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Ionization Waves in Electrical Breakdown of Gases PDF

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Ionization Waves in Electrical Breakdown of Gases A.N. Lagarkov 10M. Rutkevich Ionization Waves in Electrical Breakdown of Gases With 50 Figures Springer-Verlag New York Berlin Heidelberg London Paris Tokyo Hong Kong Barcelona Budapest A.N. Lagarkov I.M. Rutkevich Center for Applied Problems Department of Mechanical Engineering of Electrodynamics Ben-Gurion University of the Negev Russian Academy of Sciences Beer Sheva 84105 Izhorskaya 13/19 Israel 127412 Moscow Russia -Library of Congress Cataloging-in-Publication Data Lagar'kov, A. N. (Andrei Nikolaevich) Ionization waves in electrical breakdown of gases / A.N. Lagarkov and I.M. Rutkevich. p. cm. Includes bibliographical references. ISBN-13:978-1-4612-8727 ·8 1. Breakdown (Electricity). 2. Electric discharges through gases. 3. Gases, Ionized. 4. Plasma waves. I. Rutkevich, I. M. (Igor Maksimovich) II. Title. QC71 1.8 .B7L34 1993 537.5' 32 - dc20 93-27847 Printed on acid-free paper. © 1994 Springer-Verlag New York, Inc. Softcover reprint of the hardcover 1st edition 1994 All rights reserved. This work may not be translated or copied in whole or in part without the written permission of the publisher (Springer-Verlag New York, Inc., 175 Fifth Avenue, New York, NY 10010, USA), except for brief excerpts in connection with reviews or scholarly analysis. Use in connection with any form of information storage and retrieval, electronic adaptation, computer software, or by similar or dissimilar methodology now known or hereaf ter developed is forbidden. The use of general descriptive names, trade names, trademarks, etc., in this publication, even if the former are not especially identified, is not to be taken as a sign that such names, as understood by the Trade Marks and Merchandise Marks Act, may accordingly be used freely by anyone. Production managed by Hal Henglein; manufacturing supervised by Vincent R. Scelta. Camera ready copy prepared from the authors' TeX files. 987654321 ISBN-13:978-1-4612-8727 -8 e-ISBN-13:978-1-4612-4294·9 DOl: 10.1007/978-1-4612-4294·9 Preface In the years since the book of Lozanskii and Firsov "The Theory of Spark" [1975] was published, a number of experimental and theoretical studies in the physics of electric breakdown in gases were conducted. As a result of these studies, the concept of a wavelike nature of breakdown initiated by single high-voltage electric pulses or by a constant electric field was confirmed. Theoretical models in which the concept of breakdown in a constant external field was developed were first exposed in the above-named book in the chapter "Development of a streamer regarded as an ionization wave," written by Rodin and Starostin. This book treats the initial stage of electric breakdown as a wave pro cess. The wavelike nature of the phenomena under consideration is pre sented for streamers and sliding discharges, for electric breakdown develop ment in long discharge tubes as well as in gas-filled gaps. Chapter 1 gives a qualitative consideration of phenomena determin ing the electric breakdown of gases. The experimental data and theoretical results are exposed and discussed with application to streamers, plane ion ization waves, breakdown waves in long tubes, and propagation of sliding discharges. The subject of this chapter may be considered as an area of applications of different theoretical models, formulas, and estimates that are presented in other chapters of the book. Chapter 2 addresses the problem of obtaining a closed system of macro scopic equations intended for the description of the electric breakdown phenomena. In the case of strong electric fields existing in high-voltage discharge devices, the deviation of the electron distribution function from the equilibrium Maxwell distribution becomes essential. In this case, the problem of calculating correctly the effective frequency of ionization, the electron mobility, and other quantities entering into the equations of hydro dynamics and macroscopic electrodynamics arises. This chapter is written as a review and contains formulas for macroscopic description of ioniza tion waves, including the estimations of their validity. In most theoretical models of electric breakdown waves, a local dependence of the frequency of ionization upon the electric field is used. In this connection, great attention vi Preface is paid to the discussion of the conditions for applicability of such a local approach. In Chapter 3, the theory of plane electric breakdown waves is devel oped for the cases of stationary and time-dependent propagation. Station ary ionization waves belong to the class of autowaves in active media that can propagate only by the permanent action of an external source of en ergy. From the mathematical point of view, the theory of plane breakdown waves is similar to the theory of biological population waves proposed by Kolmogorov et al. The problem of determining stationary ionization wave in a given constant applied field has a continuum of solutions corresponding to a continuous spectrum of possible velocities of propagation. Analysis of the time-dependent problem based on the solution of the Cauchy problem gives a method of selection of any stationary wave with a given velocity of propagation regarded as the asymptotics of a nonstationary solution with proper initial data. Chapter 3 also contains an analysis of the formation of the moving anode-directed discontinuities of electron density. The mechanism of the formation of these discontinuities (ionization shocks) differs from the well known mechanism of breaking the Riemann waves, leading to the formation of shock waves in classical gas dynamics. Chapter 4 treats the propagation of ionizing waves of electric field in long shielded discharge tubes filled with a preliminary ionized gas. Accord ing to Loeb, these waves may be called "the ionizing waves of potential gradient." Experimental studies of breakdown waves in long tubes were carried out for many years. First observations of such waves were made as long ago as the 19th century by Wheatstone and Thompson. For a long period, rich experimental material has been stored, and the main observed properties of breakdown waves in tubes have been systematized. However, the closed theoretical description, which allows us to calculate the structure of these waves and the velocities of their propagation, has appeared only recently. Unlike the case of a plane discharge gap, the electric field in a shielded tube attenuates far ahead of the breakdown wave front. The leading edge of such a wave is determined by a wave of surface charge propagating along the plasmald ielectric wall boundary. The spatial scale of the ionization wave depends upon the geometrical parameters of a discharge device as well as on the degree of preliminary ionization. In order to describe the ionization wave propagation, a proper quasi-one-dimensional system of equations is formulated. Numerical and analytical solutions of this system are obtained in the form of stationary waves. These solutions show that the electric breakdown development in a long tube is connected with propagation of a solitary wave of an electric field. The equations describing solitary ionizing waves did not appear previously in the nonlinear theory of wave propagation in active media. Preface vii In Chapter 4, some peculiarities of the breakdown wave structures are considered, including the oscillating structure of the trailing edge of the ionization front and the solitary waves in a longitudinal magnetic field. Chapter 5 contains a generalization of the theory of ionizing solitary waves to the case of wave propagation in an unpreionized inert gas. It is assumed that generation of electrons ahead of the ionization front is deter mined by the associative ionization and the resonance radiation transfer. The results of numerical modeling of stationary waves propagating along the plasma/dielectric boundary in shielded tubes and in sliding discharge systems are presented. Similar to the motion of a breakdown wave in a tube, the propaga tion of a sliding discharge front is stipulated by a two-dimensional wave of an electric field. The transverse component of the electric field near the dielectric surface is shown to play an important role in the development of impact ionization and in the formation of a plasma sheet behind the ionization front. The theoretical model describing the propagation of slow stationary breakdown waves in tubes is presented. An important feature of these waves is the influence of ionic current on the mechanism of propagation. The effect of a longitudinal magnetic field on the structure of a slow solitary wave also is examined. The final section touches upon the problem of high-voltage breakdown waves. Runaway electrons arising at the wave front may be accelerated in the electric field of a solitary wave up to very high energies, and the relativistic approach to the problem in question is developed to describe this situation. The value of limiting electron energy that may be reached under these conditions is found. The comparison of theoretical and experimental results is given in the text, where possible. Since the book treats special topics, it does not cover all of the various phenomena existing in the electric breakdown of gases. The books concerning other aspects of the electric breakdown are listed in the references. We are grateful to E.L Asinovskii, L.M. Biberman, G.A. Lyubimov, A.Kh. Mnatsakanyan, A.V. Nedospasov, Yu.P. Raizer, A.A. Rukhadze, O.A. Sinkevich, A.N. Starostin, and LT. Yakubov for valuable discussion of a number of problems considered in this book. We also thank V.A. Vino gradov for his assistance in preparation of the manuscript. We wish to acknowledge E.E. Kunhardt and R. Morrow, who sent us the reprints of their papers used in Chapter 1. Finally, we wish to express our thanks to Springer-Verlag New York for their encouragement in preparing this book and excellent editorial work with our manuscript. Contents Preface .......................................................... v Chapter 1. Wave Phenomena Determining Discharge Development in Gas Gaps .................................................... " 1 1 DynaIllics of StreaIllers ......................................... " 2 1.1 Development of an Electron Avalanche ........................ 2 1.2 Propagation of Anode- and Cathode-Directed StreaIllers ....... 11 2 Ionization Waves in Discharge 'lUbes and in a Sliding Discharge Formation System .................................... 23 2.1 Experimental Study of Ionization Waves in Discharge 'lUbes ............................................ 24 2.2 Formation of a Sliding Discharge ............................. 30 Chapter 2. Macroscopic and Kinetic Description of a Weakly Ionized Gas in an Electric Field . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. 35 1 Basic Macroscopic Equations .. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. 35 2 Local Approach for the Frequency of Impact Ionization . . . . . . . . . . .. 48 2.1 The Townsend Ionization Coefficient and the Frequency of Ionization by an Electronic Impact . . . . . . . . . . . . . . . . . . . . . . . .. 48 2.2 Conditions of Applicability of the Local Approach. Equation for the Electron Distribution Function over Energies in a Nonuniform, Nonstationary Plasma ........................... 51 Chapter 3. Theory of Plane Ionization Waves. . . . . . . . . . . . . . . . . . . . . .. 59 1 Stationary Plane Electric Breakdown Waves ......... , ............ 59 1.1 Ionization-Drift Models of Anode- and Cathode-Directed Waves ..................................... 60 1.2 Influence of Diffusion and Photoprocesses on the Plane Breakdown Waves. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. 75 2 General Properties of Nonstationary Ionization Fronts ............. 94 2.1 Integrals of Nonstationary Equations. Reduction of a General Problem to the Cauchy Problem for the Electric Field Distribution. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. 94 x Contents 2.2 Solution of the Cauchy Problem by the Method of Characteristics. Conditions for the Breaking of a Continuous Solution. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. 99 2.3 Propagation of Strong and Weak Discontinuities of Electron Concentration. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. 103 3 Dynamics of Formation of the Anode- and Cathode-Directed Waves from Initial Nonuniformities. . . . . . . . . . . . . . . . . . . . . . . . . . . . .. 118 3.1 Asymptotic Behavior of the Solution of the Cauchy Problem for a Finite Initial Distribution of Electron Concentration ..................................... 118 3.2 Development of Ionization Waves from Infinitely Extended Distribution of Electron Concentration 127 Chapter 4. Propagation of Ionizing Electric-Field Solitary Waves in Shielded Discharge Tubes with Preionization ........................................ 145 1 Basic Equations and Assumptions. . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. 145 2 The Effect of the Surface Wave on the Formation of the Ionization Wave ......................................... 147 3 Averaging Two-Dimensional Equations and Formulation of a Quasi-One-Dimensional Model .................. 149 4 Numerical Simulation of Stationary Waves ....................... 153 5 Analytical Model of an Ionization Wave .. . . . . . . . . . . . . . . . . . . . . . .. 160 6 Specialized Problems of the Theory of Breakdown Waves in Tubes with Preionization .............................. 164 6.1 Limiting Transition to a Nonlinear Model of the Electric Potential Diffusion. Conditions of Nonmonotonic Increase of Current in a Wave ....................................... 164 6.2 Emergence of the Oscillating Structure of an Ionization Wave. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. 169 6.3 The Effect of a Longitudinal Magnetic Field on the Structure of a Fast Ionization Wave. . . . . . . . . . . . . . . . . . . . . . . . .. 175 Chapter 5. Propagation of Electric Breakdown Waves Along a Gas-Dielectric Boundary With No Preionization ................. 185 1 Breakdown Waves in Shielded Tubes Without Preionization . . . . . .. 186 1.1 Taking Account of Associative Ionization and Resonance Radiation Transfer ............................... 186 1.2 Results of Numerical Calculations of Breakdown Stationary Waves .......................................... 188 1.3 Analytical Estimate of Breakdown Wave Velocity ............. 192 2 Propagation of a Sliding Discharge Front as an Ionization Wave. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. 194 2.1 Assumed Equations and Problem Statement .................. 194 2.2 Formulating a Calculated Model of a Stationary Wave ......... 196 Contents xi 2.3 Structure and Velocity of Front Propagation ................. 201 3 Slow Breakdown Waves in Shielded Thbes ........ . . . . . . . . . . . . . .. 207 3.1 Features of a Quasi-One-Dimensional Solution Describing Slow Waves ..................................... 208 3.2 Influence of a Longitudinal Magnetic Field on the Structure of Slow Waves. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. 212 4 Solitary Wave of an Electric Field as a Source of Runaway Electrons . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. 214 References. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. 221 Chapter 1 Wave Phenomena Determining Discharge Development in Gas Gaps The phenomena of breakdown in gas under the effect of impulse voltage are extremely variegated. As shown in the monographs by Meek and Craggs [1953], Raether [1964], and Korolev and Mesyats [1991]' the process of breakdown formation is governed by numerous external conditions includ ing, to a considerable extent, the value of overvoltage and the specifics of the emergence of initiating electrons [the overvoltage is characterized by the coefficient K = (Uo - Ubr)/Ubn where Uo is the pulse amplitude and Ubr the value of static breakdown voltage corresponding to Paschen's law]. Best studied at present is the Townsend mechanism of breakdown starting with the development of solitary avalanches. In the case of Townsend breakdown, the appearing space charge has little effect on the value of the electric field inside the breakdown gap. The Townsend mechanism of breakdown usually is observed at low values of K Ph, where P is the gas pressure and h is the size of the interelectrode gap. In the case of high values of the K Ph parameter, a situation is possible when the appearance and propagation of a space charge serves one of the most important features characterizing the breakdown development. In this case, the breakdown exhibits a clearly pro nounced wave behavior. The closing of the breakdown gap by ionized gas occurs owing to the motion of the high ionization region from one electrode towards another, as observed, for instance, in discharge tubes or, as often happens in the case of the streamer mechanism of breakdown, from the gap center in both directions to each one of the electrodes. In some cases, the wave breakdown occurs even at low values of K Ph. For instance, Korolev and Mesyats indicate that if numerous electrons are initiated on a cathode area whose size is less than the avalanche diffusion radius, the breakdown will be of the streamer type in spite of low overvoltages. The specific features of breakdown waves that will be regarded are determined by the type of gas, the value of pressure, the value and rate of variation of voltage at the electrodes, and by the geometry of a discharge cell. The geometry determines the space distribution of the applied electric field, so structure and dynamics of ionization front are greatly dependent on it. The ionization waves described below are always characterized by the presence of space charge, which leads to external electric field screening

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