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Nuclear Safety in Light Water Reactors Severe Accident Phenomenology Edited by Bal Raj Sehgal Support provided by the SARNET (Severe Accident Network) in the Framework Programmes of Research of the European Commission AMSTERDAMlBOSTONlHEIDELBERGlLONDON NEWYORKlOXFORDlPARISlSANDIEGO SANFRANCISCOlSINGAPORElSYDNEYlTOKYO AcademicPressisanimprintofElsevier AcademicPressisanimprintofElsevier 225WymanStreet,Waltham,MA02451,USA 525BStreet,Suite1900,SanDiego,CA92101-4495,USA TheBoulevard,LangfordLane,Kidlington,OxfordOX51GB,UK Radarweg29,POBox211,1000AEAmsterdam,TheNetherlands Firstedition2012 Copyright(cid:1)2012ElsevierInc.Allrightsreserved. ContributionsfromGeorgesVayssier,BalRajSehgal,andemployeesoftheFrenchInstitutde RadioprotectionetdeSuˆrete´Nucle´aire(IRSN)(cid:1)theirrespectiveowners;exclusivedistributionrights, Elsevier,Inc. Nopartofthispublicationmaybereproduced,storedinaretrievalsystemortransmittedinanyform orbyanymeanselectronic,mechanical,photocopying,recordingorotherwisewithouttheprior writtenpermissionofthepublisherPermissionsmaybesoughtdirectlyfromElsevier’sScience& TechnologyRightsDepartmentinOxford,UK:phone(+44)(0)1865843830;fax(+44)(0)1865 853333;email:permissions@elsevier.com.Alternativelyyoucansubmityourrequestonlineby visitingtheElsevierwebsiteathttp://elsevier.com/locate/permissions,andselectingObtaining permissiontouseElseviermaterial Notice Noresponsibilityisassumedbythepublisherforanyinjuryand/ordamagetopersonsorpropertyas amatterofproductsliability,negligenceorotherwise,orfromanyuseoroperationofanymethods, products,instructionsorideascontainedinthematerialherein.Becauseofrapidadvancesinthe medicalsciences,inparticular,independentverificationofdiagnosesanddrugdosagesshouldbemade LibraryofCongressCataloging-in-PublicationData Sehgal,BalRaj. Nuclearsafetyinlightwaterreactors/BalRajSehgal.–1sted. p.cm. Includesbibliographicalreferencesandindex. ISBN978-0-12-388446-6(alk.paper) 1.Lightwaterreactors–Riskassessment.2.Lightwaterreactors–Safetymeasures. I.Title. TK9203.L45S442012 621.48035–dc23 2011039984 BritishLibraryCataloguinginPublicationData AcataloguerecordforthisbookisavailablefromtheBritishLibrary ForinformationonallAcademicPresspublications visitourwebsiteatelsevierdirect.com PrintedandboundinGreatBritain 1213141510987654321 ISBN:978-0-12-388446-6 Preface Theideaofdocumentingtheadvancesachievedinthefieldoflightwaterreactor severe accident safety research in the form of a book originated during the developmentoftheresearchprogramfortheSevereAccidentResearchNetwork of Excellence (SARNET), coordinated by IRSN France, that was started in March2004,undertheauspicesoftheSixthFrameworkResearchProgramofthe European Commission. After some discussion, it was decided that the book should be a textbook for students and young researchers in the field and not ahandbook.Itwasalsodecidedthatthebookshouldnotbeacompendiumofall theresearchinthefield,butrathershouldbewrittentoimpartunderstandingand knowledgeaboutthecomplexphysicsofsevereaccidents.Thephysicsofsevere accidents involves several disciplines, including probability theory, neutron physics,thermalhydraulics,high-temperaturematerialscience,chemistry,and structuralmechanics.Thus,impartingunderstandingandknowledgeofsevere accidentsisnotasimpletask.Itisnonethelessanimportanttaskinreactorsafety, sinceasevereaccidentistheonlysourceofrisktothepublicfromanoperating lightwaterreactorpowerplant.Preventingandmanagingtheconsequencesof asevereaccident,whichisthemaingoalofsevereaccidentresearch,contributes greatlytoreducingthepublicriskofnuclearpower. The importance of severe accident research was recognized by the EURATOM Part of the Framework Research Programs of the European Commission. The Framework Program No. 4 was totally focused on severe accident(SA)research.TheEuropeanCommissioniscontinuingitssupportof SAresearchand,throughitssupportofSARNET,isencouragingthefocusof nationalresearch effortson an integratedEuropeanprogram of thisresearch. This book, Nuclear Safety in Light Water Reactors: Severe Accident Phenomenology,describestheresultsobtainedfromtheseresearchprograms, conductedoverthelast15yearsinEurope.Thebookalsocontainstheresults of SA research conducted over the years in the United States, Japan, Korea, Russia, and other countries. The research conducted in the United States, in particular, was the forerunner of the research that has been conducted in Europe. The knowledge gained in the U.S. research forms a very important base for SA research conducted throughout the world. The book, therefore, documents the data, phenomenology, and methodology developed for the description of severe accidents in all countries. ThisbookisajointeffortsinceitisaproductofSARNET,anetwork.Itwas conceivedasapedagogicaleffort,however,writtenbyacknowledgedexpertsin xiii xiv Preface the different areas of the SA field. It was coordinated, chapter by chapter, by different expertsandfinallycompiledand edited bythe undersigned. Chapter1ofthebookprovidesahistoricalreviewofthewholefieldofreactor safety,withshortintroductionsonthevarioussevereaccidentphenomenological topics.Italsoattemptstoprovideaninsightintothelogicofadvancementsin rectorsafetysincethebirthofnuclearenergy.Themostrecenttragiceventat Fukushima is also briefly described in Chapter 1, based on the information gainedasoftheendofJune,10,2011.Thisdescriptionmayneedcorrectionsas morecompleteinformationaboutthesesevereaccidentsatFukushimaemerges in time. Chapter 1 also briefly deals with the advances in mitigating severe accidentsachievedinthedesignsofsomeofthenew(GENIII+)LWRs. The remaining contents of the book follow the severe accident scenario, starting with the loss of cooling of the decay-heated core. The resulting core heat-up,coredegradation,hydrogenproduction,coremelting,accumulationof melt in lower head, failure of the lower head, hydrogen combustion, steam explosion, molten corium– concrete interactions (MCCI), fission product release, transport in the primary system, containment, and the like, are the subjectstreatedin the book. A question that arose early in deliberations on the contents of the book concerned the maturity of the SA field. We believe that nearly all the knowl- edgegainedthroughSAresearch,anddescribedinthebook,ismatureenough and will stand the test of time. It should also be stated that severe accident is still an active field of research, and some issues remain open; notably, the knowledge base still has uncertainties, and more research (experimentation, modeling,validation,etc.)isneeded,andindeedisbeingperformed.Evenfor theseissues,however,asufficientknowledgebasehasalreadybeenacquiredto document these areas ofuncertainties. Thebookisaproductoftheeffortsanddedicationofthecontributorslisted withthetextinthebook.Verysubstantialeffortswereinvolvedineditingthe various contributions and organizing the book. We hope that it will be a worthwhile book for the education of nuclear engineering students and a reference text for the young researchers who want to work, or are already engaged, inthe field of LWR severeaccident safety. Last,butnottheleast,wethecontributors(authors)andtheEditorwishto acknowledge with thanks, the steadfast and continous support of M. Michel Hugon, the EU Program Manager for the SARNET Network of Excellence. The Editor, also wishes to acknowledge with thanks, the able assistance of Dr. Van Dorsselaere inthe “final-edit”of the book. Bal Raj Sehgal Contributors Hans Alsmeyer, Karlsruher Institut fu¨r Technologie (KIT), retired, Technologies Institut fu¨r Kern- und Energietechnik (IKET), Hermann-von-Helmholtz-Platz 1, D-76344 Eggenstein-Leopoldshafen, Germany Eberhardt Alstadt, Helmholtz-Zentrum Dresden-Rossendorf (HZDR), Institute of Safety Research, P.O.B.510119,D-01314 Dresden,Germany Marc Barrachin, Institut de Radioprotection et de Suˆrete´ Nucle´aire (IRSN), Cadarache, BP3,13115, Saint-Paul-lez-Durance, France Ahmed Bentaib,IRSN, BP17,F- 92262, Fontenayaux Roses, FRANCE Jonathan Birchley, Paul Scherrer Institut (PSI), CH- 5232, Villigen PSI, SWITZERLAND ManfredBurger,Universita¨tStuttgart(IKE),Pfaffenwaldring31,D-70569Stuttgart, Germany CataldoCaroli, IRSN,BP17, F-92262, FontenayauxRoses, FRANCE Michel Cranga,IRSN,Cadarache, BP3, 13115,St Paul-lez-Durance, France TrucNamDinh,RoyalInstituteofTechnology(KTH),AlbaNova,10691Stockholm, Sweden and IdahoNational Laboratory,Idahofalls, USA Jean-Pierre Van Dorsselaere, SARNET coordinator, IRSN, Cadarache, BP3, 13115 Saint-Paul-lez-Durance,France Gerard Ducros, Commissariat a` l’Energie Atomique et aux Energies Alternatives (CEA), Cadarache Baˆt.315,F- 13108,St Paul-lez-durance, FRANCE Peter Eisert, Gesellschaft fuˆr Anlagen Und Reaktorsicherheit mbH (GRS), Schwertnergasse7,D-50461,Ko¨ln, Germany FlorianFichot,IRSN, Cadarache,BP 3,13115St-Paul-lez-Durance, France ManfredFischer,AREVAGmbH,D-91050,Erlangen,Germany Jerzy J. Foit, KIT, Technologies Institut fu¨r Kern- und Energietechnik (IKET), Hermann-von-Helmholtz-Platz1,D-76344Eggenstein-Leopoldshafen, Germany Salih Guentay,PSI,CH- 5232,VilligenPSI, Switzerland TimHaste,IRSN, Cadarache,BP 3,13115Saint-Paul-Lez-Durance Cedex, France Luisen Herranz, Centro de Investigationes Energeticas Medio Ambientales Y Tecnologicas (CIEMAT),Avda. Complutense, 22,E-28040, Madrid,SPAIN ZoltanHozer,KFKIAtomicEnergyResearchInstitute(AEKI),KonkolyThegeut29- 33, 49,H-1525, BUDAPEST,HUNGARY Christos Housiadas, “Demokritos” National Center for Scientific Research, PO Box 60228, 15310Agia Paraskevi Attikis,Greece xv xvi Contributors Ivan Ivanov, Technical University of Sofia (TUS), 8, Kl. Ohridski Blvd., Block 12, Office 12440, 1797,Sofia, BULGARIA Thomas Jordan, KIT, Technologies Institut fu¨r Kern- und Energietechnik (IKET), Hermann-von-Helmholtz-Platz 1, D-76344Eggenstein-Leopoldshafen, Germany Christophe Journeau,CEA,Cadarache, F- 13108,St Paul-lez-Durance, FRANCE Martin Kissane,IRSN, Cadarache,BP 3,F- 13115,St-Paul-lez-durance,FRANCE Ivo Kljenak, Jozef Stefan Institute (JSI), Reactor Engineering Division, Jamova 39, Ljubljana, Slovenia MarcoKoch,Ruhr-Universita¨tBochum,LEE,IB4/127,Universita¨tsstr.150,D-44801, Bochum,GERMANY Jean-Sylvestre Lamy, Electricite´ de France (EDF), R&D, SINETICS, 1 avenue du Ge´ne´ral de Gaulle,92140Clamart, France Jean-Claude Latche,IRSN,Cadarache, BP3,F- 13115,St-Paul-lez-Durance,France Terttaliisa Lind,PSI, CH-5232, Villigen PSI,SWITZERLAND WeiminMa,RoyalInstituteofTechnology(KTH),NuclearPowerSafety,AlbaNova, 10691Stockholm,Sweden Daniel Magallon, retired Scientist, Joint Research Centre (JRC), European Commission, Institute for Energy and Transport (IET), P.O. Box 2, NL-1755 ZG Petten,The Netherlands, seconded toCEA/Cadarache ManiMathews,AtomicEnergyofCanadaLimited(AECL),ChalkRiverLaboratories, ChalkRiver,Ontario,K0J1J0,Canada Leonhard Meyer, KIT, Technologies Institut fu¨r Kern- und Energietechnik (IKET), Hermann-von-Helmholtz-Platz 1, D-76344Eggenstein-Leopoldshafen, Germany Christoph Mueller, GRS mbH, retired, Forschunginstitute, 85748, Garching b. Mu¨nchen,Germany PascalPiluso,CEA, Cadarache,13108Saint-Paul-lezDurance, France Horst Schnadt,Tu¨vRheinland Industrie Service GmbH,retired, Cologne,Germany Andreas Schumm, EDF - R&D, SINETICS, 1 avenue du Ge´ne´ral de Gaulle, 92140 Clamart, France Bal Raj Sehgal, Emeritus Professor, Royal Institute of Technology (KTH), Nuclear Power Safety, AlbaNova,10691Stockholm,Sweden Jean-Marie Seiler,CEA, 17,av. desMartyrs, F- 38054,Grenoble, France Juergen Sievers,GRSmbH, Schwertnergasse 1,50667Ko¨ln, Germany ClausSpengler,GRS, Schwertnergasse7,D- 50461,Ko¨ln, Germany Bertrand Spindler,CEA, 17av.des Martyrs, F-38054, Grenoble, France Bruno Tourniaire,CEA, 17av.des Martyrs,F- 38054, Grenoble, France Klaus Trambauer, GRS mbH, retired, Forschunginstitute, 85748, Garching b. Mu¨nchen,Germany George Vayssier, Consultant, Nuclear Services Corporation (NSC), Kamperweg 1, 4417PC Hansweert, TheNetherlands Jean-Michel Veteau, CEA,retired, 17av.desMartyrs, F- 38054, Grenoble, France Chapter 1 Light Water Reactor Safety: A Historical Review Bal Raj Sehgal Chapter Outline 1.1. Introduction 2 1.10.1. Backgroundand 1.2. TheEarlyDays 3 RBMK 1.3. TheDevelopmentof Specifics 33 CivilianLWRS 3 1.10.2. HowandWhy 1.4. EarlySafetyAssesments 5 Chernobyl 1.5. TheSitingCriteria 5 Happened 37 1.5.1. Assumptionsand 1.11. TheDifficultYears 44 Requirements 1.12. SevereAccidentResearch 45 ofTID-14844 1.12.1. In-vesselAccident and10 Progressionfora CFR100 6 PWR 48 1.6. SafetyPhilosophy 7 1.12.2. In-vessel 1.6.1. TheDefense-in- Accident DepthApproach 8 Progressionfor 1.7. SafetyDesignBasis 10 aBWR 49 1.7.1. LOCAandthe 1.12.3. FissionProduct ECCS Releaseand Controversies 12 Transportduring 1.8. PublicRiskofNuclear theIn-vessel Power(WASH-1400) 15 Accident 1.8.1. TheReactorSafety Progression 50 Study 16 1.12.4. Ex-vessel 1.9. TheTMI-2Accident 27 Accident 1.9.1. Descriptionofthe Progression 51 Accident 27 1.13. SevereAccident 1.9.2. TheAftermathof Management 57 TMI-2Accident 32 1.13.1. Cooling 1.10. TheChernobylAccident 33 aDegradedCore 58 NuclearSafetyinLightWaterReactors.DOI:10.1016/B978-0-12-388446-6.00001-0 (cid:1)2012ElsevierInc.Allrightsreserved. 1 2 NuclearSafetyinLightWaterReactors:SevereAccidentPhenomenology 1.13.2. Managementof 1.14.3. TheActual Combustible Progressionofthe Gases 60 Fukushima 1.13.3. Managementof Accidents 69 Containment 1.14.4. Concluding Temperature, Remarksonthe Pressure,and Fukushima Integrity 60 Accidents 75 1.13.4. Managementof 1.15. NewLWRPlants 78 Radioactive 1.15.1. TheIn-Vessel Releases 61 MeltRetention 1.14. TheFukushimaAccidents 62 (IVMR)Strategy 80 1.14.1. Introductionand 1.15.2. TheEx-Vessel Plant MeltRetention Characteristics 62 Strategy 82 1.14.2. Consequencesof Conclusions 85 aConservative References 86 Core-melt Scenariofor Fukushima Reactors 68 1.1. INTRODUCTION Thelightwaterreactor(LWR)safetythatweareconcernedwithinthisbookis basically about estimating the risks posed by an individual or a population of nuclear power plants (NPPs) to the public at large and the efforts to reduce theserisks.Thepublicofmostconcernisthatwhichresidesinthevicinityof anuclearpowerplantbutalsoatotherlocations,whichcouldbeaffectedbyan accident in aNPP locatedanywhere. The basic goal of safety is to ensure that a LWR will not contribute significantlytoindividualandsocietalhealthrisks.Thisbasicgoaltranslatesto the prevention of the release of radioactivity into the environment from the NPP.Acomplementaryaimistopreventdamagetotheplantandtoprotectthe personnel at the plant frominjury ordeathin anaccident. SinceLWRsafetyaimstoprotectthepublicatlarge,itisheavilyregulated. Each nuclear power country (and even some without NPPs) has regulatory commissions (bodies) that regulate every aspect of a NPP from design and construction to operation and any modifications. They require very extensive analyses,documentation,andqualitycontrol.Thereactorsafetydesignhasto follow definite rules and regulations. Some of these requirements will be described inthischapter. Chapter | 1 LightWaterReactorSafety:AHistoricalReview 3 The reactor performance, on the other hand, is concerned with long-term steady-state operations, since most LWR plants are base-loaded and strive to operate at full power, without interruption, between scheduled outages for maintenance. Reactor performance is also concerned with efficiency, the capacityfactor,fuelcyclecosts,maintenancecosts,andtheradiationdosetothe operatingstaff.Thus,itisnotregulated.However,ithasbeenfoundthatawell- runningLWRplantis,generally,asaferplantwithamuchlowerfrequencyof incidents,which,generally,aretheprecursorstomoreseriousevents. 1.2. THE EARLY DAYS The nuclear era started with the natural uranium-graphite pile built by Fermi and his associates at Stagg Field at the University of Chicago [1]. It did not involve light water as a coolant since only natural uranium was available and criticality could be achieved only with graphite or heavy water. The safetyconceptsdevelopedthere,however,wereadoptedbytheLWRplantsthat developedseveralyeas later.EnricoFermi andhis associatesrecognizedthat: l Nuclear fission reactions, which are the basis of nuclear power, emit high levels of radioactivity and thus could be a health hazard to any person exposedtoit. This impliedshielding,containment,and remote siting. l The safe operation of the reactor (or pile) would require protective and control measures, as evidenced by the provision of a control rod in the pile that Fermi and his associates built. Shieldingandremotesitingwererequiredfortheplantsthatwerebuiltfor theproductionofplutoniumintheUnitedStatesandothercountriesduringthe years before and after World War II. Remote siting of these plants not only protectedthepublicbutalsomaintainedthesecrecysurroundingtheproduction of nuclear weaponsfor anumberofyears. Thecontainmentaspectofprotectingthepublicfromanuclearaccidentwas notconsideredoremployedfortheplantsgeneratingplutonium.Thosewerethe yearsofabove-groundnuclearweaponstests,whichinanycasewerereleasing considerableamountsofradioactivefissionproductsintheatmosphere.Fortu- nately,therewerenoreportedaccidentsofanygreatsignificanceintheplutonium productionplantsineithertheUnitedStatesorotherWesterncountries. Leak-tightcontainmentasasafetysystemforacivilianNPPwasnotlongin coming.Itwasproposedin1947[2]fora sodium-cooledfastreactorthatwas thefocusofthepowerreactordevelopmentbytheU.S.DepartmentofEnergy at that time. Later, the LWR plant developers adopted leak-tight containment fortheirplants. 1.3. THE DEVELOPMENT OF CIVILIAN LWRS TheLWRdevelopmentstarted asamilitaryprogramintheUnitedStates and stemmedfromtheinitiativeofAdmiralHymanRickover,whoisconsideredthe 4 NuclearSafetyinLightWaterReactors:SevereAccidentPhenomenology fatheroftheU.S.nuclearnavy[3].Histeamconceivedthepressurizedwater- cooled reactor (PWR) as the NPP for submarine propulsion, since a sodium- cooled fast reactor, the focus of the U.S. national program, was considered unsuitable for a nuclear submarine submerged in water. Admiral Rickover obtained the necessary funding and the considerable intellectual resources neededtogeneratetheextraordinarilyrapiddevelopmentofthePWRplantfor the U.S. submarine fleet. PresidentDwightEisenhowerissuedthecallforAtomsforPeacein1954[3], whichbecamethesignalforadaptingmilitarydevelopmentsforcivilianpurposes. TheconstructionoftheShippingportPWR,Pennsylvania,USA.[3],whichwas completed in 1957, provided the prototype for NPPs, generating a reasonable amountofelectricalpowerforpublicconsumption.EBR-1,afastreactor,wasthe firstnuclearreactorintheUnitedStatestogenerateelectricalpower.However,the quantitygeneratedwasinsufficienttotransmitforpublicconsumption. The development of the other civilian water-cooled nuclear power reactor, thatis,theboilingwaterreactor(BWR),wasstartedalmostinparallelwiththatof the PWR and the construction of the Shippingport PWR plant. The BWR developmentwasspearheadedbytheGeneralElectric(GE)Company,aprivate enterprise, which, in fact, invested its own funds to develop the BWR as acommercialNPP.Inthisefforttheywereaidedbynationallaboratoriesinthe UnitedStatesdforexample,ArgonneNationalLaboratory,whichbuilta5-MW BWRsystem[3],andtheIdahoLaboratories,whereexperimentswereperformed [4]todemonstratethestabilityandsafetyoftheBWRsystem.Thefirstprototype commercialBWRplantwasdesignedandbuilt,asadual-cycle(i.e.,ithadasteam generatorforthesteamthatwenttotheturbine)plant,alreadyin1960byGE. In the United States, the first truly commercial NPP was the Yankee-Rowe plant, a PWR, which was also built in 1960. This plant was conceived as acommercialventureand wasspecificallycommissionedbyautilitycompany thatsuppliedelectricity tothe public. The Yankee-Roweplant was constructed withaleak-tightcontainment,anditwasapprovedforcommercialoperationby theregulatoryauthoritiesintheUnitedStatesAtomicEnergyCommission(AEC). Theplantdesignersatthattimedidnotrealizethattheirdecisiontoemployaleak- tight,pressure-bearingcontainmentwastheirmostimportantsafetydecision. Thecivilianuseofnuclearenergywasverypopularwiththepublicduring 1960s. Claims were being made that nuclear energy could provide unlimited andcheapelectricpower:toocheaptometer.Projectionswerebeingmadeof constructinghundreds(orevenathousand)powerreactorsintheUnitedStates alone.Someproposalsinvolvedthelocationofplantsveryclosetothecitiesto providegenerationsourcesnearlargeconsumptioncenters,inordertobecome moreeconomicinthetotalcostoftheelectricitytotheconsumers.The1970s saw a large number of orders placed by U.S. utility companies with U.S. vendors. The most prominent of these companies were: Westinghouse for the PWRplants,sinceitwasthevendorforthenavalPWRs;GeneralElectricfor the BWRs, since they were the developers of this reactor type; and Babcock

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