Light scattering in pseudo-passive media with uniformly balanced gain and loss A. Basiri1, I. Vitebskiy2, T. Kottos1 1Department of Physics, Wesleyan University, Middletown, CT-06459, USA and 2Air Force Research Laboratory, Sensors Directorate, Wright Patterson AFB, OH 45433 USA (Dated: January 12, 2015) Weintroduceaclassofmetamaterialswithuniformlybalancedgainandlossassociatedwithcom- plexpermittivityandpermeabilityconstants. Therefractiveindexofsuchabalancedpseudo-passive metamaterial is real. An unbounded uniform pseudo-passive medium has transport characteristics similar to those of its truly passive and lossless counterpart with the same real refractive index. However, bounded pseudo-passive samples show some unexpected scattering features which can be further emphasized by including such elements in a photonic structure. 5 PACSnumbers: 42.82.Et,42.25.Bs,11.30.Er 1 0 2 In the last decade we have witnessed unprecedented advancements in realizing artificial materials which are n a specifically designed to exhibit features not found in na- J ture. Intheelectromagneticdomain,suchmetamaterials 9 are using their structural composition in order to obtain access of all four quadrants in the real (cid:15)−µ plane. Var- ] s ious exotic phenomena ranging from negative refraction c to electromagnetic cloaking and super-lensing have been i t actively pursued [1–8]. While these opportunities have p been extraordinary, optical materials exhibiting exotic o . values of permittivity ε and/or permeability µ are often s c prohibitively lossy. This is especially true for composite i optical meta-materials. A natural solution to the prob- s y lemistoaddagaincomponentand,thereby,tooffsetthe FIG. 1: (color online) The electric E(z) (y-z plane) and the h losses. A pathway to achieve this goal has been recently magnetic H(z) (x-z plane) field distribution of a resonance p proposedinRef. [9],andsubsequentlyexploredinanum- localizedmodeλr =1.256µmforaBragggratingwithanem- [ beddedPP-defect(green). Thegratingconsistsof20lossless ber of publications [10–28]. This proposal capitalizes on bilayers (orange and white) at each side of the defect. Their 1 the notion of Parity-Time (PT) symmetry by utilizing index of refraction is n = 1.45 and n = 1.755 and their 1 2 v balanced gain and loss elements which are judiciously width is d = 0.2167µm and d = 0.179µm. The pseudo- 1 2 0 distributed in space such that the complex index of re- passive (PP) defect layer has index of refraction np = 3.48 06 fraction n(r) satisfies the relation n(r) = n∗(−r). This correspondingtoconstituents(cid:15)p =3.48−i0.01,µp =(cid:15)∗p while its width is d =0.0542µm. 2 research line gave many intriguing transport properties p 0 like double refraction, unidirectional invisibility, asym- . metric transport, CPA/ Lasers etc. 1 oscillating magnetic fields. If both ε and µ are com- 0 An alternative approach is to compensate the losses plex, a real-value refractive index n can only be realized 5 1 withgainwhilepreservingtheuniformityofthemedium. if ε = ρ2µ∗ (where ρ is real), which is quite possible in Thiscanbedonesimplybydopingthelossymediumwith : media with gain. In this case n = ρ|µ| and thus one v active elements (dies), so that the doped material would i √ expects that an unbounded medium consisting of such X have a real refractive index n(r) = εµ = n∗(r). The material will support traveling waves as its lossless pas- question, however, is whether such a balanced loss/gain r sive counterpart with the same index of refraction. We a medium with real and uniform refractive index will au- will therefore refer to media with real refractive index n tomatically behave as a regular passive lossless medium. and complex ε(cid:48)(cid:48) and µ(cid:48)(cid:48) as pseudo-passive (PP) media. This is certainly true if the permeability µ is real, in Surprisingly, once a pseudo-passive medium is confined whichcasethenegativecontributiontoε(cid:48)(cid:48) fromgainwill inspace,itsscatteringpropertiesarecompletelydifferent simply offset the positive contribution from absorption than the ones of its passive counterpart. The difference [29–31]. becomes even more striking when a pseudo-passive ma- In this Letter we will concern with a different scenario terial is a component of a photonic structure. For exam- where both ε and µ are complex i.e. ε = ε(cid:48)+iε(cid:48)(cid:48), µ = ple, the Fabry-Perrot resonances of a Bragg grating that µ(cid:48) +iµ(cid:48)(cid:48). A typical example is plasmonic metamateri- contains pseudo-passive composite layers display sub- or als where the effective permeability is associated with superunitarytransmittanceattheband-edges. Remark- the electric current induced in tiny ring resonators by ably, under different circumstances, the same pseudo- 2 passive material can act as a perfect absorber, or it can Furthermore,wecanshowthatdetM=1andthust = L trigger lasing instability. t =t. The associated transmittance T and reflectances R The scattering properties of a pseudo-passive struc- R are T =|t|2 and R =|r |2. L,R L,R L,R ture are understood better by considering monochro- An alternative formulation of the scattering process maticwavepropagationinanone-dimensionalscattering is provided by the scattering matrix S which connects set-up. In this case, the steady state (TE) electric field incoming and outgoing wave amplitudes i.e. E(z) is scalar and satisfies the Helmholtz equation (cid:18)E− (cid:19) (cid:18) E+ (cid:19) L =S L (5) d2E(z) (cid:16)ω(cid:17)2 E+ E− +n2(z) E(z)=0 (1) R R dz2 c ThescatteringmatrixcanbewrittenintermsoftheM- where ω is the frequency of the field and c is the speed matrix elements as of light in vacuum while the spatially dependent index (cid:18) (cid:19) (cid:18) (cid:19) (cid:112) r t 1 −M 1 of refraction n(z)= ε(z)µ(z) is considered real for any S = L R = 21 (6) positionz. Inthecasethatthepseudo-passivemediumis tL rR M22 det(M) M12 extendedoverthewholespace,Eq. (1)admitswavesolu- and is useful for the theoretical analysis of lasing insta- tionsoftheformE(z)=E+exp(iknz)+E−exp(−iknz) bilities and perfect absorption. Below we provide some where k =ω/c is the free space wavevector. These solu- exampleswhichillustratetheanomalousscatteringprop- tionsareidenticaltotheonesfoundataninfinitelossless ertiesofaboundedstructurethatincludesaPP-medium. passive medium with index of refraction n. We start our analysis with the investigation of the These similarities between a PP medium and a loss- transportpropertiesofasinglePP-layer. Theassociated less passive medium cease to exist once we turn to the TM that describes the scattering process is analysis of the associated scattering problem involving n µ n µ bounded structures. For simplicity we assume that the M = D(L;n )−1K( p; 0)D(L;n )K( 0; p) (7) domain which contains the pseudo-passive structure ex- 0 n0 µp p np µ0 tends in the interval 0<z <L. We further assume that where the matrices D and K are defined as thescattererisembeddedinahomogeneousmediumwith uctiononinfsoiodrfmerEiqint.dt(eo1x)boaefterteqhfueraallcetftitoonoufnntih0tyewsihc.eiac.tht,ner0fion=rgss1ima.mpTplihlceietzys,o<lwu0e- K(nnml ;µµml ) = (cid:18)12(cid:18)11+−((nnnnmmll ))((µµµµmmll )) 11+−((nnnnmm(cid:19)ll ))((µµµµmmll ))(cid:19) exp(iknL) 0 is E = E+exp(ikz)+E−exp(−ikz) while on its right D(L;n) = (8) L L L 0 exp(−iknL) z > L is E = E+exp(ikz)+E−exp(−ikz). We can R R R relate the amplitudes of forward and backward propa- Using Eq. (4) we evaluate the transmission and reflec- gating waves on the left of the scattering domain with tion amplitudes of a single PP-layer: the amplitudes on its right via the transfer matrix M t= 2exp[−ikL] (9) (cid:18)ER+(cid:19) = M(cid:18)EL+(cid:19). (2) 2cos[knpL]−i(yp+y1p)sin[knpL] ER− EL− r = r = i(yp−y1p)sin(knpL) ; r =rexp(−2ikL) L 2cos[knpL]−i(yp+y1p)sin[knpL] R Incaseofcompositestructuresthetransfermatrix(TM) M is a product of transfer matrices M associated with Thesubindexpindicatesthatwerefertotheconstituents n (cid:113) each individual composite element i.e. M = (cid:81) M . ofthePP-layerandy ≡ (cid:15)p isitscomplexadmittance. n n p µp The individual TM’s are evaluated by imposing the ap- The Fabry-Perrot resonances are defined by the re- propriate boundary conditions at the interface between quirements T = 1 and R = 0 and occur at frequencies consequentlayers nandn+1ofthestructure. ForaTE ω = k c for which sin(k n L) = 0. This implies FP FP FP p mode we have that the field itself is continuous while its perfectresonanttransmissionwithnolossesandnogain, spatial derivative satisfies the relation: regardless of the value of y and despite the fact that p (cid:20) (cid:18) (cid:19) (cid:18) (cid:19)(cid:21) the constituents are complex. Let us now calculate the 1 ∂E (z) 1 ∂E (z) n = n+1 . (3) transportcharacteristicsofthePP-layeratω (cid:54)=ω . For FP µ ∂z µ ∂z n n+1 interface example, at the middle between two consecutive Fabry- Perrot resonances, i.e. when cos[kn L]=0, we have: The transmission t and reflection r amplitudes for p left and right incident waves are defined as t ≡ TEhR+e/yEaL+r,erwLr≡ittEenL−i/nEtL+eramnsdotfRth≡eETL−M/EelR−em,reRnt≡s aEsR+L/ER−. T =(cid:12)(cid:12)(cid:12)yp+21/yp(cid:12)(cid:12)(cid:12)2, R =(cid:12)(cid:12)(cid:12)(cid:12)((yypp+−11//yypp))(cid:12)(cid:12)(cid:12)(cid:12)2, (10) tL = dMet2M2 ,tR = M122,rL =−MM2212,rR = MM1222. (4) A ≡1−T −R = 2(cid:0)(cid:12)(cid:12)yyp2p+−1y(cid:12)(cid:12)p∗2(cid:1)2 =−8(|Iymp2+[yp1]|)22 <0 3 Remarkably, the off-resonance value of A is always neg- energy, due to the PP-layer, gives A≈|E |2Im((cid:15)(cid:48)(cid:48))<0 d ative and independent of the slab thickness L indicating and thus T +R = 1−A (cid:29) 1. The transmission and thatitsoriginisassociatedwithsurfacescatteringrather reflectionspectrumareshowninFig. 2aandconfirmthe than bulk scattering precesses. In fact, it is straightfor- previous expectations. ward to show that a PP-layer will result in amplification The opposite scenario is observed in the case that A<0,foranyfrequencyω,irrespectiveofthesignof(cid:15)(cid:48)(cid:48). the magnetic field H(z) has a maximum in the domain Next we consider the transport properties of a loss- aroundthedefectlayer. Inthiscase T +R=1−A(cid:28)1 less Bragg grating (BG) with one PP-defect layer. We (we recall that A≈|H |2Im(µ(cid:48)(cid:48))>0) and thus we have d assume, without loss of generality, that (cid:15)(cid:48)(cid:48) < 0. Before attenuation of the incident light. going on with our analysis we recall that a lossless pas- The amplification/attenuation mechanism is bet- sive defect layer supports a resonant defect mode with a ter investigated by introducing the overall amplifica- frequency ω lying inside the photonic band gap of the tion/absorption coefficient Θ((cid:15)(cid:48)(cid:48),ω) defined as the ratio r BG. This resonance mode is localized in the vicinity of of the total intensity of outgoing to incoming waves: the defect layer and decays exponentially away from the |E−|2+|E+|2 defect. Near ωr, the entire composite structure displays Θ((cid:15)(cid:48)(cid:48),ω)≡ |EL+|2+|ER−|2 (11) a strong resonant transmission with T = 1 (and thus L R R=0) due to the excitation of the localized mode. Theaboveexpressioncanbewritteninthefollowingform Θ((cid:15)(cid:48)(cid:48),ω)= (cid:12)(cid:12)(cid:12)1+ EERL−+M12(cid:12)(cid:12)(cid:12)2+(cid:12)(cid:12)(cid:12)EERL−+ −M21(cid:12)(cid:12)(cid:12)2 (12) |M22|2(cid:18)1+(cid:12)(cid:12)(cid:12)EER−+(cid:12)(cid:12)(cid:12)2(cid:19) L where we have used the fact that detM = 1. The case Θ((cid:15)(cid:48)(cid:48),ω) > 1 indicates that an overall amplification has been achieved at the system. The opposite limit of Θ((cid:15)(cid:48)(cid:48),ω) < 1 corresponds to attenuation. The two ex- treme cases of Θ((cid:15)(cid:48)(cid:48),ω ) → ∞ and Θ((cid:15)(cid:48)(cid:48) ,ω ) → 0 L L CPA CPA indicate that the system has reached a lasing instability or behaves as a coherent perfect absorber (CPA) respec- tively. TheconditionfortheformercaseisM ((cid:15)(cid:48)(cid:48),ω)= 22 0 which is satisfied for some values (cid:15)(cid:48)(cid:48) =(cid:15)(cid:48)(cid:48) and ω =ω . L L Infact,thecomplexzerosofM correspondtothepoles 22 of the scattering matrix S, see Eq. (6). If (cid:15)(cid:48)(cid:48) =0 they lie at the lower part of the complex-ω plane due to causal- FIG. 2: (color online) (a) The transmittance T(ω), re- flectance R(ω) and absorption A(ω) for the set-up of Fig. ity. As|(cid:15)(cid:48)(cid:48)|increasesthepolesmovetowardstherealaxis 1 ((cid:15)(cid:48)(cid:48) < 0). A super-unitary transmittance and reflectance andatacriticalvalue(cid:15)(cid:48)(cid:48) =(cid:15)(cid:48)(cid:48) oneofthesepolesbecomes L is evident in the frequency domain around the resonance fre- realω =ω , thussignifyingthetransitiontoalasingac- L quency. (b)Theamplification/absorptioncoefficientΘversus tion. We have confirmed in Fig. 2b that the singularity frequency has a singular point at resonance frequency which in Θ((cid:15)(cid:48)(cid:48) = (cid:15)(cid:48)(cid:48),ω = ω ) → ∞ corresponds to the lasing signifies a lasing action. (c) The same set-up as in Fig. 1 for L L point as it is calculated from the analysis of the poles of the case of CPA frequency. In this case the electric field as the associated scattering matrix. a minimum at the defect layer while the magentic field has a maximum (d) The amplification/absorption coefficient Θ The other limiting case of CPA is achieved when the versus frequency shows a zero at the CPA frequency. two terms in the numerator of Eq. (12) become simul- taneously zero i.e. when E− = E+M and E− = R L 21 R A completely different scenario emerges when the de- −E+/M . These two relations are simultaneously sat- L 12 fectlayerconsistsofaPP-medium. Wefindthattheres- isfied when M M + 1 = 0 → M M = 0 (re- 21 12 11 22 onancelocalizedmodehastransmittanceandreflectance call that detM = 1). The CPA frequency ω = ω CPA values which are larger (smaller) that unity in distinct is evaluated from the condition M (ω ) = 0 (the 11 CPA contrast to the case of lossless defect layers. The super frequencies for which M (ω) = 0 are excluded since 22 (sub)-unitary transmission/reflection is related with the they correspond to lasing action). It should be stressed distribution of the electro-magnetic field around the PP- that a CPA requires coherent incident fields which sat- defect. Letusconsiderthecaseforwhichtheelectricfield isfy an appropriate phase and amplitude relationship E(z) takes its maximum value (anti-nodal point) at the E− = E+M = −E+/M . An example of a CPA R L 21 L 12 positionofthedefectlayer(seeFig. 1). Obviouslytheas- is shown in Fig. 2d. sociatedmagneticfieldH(z)willbehavinganodalpoint The above super/sub-unitary scattering features be- at the defect layer. Then, an estimation of the absorbed comemorepronouncedwhenoneofthecompositelayers 4 of the Bragg grating is substituted by a pseudo-passive netic field node) in the middle of each A-layer [33]. As a medium. Specifically, the Fabry-Perrot (FP) resonances consequence, Fabry-Perrot resonances close to neighbor- which are closer to the band edges will correspond to ing photonic band edges will have different dominating photons with small group velocities. Therefore each in- components-electricormagnetic-oftheoscillatingfield dividualphotonatthisfrequencyresidesinthePP-layers inside a particular layer. for a long time. This long time interaction with the PP- InourexampleinFig. 3theA-layersconsistsofaPP- medium leads to strong amplification/attenuation fea- medium with negative (cid:15)(cid:48)(cid:48) and positive µ(cid:48)(cid:48), which means tures. The magnitude of the enhancement/suppression thattheFabry-Perrotresonanceswiththedominantelec- is a growing function of the total thickness of the stack, tric field component in the A-layers will be enhanced, asopposedtothecaseofauniformpseudo-passiveslab. while the resonances with dominant magnetic field com- In Fig. 3 we show a typical transmission spectrum of ponentintheA-layerswillbesuppressed. Thisisexactly such composite structure. whatweseeinFig. 3,wheretheresonanttransmissionat everyotherphotonicbandedgeisenhanced(suppressed). In conclusion, we have introduced a class of pseudo- passive metamaterials for which the losses are balanced by gain in a way that the index of refraction is real and uniform throughout the medium. Although the light propagation in an unbounded pseudo-passive medium has the same characteristics as in a passive lossless medium with the same index of refraction, their scat- tering properties differ dramatically. When such me- dia are incorporated in a photonic structure, it can lead to super/sub-unity transmittance/reflectance indicating strong absorption and amplification mechanisms for the total structure. In many occasions these effects can turn to a coherent perfect absorption of incident waves or to lasing instabilities. It will be interesting to investigate the realization of these phenomena under vectorial con- FIG. 3: (color online) The electric E(z) (blue line at y-z ditions and in higher dimensions. plane)andthemagneticH(z)(redlineatthex-zplane)fields Acknowledgment - This work was partially supported oftworepresentativeFPmodeswhichresideattheupper(left by an AFOSR MURI grant FA9550-14-1-0037, by a inset)andlower(rightinset)bandedges. Thegratingconsists LRIR-09RY04COR,andbyaNSFECCS-1128571grant. of50bilayers(orangeindicatesaPP-layerandwhitealossless passive layer). In the insets we show the field profiles for the first half of the structure, i.e. 25 layers. 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