IIIIInnnnntttttrrrrroooooddddduuuuuccccctttttiiiiiooooonnnnn tttttooooo NNNNNuuuuucccccllllleeeeeaaaaarrrrr RRRRRaaaaadddddiiiiiaaaaatttttiiiiiooooonnnnn DDDDDeeeeettttteeeeeccccctttttooooorrrrrsssss LLLLAAAABBBBOOOORRRRAAAATTTTOOOORRRRYYYY IIIINNNNSSSSTTTTRRRRUUUUMMMMEEEENNNNTTTTAAAATTTTIIIIOOOONNNN AAAANNNNDDDD TTTTEEEECCCCHHHHNNNNIIIIQQQQUUUUEEEESSSS SSSSeeeerrrriiiieeeessss EEEEddddiiiittttoooorrrr:::: GGGGaaaalllleeeennnn WWWW.... EEEEwwwwiiiinnnngggg SSSSeeeettttoooonnnn HHHHaaaallllllll UUUUnnnniiiivvvveeeerrrrssssiiiittttyyyy VVVVoooolllluuuummmmeeee IIII:::: TTTThhhheeee LLLLaaaabbbboooorrrraaaattttoooorrrryyyy RRRReeeeccccoooorrrrddddeeeerrrr BBBByyyy GGGGaaaalllleeeennnn WWWW.... EEEEwwwwiiiinnnngggg aaaannnndddd HHHHaaaarrrrrrrryyyy AAAA.... AAAAsssshhhhwwwwoooorrrrtttthhhh ----1111999977774444 VVVVoooolllluuuummmmeeee 2222:::: IIIInnnnttttrrrroooodddduuuuccccttttiiiioooonnnn ttttoooo NNNNuuuucccclllleeeeaaaarrrr RRRRaaaaddddiiiiaaaattttiiiioooonnnn DDDDeeeetttteeeeccccttttoooorrrrssss BBBByyyy PPPP.... JJJJ.... OOOOuuuusssseeeepppphhhh ---- 1111999977775555 AAAA CCCCoooonnnnttttiiiinnnnuuuuaaaattttiiiioooonnnn OOOOrrrrddddeeeerrrr PPPPllllaaaannnn iiiissss aaaavvvvaaaaiiiillllaaaabbbblllleeee ffffoooorrrr tttthhhhiiiissss sssseeeerrrriiiieeeessss.... AAAA ccccoooonnnnttttiiiinnnnuuuuaaaattttiiiioooonnnn oooorrrrddddeeeerrrr wwwwiiiillllllll bbbbrrrriiiinnnngggg ddddeeeelllliiiivvvveeeerrrryyyy ooooffff eeeeaaaacccchhhh nnnneeeewwww vvvvoooolllluuuummmmeeee iiiimmmmmmmmeeeeddddiiiiaaaatttteeeellllyyyy uuuuppppoooonnnn ppppuuuubbbblllliiiiccccaaaattttiiiioooonnnn.... VVVVoooolllluuuummmmeeeessss aaaarrrreeee bbbbiiiilllllllleeeedddd oooonnnnllllyyyy uuuuppppoooonnnn aaaaccccttttuuuuaaaallll sssshhhhiiiippppmmmmeeeennnntttt.... FFFFoooorrrr ffffuuuurrrrtttthhhheeeerrrr iiiinnnnffffoooorrrrttttnnnnaaaattttiiiioooonnnn pppplllleeeeaaaasssseeee ccccoooonnnnttttaaaacccctttt tttthhhheeee ppppuuuubbbblllliiiisssshhhheeeerrrr.... Introduction to Nuclear Radiation Detectors PJOuseph Department of Physics College of Arts and Sciences University of Louisville Louisville, Kentucky PLENUM PRESS • NEW YORK AND LONDON Library of Congress Cataloging in Publication Data Ouseph, P J 1933· Introduction to nuclear radiation detectors. (Laboratory instrumentation and techniques ; v. 2) Bibliography: p. Includes index. 1. Nuclear counters. I. Title. QC787.C6088 539.7'7 75·15744 ISBN-13: 978-1-4684-0837-9 e-ISBN-13: 978-1-4684·0835·5 DOl: 10.1007/978·1-4684-0835-5 @1975 Plenum Press, New York Softcover reprint of the hardcover 18t edition 1975 A Division of Plenum Publishing Corporation 227 West 17th Street New York N.Y. 10011 United Kingdom edition published by Plenum Press, London A Division of Plenum Publishing Company, Ltd. Davis House (4th Floor), 8 Scrubs Lane, Harlesden, London NWI0 6SE, England All rights reserved No part of this book may be reproduced, stored in a retrieval system, or transmitted, in any form or by any means, electronic, mechanical, photocopying, microfilming, recording, or otherwise, without written permission from the Publisher To Ann, Rosemary, John, and Maryann Preface There have been many interesting developments in the field of nuclear radiation detectors, especially in those using semiconduct ing materials. The purpose of this book is to present a survey of the developments in semiconductor detectors along with discus sions about gas counters and scintillation counters. These discus sions are directed to detector users, usually scientists and technicians in different fields such as chemistry, geology, bio chemistry, and medicine. The operation of these detectors is discussed in terms of basic properties, such as efficiency, energy resolution, and resolving time, which are defmed in the first chapter. Differences among these detectors in terms of these properties are pointed out. Chapter 2, on interaction of radiations with matter, discusses how different radiations lose energies in matter and how differences in their behavior in matter affect the design and operation of detectors. Although emphasis is placed on fundamentals throughout the book, the reader is also made aware quite often of the new developments in the field of radiation detection. The author has taught a course in radioisotopes for several years for science, engineering, medical, and dental students. The emphasis on topics varied from time to time to satisfy the varying interests of the students. However, the contents of this book formed the core of the course. About ten selected experiments on detectors were done along with this course (a list of these vii viii Preface experiments may be supplied on request). The enthusiastic response received from the students encouraged the writing of this book. The help I received from several individuals during the preparation of this book deserves special mention. Professor Manual Schwartz initiated and developed the course on radioiso topes and radiation detection at our university. As mentioned earlier, this book originated with this course, modified through years of teaching. Without his help in reading, correcting and modifying the manuscript, especially in its early stages, this book would not have been possible. I am deeply indebted to Professor Schwartz for this help and for his collaboration in writing two articles on detectors which gave me additional impetus in writing this book. I should also acknowledge the help I received from Thomas Lanigan and Ralph Cutler of the editorial staff of Plenum Press. I am especially grateful to Dr. Galen Ewing, the editor of this series, for his patient efforts in correcting and editing this book. In preparing the diagrams, the help I received from Mrs. Catherine M. Bauscher deserves special recognition. Nor should I forget the assistance provided by Miss Lisa Hark in the typing of this manuscript. Finally, my appreciation goes to my family for their patience and encouragement. Louisville, Kentucky P. J. OUSEPH May, 1975 Contents Chapter 1 INTRODUCTION 1 Chapter 2 NUCLEAR RADIATIONS AND THEIR INTERACTION WITH MATTER _________________ ~------------------- 7 2.1. Radioactivity __________________________________ 8 2.2. Radioactivity Calculations ______________________ 10 2.3. Calculation of Activities Produced by Nuclear Reactions ____________________________________ 15 2.4. Interaction of Heavy Charged Particles with Matter 20 2.5. Electron Interaction ____________________________ 29 2.6. Backscattering of Electrons ____________________ 34 2.7. Interaction of Gamma and X Rays with Matter 37 2.8. Interaction of Neutrons ________________________ 44 2.9. Cosmic Rays __________________________________ 46 References ____________________________________ 46 Bibliography __________________________________ 46 Chapter 3 GAS COUNTERS ______________________________________ 47 3.1. General Properties of Gas Counters ______________ 47 ix x Contents 3.2. Ionization Counters ____________________________ 52 3.3. Air-Wall Ionization Chamber ____________________ 52 3.4. Pocket Dosimeter ______________________________ 53 3.5. Pulse-Type Ionization Counter __________________ 54 3.6. Proportional Counter __________________________ 60 3.7. Position-Sensitive Proportional Counters ________ 66 3.8. Neutron Counters ____________________________ 67 3.9. Geiger-Miiller Counters ________________________ 68 3.10. Counter Gas __________________________________ 74 3.11. Detection of Alpha and Beta Radiations by Geiger Counters ______________________________ 76 3.12. Detection of X Rays and Gamma Rays by Gas Counters ________________________________ 77 3.13. Application of Internal Counting Methods ________ 79 References ____________________________________ 81 Bibliography __________________________________ 82 Chapter 4 SCINTILLATION COUNTERS .. _____ • __ .. _. .._ ____ 83 ~-----__ 4.1. General Characteristics of Scintillation Counting Systems .. _______________ .________ 83 4.2. Scintillant Materials and Mechanism of Scintillation 85 4.3. Photomultipliers .. ____________________________ 95 4.4. The Shape of the Pulse _________ .. _____ .. ________ 100 4.5. Scintillation Counter Assembly __________________ 101 4.6. Relationship between Pulse Height and Energy 102 4.7. Detection of Gamma Rays by Scintillation Counters ______________________________________ 104 4.8. Integral Counting ______________________________ 109 4.9. Differential Counting and Determination of Energy of Gamma Rays ________________________ 111 4.10. Efficiency of Scintillation Counters for Gamma Detection ____________________________ 115 4.11. Energy Resolution in Scintillant Detectors ________ 117 Contents xi 4.12. Detection of Charged Particles with Scintillation Counters ___________________________ 120 4.13. Detection of Neutrons __________________________ 121 4.14. Particle Identification by Pulse Shape Discrimination _________________________________ 123 4.15. Other Methods for Particle Identification and Discrimination ________________________________ 124 References ____________________________________ 127 Bibliography __________________________________ 127 Chapter 5 SEMICONDUCTOR DETECTORS 129 5.1. Operation of a Semiconductor Counter __________ 129 5.2. Impurity Semiconductors ______________________ 133 5.3. Detector Types ________________________________ 140 5.4. Pulse Shape and Rise Time ____________________ 148 5.5. Factors Affecting Energy Resolution ____________ 149 5.6. Radiation Damage ____________________________ 152 5.7. Detection of Charged Particles __________________ 153 5.8. X-Ray and Gamma-Ray Detection ______________ 158 5.9. Neutron Detectors ____________________________ 161 5.10. Other Applications ____________________________ 161 5.11. Special Techniques ____________________________ 164 5.12. Concluding Remarks __________________________ 166 References __________________________________ 167 Bibliography ________________________________ 167 Chapter 6 CORRECTIONS IN RADIATION COUNTING 169 6.1. Introduction __________________________________ 169 6.2. Absolute Activity Determination ________________ 178 6.3. Random Nature of Decay Process ______________ 180 6.4. Frequency Distributions ________________________ 181 6.5. Statistical Errors in Nuclear Particle Counting ____ 185 References ____________________________________ 187 Bibliography __________________________________ 187