplications,forlongitudinalandtransversepumping,arealso discussed[Chapt.7]. vii viii Preface 6. Laser mode-locking is considered at much greater length to account for e.g. new mode-locking methods, such as Kerr-lens mode-locking. The effects produced by second-orderandthird-orderdispersionofthelasercavityandtheproblemofdisper- sioncompensationtoachievetheshortestpulse-durationsarealsodiscussedatsome length[Chapt.8]. 7. New tunable solid-state lasers, such as Ti: sapphire and Cr: LISAF, as well as new rare-earth lasers such as Yb3C, Er3C, and Ho3C are also considered in detail [Chapt.9]. 8. Semiconductor lasers and their performance are discussed at much greater length [Chapt.9]. 9. The divergence properties of a multimode laser beam as well as its propagation through an optical system are considered in terms of the M2-factor and in terms of theembeddedGaussianbeam[Chapt.11and12]. 10. The production of ultra-high peak intensity laser beams by the technique of chirped-pulse-amplificationandthe relatedtechniquesofpulse expansionandpulse compressionarealsoconsideredindetail[Chapt.12]. The book also contains numerous, thoroughly developed, examples, as well as many tablesandappendixes.Theexampleseitherrefertorealsituations, asfoundintheliterature or encountered through my own laboratory experience, or describe a significative advance in a particulartopic.Thetablesprovidedataonoptical, spectroscopicandnonlinear-optical propertiesoflasermaterials,thedatabeingusefulfordevelopingamorequantitativecontext aswellasforsolvingtheproblems.Theappendixesareintroducedtoconsidersomespecific topicsinmoremathematicaldetail.Agreatdealofefforthasalsobeendevotedtothelogical organizationofthebooksoastomakeitscontentmoreaccessible. Thebasicphilosophyofthebookistoresort,whereverappropriate,toanintuitivepicture rather than to a detailed mathematical description of the phenomena under consideration. Simple mathematical descriptions, when useful for a better understanding of the physical picture, are includedin the textwhile the discussion of more elaborateanalyticalmodelsis deferredtotheappendixes.Thebasicorganizationstartsfromtheobservationthatalasercan beconsideredtoconsistsofthreeelements,namelytheactivemedium,theresonator,andthe pumpingsystem.Accordingly,afteranintroductorychapter,Chapters2–3,4–5and6describe themostrelevantfeaturesoftheseelements,separately.Withthecombinedknowledgeabout these constituentelements, chapters7 and 8 then allow a discussion of continuos-waveand transientlaserbehavior,respectively.Chapters9and10thendescribethemostrelevanttypes oflaserexploitinghigh-densityandlow-densitymedia,respectively.Lastly,chapters11and 12 consider a laser beam fromthe user’s view-pointexaminingthe propertiesof the output beamaswellassomerelevantlaserbeamtransformations,suchasamplification,frequency conversion,pulseexpansionorcompression. Withsomanytopics,examples,tablesandappendixes,itisclearthattheentirecontent of the book could not be covered in only a one semester-course. However the organization ofthebookallowsseveraldifferentlearningpaths.Forinstance,onemaybemoreinterested inlearningthePrinciplesofLaserPhysics.Theemphasisofthestudyshouldthenbemostly concentratedonthefirstsectionofthebook[Chapt.1–5andChapt.7–8].If,ontheotherhand, thereaderismoreinterestedinthePrinciplesofLaserEngineering,effortshouldmostlybe concentrated on the second part of the book Chap. 6 and 9–12. The level of understanding Preface ix of a given topic may also be suitably modulated by e.g. considering, in more or less detail, the numerousexamples, which often representan extensionof a giventopic, as well as the numerousappendixes. Writingabook,albeitasatisfyingculturalexperience,representsaheavyintellectualand physicaleffort.This efforthas, however, been gladly sustained in the hope that this edition canservethepressingneedforageneralintroductorycoursetothelaserfield. ACKNOWLEDGMENTS. I wish to acknowledge the following friends and colleagues, whose suggestionsand encouragementhave certainly contributedto improvingthe book in anumberofways:ChristoferBarty,VittorioDeGiorgio,EmilioGatti,DennisHall,Gu¨nther Huber, Gerard Mourou, Colin Webb, Herbert Welling. I wish also to warmly acknowl- edge the critical editing of David C. Hanna, who has acted as much more than simply a translator. Lastly I wish to thank, for their useful comments and for their critical reading of the manuscript, my former students: G. Cerullo, S. Longhi, M. Marangoni, M. Nisoli, R.Osellame,S.Stagira,C.Svelto,S.Taccheo,andM.Zavelani. Milano OrazioSvelto Contents ListofExamples . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . xix 1. IntroductoryConcepts . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 1 1.1. SpontaneousandStimulatedEmission,Absorption . . . . . . . . . . . . . . . . . . 1 1.2. TheLaserIdea . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 4 1.3. PumpingSchemes . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 6 1.4. PropertiesofLaserBeams . . . . . . . . . . . . . . . . . . . . . . . . . . . 8 1.4.1. Monochromaticity . . . . . . . . . . . . . . . . . . . . . . . . . . . 9 1.4.2. Coherence . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 9 1.4.3. Directionality . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 10 1.4.4. Brightness . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 11 1.4.5. ShortTimeDuration . . . . . . . . . . . . . . . . . . . . . . . . . . 13 1.5. TypesofLasers . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 14 1.6. OrganizationoftheBook . . . . . . . . . . . . . . . . . . . . . . . . . . . . 14 Problems . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 15 2. InteractionofRadiationwithAtomsandIons . . . . . . . . . . . . . . . . . . 17 2.1. Introduction . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 17 2.2. SummaryofBlackbodyRadiationTheory . . . . . . . . . . . . . . . . . . . . . 17 2.2.1. ModesofaRectangularCavity . . . . . . . . . . . . . . . . . . . . . . 19 2.2.2. TheRayleigh-JeansandPlanckRadiationFormula . . . . . . . . . . . . . . 22 2.2.3. Planck’sHypothesisandFieldQuantization . . . . . . . . . . . . . . . . . 24 2.3. SpontaneousEmission . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 26 2.3.1. SemiclassicalApproach . . . . . . . . . . . . . . . . . . . . . . . . . 26 2.3.2. QuantumElectrodynamicsApproach . . . . . . . . . . . . . . . . . . . . 30 2.3.3. AllowedandForbiddenTransitions . . . . . . . . . . . . . . . . . . . . . 31 xi xii Contents 2.4. AbsorptionandStimulatedEmission . . . . . . . . . . . . . . . . . . . . . . . 32 2.4.1. RatesofAbsorptionandStimulatedEmission . . . . . . . . . . . . . . . . 32 2.4.2. AllowedandForbiddenTransitions . . . . . . . . . . . . . . . . . . . . . 36 2.4.3. TransitionCrossSection,AbsorptionandGainCoefficient . . . . . . . . . . . 37 2.4.4. EinsteinThermodynamicTreatment . . . . . . . . . . . . . . . . . . . . 41 2.5. LineBroadeningMechanisms . . . . . . . . . . . . . . . . . . . . . . . . . . 43 2.5.1. HomogeneousBroadening . . . . . . . . . . . . . . . . . . . . . . . . 43 2.5.2. InhomogeneousBroadening . . . . . . . . . . . . . . . . . . . . . . . 47 2.5.3. ConcludingRemarks . . . . . . . . . . . . . . . . . . . . . . . . . . 49 2.6. NonradiativeDecayandEnergyTransfer . . . . . . . . . . . . . . . . . . . . . . 50 2.6.1. MechanismsofNonradiativeDecay . . . . . . . . . . . . . . . . . . . . 50 2.6.2. CombinedEffectsofRadiativeandNonradiativeProcesses . . . . . . . . . . . 56 2.7. DegenerateorStronglyCoupledLevels . . . . . . . . . . . . . . . . . . . . . . 58 2.7.1. DegenerateLevels . . . . . . . . . . . . . . . . . . . . . . . . . . . 58 2.7.2. StronglyCoupledLevels . . . . . . . . . . . . . . . . . . . . . . . . . 60 2.8. Saturation . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 64 2.8.1. SaturationofAbsorption:HomogeneousLine . . . . . . . . . . . . . . . . 64 2.8.2. GainSaturation:HomogeneousLine . . . . . . . . . . . . . . . . . . . . 67 2.8.3. InhomogeneouslyBroadenedLine . . . . . . . . . . . . . . . . . . . . . 69 2.9. DecayofanOpticallyDenseMedium . . . . . . . . . . . . . . . . . . . . . . . 70 2.9.1. RadiationTrapping . . . . . . . . . . . . . . . . . . . . . . . . . . . 71 2.9.2. AmplifiedSpontaneousEmission . . . . . . . . . . . . . . . . . . . . . 71 2.10. ConcludingRemarks . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 76 Problems . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 77 References . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 78 3. EnergyLevels,RadiativeandNonradiativeTransitionsinMolecules andSemiconductors . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 81 3.1. Molecules . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 81 3.1.1. EnergyLevels . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 81 3.1.2. LevelOccupationatThermalEquilibrium . . . . . . . . . . . . . . . . . . 85 3.1.3. StimulatedTransitions . . . . . . . . . . . . . . . . . . . . . . . . . . 87 3.1.4. RadiativeandNonradiativeDecay . . . . . . . . . . . . . . . . . . . . . 91 3.2. BulkSemiconductors . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 93 3.2.1. ElectronicStates . . . . . . . . . . . . . . . . . . . . . . . . . . . . 93 3.2.2. DensityofStates . . . . . . . . . . . . . . . . . . . . . . . . . . . . 97 3.2.3. LevelOccupationatThermalEquilibrium . . . . . . . . . . . . . . . . . . 98 3.2.4. StimulatedTransitions . . . . . . . . . . . . . . . . . . . . . . . . . . 101 3.2.5. AbsorptionandGainCoefficients . . . . . . . . . . . . . . . . . . . . . 104 3.2.6. SpontaneousEmissionandNonradiativeDecay . . . . . . . . . . . . . . . . 110 3.2.7. ConcludingRemarks . . . . . . . . . . . . . . . . . . . . . . . . . . 112 3.3. SemiconductorQuantumWells . . . . . . . . . . . . . . . . . . . . . . . . . 113 3.3.1. ElectronicStates . . . . . . . . . . . . . . . . . . . . . . . . . . . . 113 3.3.2. DensityofStates . . . . . . . . . . . . . . . . . . . . . . . . . . . . 116

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Principles of Lasers FIFTH EDITION Orazio Svelto Polytechnic Institute of Milan and National Research Council Milan, Italy Translated from Italian and edited by
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