Intermediate-Energy Nuclear Physics A. S. Iljinov M. V. Kazarnovsky E. Ya. Paryev Institute for Nuclear Research of the Academy of Sciences of Russia Moscow, Russia Boca Raton London New York CRC Press is an imprint of the Taylor & Francis Group, an informa business First published 1994 by CRC Press Taylor & Francis Group 6000 Broken Sound Parkway NW, Suite 300 Boca Raton, FL 33487-2742 Reissued 2018 by CRC Press © 1994 by CRC Press, Inc. CRC Press is an imprint of Taylor & Francis Group, an Informa business No claim to original U.S. Government works This book contains information obtained from authentic and highly regarded sources. Reasonable efforts have been made to publish reliable data and information, but the author and publisher cannot assume responsibility for the validity of all materials or the consequences of their use. 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CCC is a not-for-profit organization that provides licenses and registration for a variety of users. For organizations that have been granted a photocopy license by the CCC, a separate system of payment has been arranged. Trademark Notice: Product or corporate names may be trademarks or registered trademarks, and are used only for identification and explanation without intent to infringe. Library of Congress Cataloging-in-Publication Data Il’inov, A. S., 1944- Intermediate-energy nuclear physics/A.S. Iljinov, M.V. Kazarnovsky, E. Ya. Paryev. p. cm. Includes bibliographical references and index. ISBN 0-8493-4827-7 1. Nuclear reactions. 2. Hardron Interactions. I. Kazarnovskii, M. V. II. Par’ev, E. IA. III. Title. Qc794.144 1993 539.7’5--dc20 93-9456 A Library of Congress record exists under LC control number: 93009456 Publisher’s Note The publisher has gone to great lengths to ensure the quality of this reprint but points out that some imperfections in the original copies may be apparent. Disclaimer The publisher has made every effort to trace copyright holders and welcomes correspondence from those they have been unable to contact. ISBN 13: 978-1-315-89470-6 (hbk) ISBN 13: 978-1-351-07380-6 (ebk) Visit the Taylor & Francis Web site at http://www.taylorandfrancis.com and the CRC Press Web site at http://www.crcpress.com PREFACE During the last two decades, qualitatively new high-intensity proton accelerators up to 1 GeV with mean current of about 1 rnA have been created. These are the so-called "meson facilities". The "kaon facilities", i.e., high-intensity proton accelerators which produce particles with energies of several tens Ge V, are currently being constructed. As a result of the interaction of such protons with various targets, intensive secondary beams of neutrons, pions, kaons, antinucleons and other par- ticles, as well as radionuclides, are generated. All such particles are usually called intermediate-energy particles and their interaction with nuclei is referred to as intermediate-energy nuclear reactions. The high intensity of beams of intermediate-energy particles makes it possible to carry out experimental investigations of their interaction with nuclei with a high degree of statistical reliability. Owing to the considerable advances made in in- strument design and the methods used for registering the products of nuclear re- actions and computerization of the experimental procedure, the possibilities to obtain, process, and analyze a large body of experimental data have grown con- siderably. All this ensures a rapid influx of data (and a significantly higher order of accuracy) on nuclear reactions in the intermediate-energy range. A large body of such information has been accumulated so far. In turn, these developments have given impetus to intensive theoretical studies in this field, especially to the study of deep inelastic processes, such as branched nucleonic-mesonic cascade and break-up of highly-excited nuclei, which are char- acteristic of the energy range under consideration. On the other hand, the entire body of this information has not been systematized. Our monograph aims at r.IIing this gap. In this connection, it should be emphasized that intermediate-energy nuclear physics has two peculiar features which make it a separate line of scientific inves- tigation. Indeed, nuclear reactions in the domain of low energies have, as a rule, a relatively small number of open channels (witb the only exception being that of fission of heavy nuclei). Therefore, the exclusive experimental and corresponding theoretical investigation of a reaction is quite possible and often realized in practice. As the energy increases, new channels readily open and, in particular, channels involving the emission of an every-increasing number of particles. In this case, complete, exclusive experimental investigation of a reaction involves considerable difficulties and, finally, becomes practically impossible in spite of the previously mentioned achievements of the experimental technique. This is just the case in the domain of intermediate energies. This is the first peculiarity that distinguishes this energy range. The second peculiarity is associated with specific features of the theoretical description of nuclear reactions in this energy range. In this instance a statistical approach must be used to describe such a complicated and branched nuclear process involving a large number of different states of the system at the same energy. Moreover, in this energy range the wavelength of an incident hadron is small as compared to the separation between nucleons in a nucleus; its energy is large as compared to the mutual interaction energy and the kinetic energy of intranuclear nucleons. Therefore, to describe the behavior of intermediate-energy particles in a nucleus we can use simplified approaches (such as semiclassical, eikonal, and other approximations) which are characteristic of this energy range. The monograph is devoted mainly to the interaction of hadrons with nuclei which leads to the excitation of a large number of degrees of freedom in a nucleus and, as a result, to the emission of several particles during an intranuclear cascade and subsequent decay of a highly-excited residual nucleus. These processes are described on the basis of a unified approach which reflects the peculiar features of intermediate-energy nuclear physics as outlined. Namely, the stage of an intranuclear cascade and the characteristics (distributions over the number of protons and neu- trons, over the excitation energy, etc.) of a residual nucleus are treated by the method of classical (more precisely, semiclassical) kinetic equations, whereas the decay of a residual nucleus is described within the framework of a statistical model. The methods and results of the calculation of probabilities of various processes initiated by intermediate-energy hadrons in nuclei and experimental data are set forth and discussed. The possibility of obtaining information on the structure and properties of nuclei, in particular on the properties of highly-excited nuclear matter, by comparing the experimental data with the theoretical results is analyzed. Special attention is paid to new issues, like analytic methods for solution of kinetic equations describing the cascade. In particular, the exclusive description of an intranuclear cascade on the basis of the Liouville equation is given for the first time, to our knowledge, in Chapter 1. Other new areas of attention are nuclear absorption of hadrons from bound states of hadronic atoms, interaction of antinucleons with nuclei, multifragmentation of highly-excited residual nuclei, and polarization phe- nomena. These also have not been previously discussed in detail in the current literature. The study of the interaction between nuclei, which is closely related to the previously mentioned issues, is a separate, large problem which is extensively studied in the literature. Therefore, we shall not dwell on this problem here. How- ever, a peculiar nature of physics of hadron-nucleus interactions which bridges the gap between low-energy nuclear and heavy-ions physics will be demonstrated. This range of issues can be useful in the analysis of problems associated with the evolution of the early (hot) universe, neutron stars and supernovas, and in solving a number of applied problems (e.g., the problems associated with the after- burning of radioactive waste in nuclear energy installations and with electronuclear breeding of energy). In conclusion, the authors would like to express their thanks to Andrei R. Isaakian who worked laboriously and skillfully to present this book in English. Additionally, A. S. I1jinov is grateful to his co-authors, V. S. Barashenkov, A. S. Botvina, E. A. Cherepanov, S. E. Chigrinov, F. G. Gereghi, Ye. S. Golubeva, K. K. Gudima, S. G. Mashnik, M. V. Mebel, I. N. Mishustin, V. I. Nazaruk, I. A. Pshenichnov, N. M. Sobolevsky, and V. D. Toneev, with whom he developed models of nuclear reactions, for helpful discussions and fruitful collaboration. THE AUTHORS A. S. Iljinov, Ph.D., is a head of the radioisotope laboratory at the Institute for Nuclear Research of the Academy of Sciences of Russia. He has been associated with the institute since 1974. This site is the Moscow meson facility. Prior to 1970 he was associated with the Joint Institute for Nuclear Research, Dubna. He received his first doctoral degree in physics in 1971 while working at the Laboratory of Theoretical Physics of the Joint Institute for Nuclear Research, Dubna. He received his second doctoral degree in 1985 while at the Institute for Nuclear Research. His current interests focus on the theory of nuclear reaction. Together with his colleagues he has formulated the optical-cascade model of nuclear absorption of stopped pions and antiprotons and has also developed the statistical model of multi- fragmentation of nuclei by intermediate energy particles. He has also participated in the discovery and study of the cold fusion of two nuclei which has been used in the synthesis of chemical elements 106 through 109. In 1984 he proposed the use of the Moscow meson facilty for production of high intensity radioactive nuclear beams. Dr. Iljinov is the author or co-author of 140 scientific articles. He is co-author, along with Professor G. N. Flerov, of On the Way to Super-Elements (Pedagogics Publishers, Moscow, 1982) which has been translated into several languages, and of the handbook of Production ofR adionuclides ofI ntermediate Energies (Landolt- Bornstein, Vol. 13, Springer-Verlag, Berlin, 1991). M. V. Kazarnovsky, Ph.D., is the head of one of the theoretical laboratories of the Institute for Nuclear Research of the Russian Academy of Sciences and has been associated with the institute since 1970. He is also a Professor at the Moscow Physical-Technical Institute, where he is a lecturer in nuclear physics. Prior to 1970 he was associated with the Lebedev Physical Institute of the Academy of Sciences of the U.S.S.R. He received his first doctoral degree in 1955, a second doctoral degree in 1971, and the title of professor in 1987. Dr. Kazarnovsky is the author or co-author of more than 120 scientific works and two monographs, primarily on the following topics: the theory of non-stationary neutron transport, the theory of nuclear reactions at intermediate energies, and the physics of ultracold nuetrons. E. Ya. Paryev, Ph.D., is a senior scientist at the Institute for Nuclear Research of the Academy of Sciences of Russia and has been associated with the institute since 1974. He received his doctoral degree in 1985; the subject of his thesis was the application of the kinetic equations method in theory of nucleon-nucleus re- actions at intermediate energies. Together with Professor M. V. Kazarnovsky, he has developed, on the basis of these equations, the new analytic approach for the description of inclusive in- termediate-energy nucleon-nucleus reactions, which take into account the spin de- pendence of the NN-interaction and quantum-mechanical effects at the initial state of this reaction as well. He has also worked out various problems in the field of applied nuclear physics: transport of neutrons, charged particles in solids, and radiation protection of high- current accelerators. His current focus of interest is on the theory of production of various mesons (K"', 11, w) in the nucleon-nucleon and nucleon-nucleus collisions at different energies. Dr. Paryev has published 40 scientific papers and has presented reports at a variety of international conferences. TABLE OF CONTENTS INTRODUCTION ............................................................... 1 I. Notation . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 1 II. Classification of Cross-Sections of NRs ................................. 2 III. Quantum Formulation of Collision Problem ............................. 5 A. Reaction Channels ................................................ 5 B. Transition Probabilities and S-Matrix ............................. 6 C. S-Matrix and Cross-Sections-Scattering Amplitude ............. 8 D. Quantum-Mechanical Models of NRs ........................... 10 IV. Statistical Description of Dynamical Many-Particle Systems ............ 14 A. Phase Density and Liouville Equation ........................... 14 B. Density Matrix-Quantum Liouville-von Neumann Equation ......................................................... 16 C. Wigner Probability Function ..................................... 18 References. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 1. 9. . . . . . . . . . . . . Chapter 1 INTRANUCLEAR CASCADE MODEL ....................................... 21 I. Formulation of the Problem and Basic Assumptions .................... 21 A. Prolegomena .................................................... 21 B. Basic Assumptions of the INC-Model ........................... 22 II. Exclusive Description of the INC ....................................... 23 A. Phase Density and Hamiltonian of the INC-Model .............. 23 B. A Streaming and a Collision Term .............................. 24 C. Incorporation of the Pauli Exclusion Principle in the Collision Term .................................................. 27 D. Formulation of the Equation, the Initial, and the Boundary Conditions ............................................ 28 E. Integral Forms of the Liouville Equation ........................ 29 F. Solution of the Integral Liouville Equation in the Form of the von Neumann Series ...................................... 32 G. "Macroapproximation" ......................................... 33 III. Inclusive Description of the INC ........................................ 35 A. Bo1tzmann-Ueh1ing-Uhlenbeck Equation ........................ 35 B. Linearization of the BUD-Equation .............................. 37 IV. Characteristics of NRs .................................................. 39 A. Preliminary Remarks ............................................ 39 B. Total Cross-Section of Inelastic Interaction ...................... 41 C. Topological and Exclusive Cross-Sections ....................... 42 D. Inclusive Cross-Sections ......................................... 43 E. Distribution of Nuclei Produced in the Cascade Over the Number of Neutrons and Protons, Excitation Energy, Momentum, and Angular Momentum .................. 43 V. Taking Account of Quantum Effects in the INC-Model. ................ 44 A. Density Matrix-Quantum Liouville-von Neumann Equation ......................................................... 44 B. Transformation of the Liouville-von Neumann Equation to the Form Close to the Classical One ................ 45 C. Validity Conditions of the INC-Model .......................... 48 VI. Conclusions ............................................................. 51 References ...................................................................... 53 Chapter 2 METHODS FOR SOLUTION OF THE SYSTEM OF KINETIC EQUATIONS OF THE INTRANUCLEAR CASCADE MODEL .............. 55 I. Analytic Methods of Solution ........................................... 55 A. Cross-Section of Inelastic Interaction and Quasifree Nucleons ........................................................ 55 B. Quantum-Mechanical Calculation of a Quasifree Component of the Inclusive Cross-Section ...................... 60 C. Solution of the System of KEs for Cascade Nucleons in the Small-Angle Approximation-the Domain of Relatively High Energies of Secondary Nucleons ............... 64 D. Solution of the System of KEs for Cascade Nucleons in the P -Approximation-the Domain of Low 1 Energies of Secondary Nucleons ................................ 70 E. Nucleonic Cascade at Low Energies ............................. 75 1. Cross-Section for Production of Quasifree and Cascade Nucleons at Low Energies ...................... 75 2. Pre-Equilibrium Models of NRs at Low Energies ................................................. 80 IT. Solution of the System of KEs of the INC-Model by Means of the Monte Carlo Technique .......................................... 83 A. Standard Monte Carlo INC-Model. .............................. 84 1. General Scheme of the Monte Carlo Simulation of INCs .................................................. 84 2. Model of a Target Nucleus .............................. 86 3. Characteristics of an Incident Particle Inside a T-Nucleus ................................................ 87 4. Search of a Partner and an Interaction Point ............. 88 5. Calculation of an Elementary Interaction ................. 88 6. Cut-Off Energy .......................................... 91 7. Characteristics of an R-Nucleus .......................... 92 B. Trawling Effect in the INC ...................................... 93 Ill. Conclusions ............................................................. 95 References ...................................................................... 96 Chapter 3 DECAY AND PROPERTIES OF HIGHLY EXCITED NUCLEI ............... 99 I. Decay of a C-Nucleus with Zero Angular Momentum .................. 99 A. Basic Tenets of Statistical Model of Decay of a C-Nucleus ....................................................... 99 B. Level Density of Highly Excited Nuclei. ....................... 101 C. Effect of a High Excitation of a Nucleus on its Structure ........................................................ 106 1. Disappearance of Shell Effects at High Values of the Excitation Energy ................................ 106 2. Changes in Macroscopic Properties of a Nucleus Caused by an Increase in its Excitation Energy .................................................. 111 II. Decay of a C-Nucleus with High Angular Momentum ................. 115 A. Basic Relations of Semiclassical Model ........................ 115 B. The Effect of a High Value of the Angular Momentum on the Properties of a Nucleus ................................. 117 III. General Pattern of Decay of a Highly Excited Nucleus and Methods Used in Calculation of the Evaporation Cascade ............. 118 IV. Analysis of Data Concerned with the Properties and Decay of Excited C-Nuclei. ...................................................... 122 A. Statistical Properties of C-Nuclei Produced in Reactions with Low-Energy Particles ........................... 122 B. Decay of C-Nuclei Produced in Heavy-Ion-Induced Reactions ....................................................... 128 V. Explosive Decay of Hot Nuclei ........................................ 130 A. Fermi Breakup of Light Nuclei ................................. 132