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YongAn Huang · Zhouping Yin · Xiaodong Wan Modeling and Application of Flexible Electronics Packaging Modeling and Application of Flexible Electronics Packaging YongAn Huang Zhouping Yin (cid:129) (cid:129) Xiaodong Wan Modeling and Application of Flexible Electronics Packaging 123 YongAnHuang ZhoupingYin State Key Laboratoryof Digital State Key Laboratoryof Digital Manufacturing Equipment andTechnology Manufacturing Equipment andTechnology HuazhongUniversity of Science HuazhongUniversity of Science andTechnology (HUST) andTechnology (HUST) Wuhan, People’sRepublic ofChina Wuhan, People’sRepublic ofChina Xiaodong Wan State Key Laboratoryof Digital Manufacturing Equipment andTechnology HuazhongUniversity of Science andTechnology (HUST) Wuhan, People’sRepublic ofChina ISBN978-981-13-3626-3 ISBN978-981-13-3627-0 (eBook) https://doi.org/10.1007/978-981-13-3627-0 JointlypublishedwithSciencePress,Beijing,China TheprinteditionisnotforsaleinChinaMainland.CustomersfromChinaMainlandpleaseorderthe printbookfrom:SciencePress,Beijing,China. LibraryofCongressControlNumber:2018968102 ©SciencePressandSpringerNatureSingaporePteLtd.2019 Thisworkissubjecttocopyright.AllrightsarereservedbythePublishers,whetherthewholeorpart of the material is concerned, specifically the rights of translation, reprinting, reuse of illustrations, recitation, broadcasting, reproduction on microfilms or in any other physical way, and transmission orinformationstorageandretrieval,electronicadaptation,computersoftware,orbysimilarordissimilar methodologynowknownorhereafterdeveloped. The use of general descriptive names, registered names, trademarks, service marks, etc. in this publicationdoesnotimply,evenintheabsenceofaspecificstatement,thatsuchnamesareexemptfrom therelevantprotectivelawsandregulationsandthereforefreeforgeneraluse. Thepublishers,theauthors,andtheeditorsaresafetoassumethattheadviceandinformationinthis book are believed to be true and accurate at the date of publication. Neither the publishers nor the authorsortheeditorsgiveawarranty,expressorimplied,withrespecttothematerialcontainedhereinor for any errors or omissions that may have been made. The publishers remain neutral with regard to jurisdictionalclaimsinpublishedmapsandinstitutionalaffiliations. ThisSpringerimprintispublishedbytheregisteredcompanySpringerNatureSingaporePteLtd. Theregisteredcompanyaddressis:152BeachRoad,#21-01/04GatewayEast,Singapore189721, Singapore Foreword Flexible electronics represent the next-generation microelectronics that offer the electricalfunctionsofconventional,rigidICtechnologiesbutwiththeabilitytobe stretched, compressed, twisted, bent, and deformed into arbitrary shapes. They overcome the fundamental mismatch in mechanics and form and have enabled applications that are impossible to achieve with hard, planar integrated circuits. Theirrepresentativeapplicationsincludeepidermiselectronicsthatareconformalto humanskin,wearablemicrofluidicdeviceforhealthmonitoringsystems,RFIDtags made up of rigid chips, and flexible antennas. Some of these devices (e.g., RFID tags) are obtained by packaging high-modulus, rigid, state-of-the-art chip-scale elements(e.g.,ICchips,MEMS,sensors,andpowersources)thatarefabricatedon the donor wafer onto flexible/stretchable substrates. Therefore, the chip-scale ele- ments have to be peeled off from the donor wafer, picked up, and placed on the receptor flexible/stretchable substrates, where the interfacial mechanics plays a critical role in the process. The transfer manipulation (peeling-picking-placing) of chips, such as resistor, capacitor, sensor, and interconnector is a key technology for advanced packaging. Majoradvancesintransfermanipulationofelectroniccomponentsanddeviceshave beenmadeoverthepastdecade.Forflexibleelectronics,thechipstendtobemuch smaller, thinner, or more flexible to meet the deformability and conformability. It becomes challenging for transfer manipulation, especially in the large-scale roll-to-roll production. Thisbookisthefirstoneabouttheinterfacialmechanicsoftransfermanipulation for flexible electronics packaging. It covers the state-of-the-art and comprehensive workonmodeling,simulations,andexperimentsoftheauthors,fromthetheoretical andexperimentalstudiesontheinterfacialmechanics,tothedesignandfabrication of stamp for transfer manipulation, and the applications in roll-to-roll assembly of flexibleelectronics.Multiplyprocessesaredevelopedforthetransfermanipulation of the chips with wide ranges of the mechanical and interfacial properties for flexible electronics, including single/multiple-needle peeling, conformal peeling, laser-induced peeling, vacuum-based picking-up, and low residual stress placing-on. The theoretical model and experimental verification are conducted v vi Foreword collaboratively to reveal the underlying mechanisms and optimize the peeling process. A competing index is proposed to characterize the competing fracture mechanism, namely fracture of the chip and interfacial delamination of the adhe- sive. These comprehensive analytical, computational, and experimental studies are very useful for advanced packaging of flexible electronics, as have been demon- strated in the flip-chip in RFID packaging, membrane electrode assembly in fuel cell stack, and laser lift-off in flexible devices. This is an excellent reference book for both academic research and industrial design offlexible electronics packaging. Yonggang Huang Member, US National Academy of Engineering Foreign Member, Academia Europaea Foreign Member, Chinese Academy of Sciences Northwestern University Evanston, IL, USA Preface Over the past decade, technological developments have enabled the flip-chip packaging for applications in computing, communications, and consumer elec- tronics. With the developing trends of electronic devices towards large-area and ultra-thin direction, the demand for the flip-chip packaging continues to grow to meet the requirements for performance, size, and flexibility, e.g., the flexible dis- play, radio frequency identification (RFID), wearable electronics, and bio-integrated electronics. The transfer manipulation(peeling-picking-placing) ofmicroscale and thinchip isoneofthekeytechnologiesofadvancedpackagingtoaccuratelytransferasingle chip from the wafer to a target circuit. Especially as the chips tend to be much thinner than before, a reliable peeling-picking-placing process is essential to the electrical performance, cost-effectiveness, service reliability, and life span of electronic devices. This book addresses important issues concerning the nonde- structive peeling-picking-placing technique for ultra-thin chip, including single/multi-needle peeling, conformal peeling, laser lift-off, and vacuum-based picking-up and placing-on. The theoretical model, physical mechanism, and experimental verification are conducted. The review on the developments of the transfer manipulation is discussed in Chap. 1. In Chap. 2, the interfacial peeling mechanism of the chip-on-substrate structure subjected to a transversely concentrated load resulting from the single ejector needle is first investigated, where the adhesive layer is neglected. A finite element simulation technique is also performed to obtain the energy release rate (ERR) of interfacial peeling. Then, an analytical model for the chip-adhesive-substrate structure is established. The corresponding analytical solutions for internal forces, displacements, and stresses are obtained. The theoretically and numerically esti- mated ERR of interfacial peeling is used to indicate the peeling behavior at the adhesive layer. In Chap. 3, the fracture strength of the ultra-thin silicon chip is first evaluated combining the geometrically nonlinear theory. The classical linear theory on the three-point bending test is found failed to match the geometrically nonlinear characteristics of ultra-thin silicon chip. The peeling behavior of the adhesive tape vii viii Preface from the adherend is then investigated experimentally. A novel homemade angle/speed controlled peeling platform is developed to assist in estimating the adhesivefractureenergy,wherethestretchabilityoftheadhesivetapeisconsidered in the evaluation model. In Chap. 4, an analytical solution is first presented based on the chip-adhesive- substrate structure model to determine the adhesive stresses in balanced and unbalanced stiffened plate, single-strap, and single-lap joints under mixed force loading and/or displacement boundary conditions. The adhesive stresses are expressedintermsofgeometricdimensionsandmaterialproperties,combinedwith integration constants obtained numerically. Then, a mechanical chip-adhesive- substratemodelisproposedtopredictthepeelingbehaviorofaperiodicarrayofIC chipsadhesivelybondedtoastretchedsubstrateviathemulti-segmentanalysis.The process parameters (substrate tension), the geometric parameters (chip thickness, and chip distance), and the material parameters (Young’s moduli of the chip and substrate) are considered to predict the peeling status at the adhesive layer. In Chap. 5, the interfacial peeling mechanism of chip-on-substrate and chip- adhesive-substratestructuressubjectedtoatransverselyconcentratedloadresulting fromsingleejectorneedleisfirstinvestigatedfromthefracture mechanicspointof view. Effects of key factors including the chip size, initial crack length, and sub- stratematerialareuncovered.AnalyticalexpressionsforadhesivestressesandERR of interfacial peeling are derived by using structural parameters and integration constants. Process limitation of the single-needle ejecting technique is discussed. The competing relationship between the chip peeling and chip cracking in the single-needle ejecting process isthen investigated combining thechip-on-substrate structure.Themechanismofcompetingfractureisrevealedfundamentallyusingthe proposed competing index. Finally, the finite element analysis is adopted to investigate the contact-impact effect during the single-needle ejecting process consideringtheimpactspeed,thedistancefromthecontactcenter,andthesubstrate penetration. InChap.6,ananalyticalmodelisfirstpresentedtoestimatethebendingnormal stress of the chip layer and ERR of interfacial peeling in the multi-needle ejecting process. A competing fracture model and failure criterion of the chip-adhesive- substratestructurebasedonchippeelingandchipcrackingindexesareputforward tosolvetheconflictbetweenthechippeelingandchipcrackingforultra-thinchips. Improvementontheultra-thinchippeeling-offthroughthemulti-needleadoptionis discussed and compared with the single-needle ejecting process. The process windowispreliminarilyexploredconsideringthechipgeometry,thestrengthofthe adhesive layer, and the layout of ejector needles. A modified multi-needle ejecting process using independently controlled ejector needles is finally proposed to improve the peelability of ultra-thin chips. In Chap. 7, a mechanical model is first established to address the roll-to-roll (R2R) conformal peeling of the device-adhesive-substrate structure. Analytical expressionsofthepeelstressandshearstressattheintermediateadhesivelayerare derivedundertheconformalconditionofthecurvedsurface.Theallowableranges of thethickness of thedevice and substrate layers aredeterminedfor a safe device Preface ix peeling-off. A competition model is established combining the conformal criterion to distinguish the device breakage and successful peeling-off. The peelability cri- terionfortheconformalpeelingprocessisproposedthroughthetheoreticalanalysis andexperimentalverification.Thedesignofthepeelbladeisstudiedcombiningthe peel radius and validated through the R2R peeling experiment of RFID tags. In Chap. 8, the laser lift-off (LLO) mechanism of ultra-thin polyimide (PI) film from the rigid glass carrier is revealed experimentally. The ultra-thin PI film is separated completely with low internal stress. Process parameters of the laser flu- ence and irradiation time are considered to determine the process window. The processmechanismisinterpretedcombiningthegasproductsgeneratedbythelaser irradiation, interface adhesion strength, and interface microstructure. In Chap. 9, a theoretical model of the chip-adhesive-substrate structure is first developed to reveal the process mechanism of theultra-thin chip picking-up under the condition of the vacuum adsorption with fixed adhesive tape length. An improved model consideringtheeffective tape length isfurtherproposedusing the bisection algorithm. The theoretical process window for the ultra-thin chip picking-up is determined. The mechanism of the R2R transferring with low inter- facialresidualstressistheninvestigated.Thecollaborativeoptimizationofmaterial properties and structural parameters is performed. The feasibility of reducing the interfacial residual stress is validated by using the R2R experimental platform. Additionally, with respect to the chip placing-on process, a layerwise thermal-mechanical model of the ultra-thin chip-on-flex structure considering the adhesive curing and cooling is developed to predict the ultra-thin chip warpage. We deeply acknowledge contributors of theoretical and experimental studies, includingJiankuiChen,BoPeng,ZunxuLiu,JingBian,ZhoulongXu,HuiminLiu, and Pengpeng Tang. In addition, we want to express our gratitude to the support from the national natural science foundation of China (No. 51635007, 51705180). Wuhan, China YongAn Huang August 2018 Zhouping Yin Xiaodong Wan Contents 1 Advanced Electronic Packaging . . . . . . . . . . . . . . . . . . . . . . . . . . . . 1 1.1 Introduction . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 1 1.2 Adhesively Bonded Multilayer Structure . . . . . . . . . . . . . . . . . . . 5 1.3 Interfacial Peeling-off . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 6 1.3.1 Needle Ejecting for Thin Chips. . . . . . . . . . . . . . . . . . . . 6 1.3.2 Conformal Peeling for Large-Area Devices . . . . . . . . . . . 8 1.3.3 LLO for Large-Area Flexible Electronics. . . . . . . . . . . . . 9 1.4 Vacuum-Based Chip Picking-up . . . . . . . . . . . . . . . . . . . . . . . . . 12 1.5 Vacuum-Based Chip Placing-on . . . . . . . . . . . . . . . . . . . . . . . . . 13 1.6 Competing Fracture . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 16 1.6.1 Competing Fracture Behavior . . . . . . . . . . . . . . . . . . . . . 16 1.6.2 Fracture Strength and Adhesive Fracture Energy . . . . . . . 16 References . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 17 2 Interfacial Modeling of Flexible Multilayer Structures . . . . . . . . . . . 29 2.1 Introduction . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 29 2.2 Modeling of Chip-on-Substrate Structure . . . . . . . . . . . . . . . . . . . 29 2.2.1 Mechanical Model . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 29 2.2.2 Analytical Evaluation on ERR of Interfacial Peeling . . . . 31 2.2.3 Virtual Crack Closure Technique (VCCT). . . . . . . . . . . . 33 2.2.4 Numerical Model. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 34 2.3 Modeling of Chip-Adhesive-Substrate Adhesively Bonded Joints. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 34 2.3.1 Adhesive Model on Overlapped Joints . . . . . . . . . . . . . . 34 2.3.2 Equilibrium Equations . . . . . . . . . . . . . . . . . . . . . . . . . . 36 2.3.3 Establishment of Differential Equation Set. . . . . . . . . . . . 38 2.3.4 Solutions for Internal Forces and Displacements . . . . . . . 40 2.3.5 Relationships Among Integration Constants. . . . . . . . . . . 44 2.3.6 Theoretical Calculation of ERR of Interfacial Peeling. . . . 46 xi

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