FUEL BEHAVIOUR AND MODELLING UNDER SEVERE TRANSIENT AND LOSS OF COOLANT ACCIDENT (LOCA) CONDITIONS The following States are Members of the International Atomic Energy Agency: AFGHANISTAN GUATEMALA PANAMA ALBANIA HAITI PAPUA NEW GUINEA ALGERIA HOLY SEE PARAGUAY ANGOLA HONDURAS PERU ARGENTINA HUNGARY PHILIPPINES ARMENIA ICELAND POLAND AUSTRALIA INDIA PORTUGAL AUSTRIA INDONESIA QATAR AZERBAIJAN IRAN, ISLAMIC REPUBLIC OF BAHRAIN IRAQ REPUBLIC OF MOLDOVA BANGLADESH IRELAND ROMANIA BELARUS ISRAEL RUSSIAN FEDERATION BELGIUM ITALY RWANDA BELIZE JAMAICA SAUDI ARABIA BENIN JAPAN SENEGAL BOLIVIA JORDAN SERBIA BOSNIA AND HERZEGOVINA KAZAKHSTAN SEYCHELLES BOTSWANA KENYA SIERRA LEONE BRAZIL KOREA, REPUBLIC OF SINGAPORE BULGARIA KUWAIT BURKINA FASO KYRGYZSTAN SLOVAKIA BURUNDI LAO PEOPLE’S DEMOCRATIC SLOVENIA CAMBODIA REPUBLIC SOUTH AFRICA CAMEROON LATVIA SPAIN CANADA LEBANON SRI LANKA CENTRAL AFRICAN LESOTHO SUDAN REPUBLIC LIBERIA SWAZILAND CHAD LIBYA SWEDEN CHILE LIECHTENSTEIN SWITZERLAND CHINA LITHUANIA SYRIAN ARAB REPUBLIC COLOMBIA LUXEMBOURG CONGO MADAGASCAR TAJIKISTAN COSTA RICA MALAWI THAILAND CÔTE D’IVOIRE MALAYSIA THE FORMER YUGOSLAV CROATIA MALI REPUBLIC OF MACEDONIA CUBA MALTA TOGO CYPRUS MARSHALL ISLANDS TRINIDAD AND TOBAGO CZECH REPUBLIC MAURITANIA TUNISIA DEMOCRATIC REPUBLIC MAURITIUS TURKEY OF THE CONGO MEXICO UGANDA DENMARK MONACO UKRAINE DOMINICA MONGOLIA DOMINICAN REPUBLIC MONTENEGRO UNITED ARAB EMIRATES ECUADOR MOROCCO UNITED KINGDOM OF EGYPT MOZAMBIQUE GREAT BRITAIN AND EL SALVADOR MYANMAR NORTHERN IRELAND ERITREA NAMIBIA UNITED REPUBLIC ESTONIA NEPAL OF TANZANIA ETHIOPIA NETHERLANDS UNITED STATES OF AMERICA FIJI NEW ZEALAND URUGUAY FINLAND NICARAGUA UZBEKISTAN FRANCE NIGER VENEZUELA GABON NIGERIA VIETNAM GEORGIA NORWAY GERMANY OMAN YEMEN GHANA PAKISTAN ZAMBIA GREECE PALAU ZIMBABWE The Agency’s Statute was approved on 23 October 1956 by the Conference on the Statute of the IAEA held at United Nations Headquarters, New York; it entered into force on 29 July 1957. The Headquarters of the Agency are situated in Vienna. Its principal objective is “to accelerate and enlarge the contribution of atomic energy to peace, health and prosperity throughout the world’’. IAEA-tEcdoc-cd-1709 FUEL BEHAVIoUR ANd ModELLING UNdER SEVERE tRANSIENt ANd LoSS oF cooLANt AccIdENt (LocA) coNdItIoNS PRocEEdINGS oF A tEcHNIcAL MEEtING HELd IN MIto, jAPAN, 18–21 octoBER 2011 INtERNAtIoNAL AtoMIc ENERGy AGENcy VIENNA, 2013 COPYRIGHT NOTICE All IAEA scientific and technical publications are protected by the terms of the Universal Copyright Convention as adopted in 1952 (Berne) and as revised in 1972 (Paris). The copyright has since been extended by the World Intellectual Property Organization (Geneva) to include electronic and virtual intellectual property. Permission to use whole or parts of texts contained in IAEA publications in printed or electronic form must be obtained and is usually subject to royalty agreements. Proposals for non-commercial reproductions and translations are welcomed and considered on a case-by-case basis. Enquiries should be addressed to the IAEA Publishing Section at: Marketing and Sales Unit, Publishing Section International Atomic Energy Agency Vienna International Centre PO Box 100 1400 Vienna, Austria fax: +43 1 2600 29302 tel.: +43 1 2600 22417 email: [email protected] http://www.iaea.org/books For further information on this publication, please contact: Nuclear Fuel Cycle and Materials Section International Atomic Energy Agency Vienna International Centre PO Box 100 1400 Vienna, Austria Email: [email protected] © IAEA, 2013 Printed by the IAEA in Austria JUNE 2013 IAEA Library Cataloguing in Publication Data Fuel behaviour and modelling under severe transient and loss of coolant accident (LOCA) conditions : proceedings of a technical meeting held in Mito, Japan, 18-21 October 2011. – Vienna : International Atomic Energy Agency, 2013. CD-ROM. – (IAEA-TECDOC-CD series, ISSN 1684-2073 ; no. 1709) ISBN 978-92-0-192410-0 Includes bibliographical references. 1. Nuclear reactors – Research – Congresses. 2. Nuclear fuel elements – Mathematical models. 3. Nuclear fuels – Safety measures – Congresses. I. International Atomic Energy Agency. II. Series. IAEAL 13-00812 foreword In recent years the demands on ‘fuel duties’ have increased, including transient regimes, higher burnups and longer fuel cycles. To satisfy these demands, fuel vendors have developed and introduced new cladding and fuel material designs to provide sufficient margins for safe operation of the fuel components. National and international experimental programmes have been launched, and models have been developed or adapted to take into account the changed conditions. These developments enable water cooled reactors, which contribute about 95% of the nuclear power in the world today, to operate safely under all operating conditions; moreover, even under severe transient or accident conditions, such as reactivity initiated accidents (RIAs) or loss of coolant accidents (LOCAs), the behaviour of the fuel can be adequately predicted and the consequences of such events can be safely contained. In 2010 the IAEA Technical Working Group on Fuel Performance and Technology (TWGFPT) recommended that a technical meeting on “Fuel Behaviour and Modelling under Severe Transient and LOCA Conditions” be held in Japan. The accident at the Fukushima Daiichi nuclear power plant in March 2011 highlighted the need to address this subject, and despite the difficult situation in Japan at the time, the recommended plan was confirmed, and the Japan Atomic Energy Agency (JAEA) hosted the technical meeting in Mito, Ibaraki Prefecture, Japan, from 18 to 21 October 2011. This meeting was the eighth in a series of IAEA meetings, which reflects Member States’ continuing interest in the above issues. The previous meetings were held in 1980 (jointly with OECD Nuclear Energy Agency, Helsinki, Finland), 1983 (Risø, Denmark), 1986 (Vienna, Austria), 1988 (Preston, United Kingdom), 1992 (Pembroke, Canada), 1995 (Dimitrovgrad, Russian Federation) and 2001 (Halden, Norway). The purpose of the technical meeting was to provide a forum for international experts to review the current For further information on this publication, please contact: situation and the state of the art of the performance of nuclear fuel for water cooled reactors under severe transients and LOCA conditions. The meeting was attended by 83 specialists representing fuel vendors, nuclear utilities, Nuclear Fuel Cycle and Materials Section research and development institutions, and regulatory authorities from 19 Member States. The papers submitted to International Atomic Energy Agency the meeting were organized into seven sessions covering analytical and experimental RIA and LOCA studies and Vienna International Centre international programmes, power ramp, and severe accident analysis. These proceedings contain all the papers that PO Box 100 were presented and discussed during the meeting, and highlight key findings and recommendations based on the 1400 Vienna, Austria summaries of the session chairpersons. While the Fukushima Daiichi accident influenced the discussions, it was Email: [email protected] not directly considered because of the lack of fuel behaviour data available at the time of the technical meeting. The IAEA wishes to thank the hosts and all participants for their contributions to the technical meeting, in particular © IAEA, 2013 K. Kamimura (JNES) and F. Nagase (JAEA). The IAEA officer responsible for this publication was V. Inozemtsev Printed by the IAEA in Austria of the Division of Nuclear Fuel Cycle and Waste Technology. MAY 2013 EDITORIAL NOTE This CD-ROM has been prepared from the original material as submitted by contributors. Neither the IAEA nor its Member States assume any responsibility for the information contained on this CD ROM. This publication (including the figures, tables and references) has undergone only the minimum copy editing considered necessary for the reader’s assistance. The use of particular designations of countries or territories does not imply any judgement by the publisher, the IAEA, as to the legal status of such countries or territories, of their authorities and institutions or of the delimitation of their boundaries. The mention of names of specific companies or products (whether or not indicated as registered) does not imply any intention to infringe proprietary rights, nor should it be construed as an endorsement or recommendation on the part of the IAEA. The authors are responsible for having obtained the necessary permission for the IAEA to reproduce, translate or use material from sources already protected by copyrights. . CONTENTS SUMMARY ............................................................................................................................... 1 R&D PROGRAMME ON FUEL BEHAVIOUR UNDER TRANSIENTS (Session 1) Fuel safety research at JAEA ................................................................................................................ 17 F. Nagase IRSN R&D studies on fuel behaviour under RIA conditions ............................................................... 25 M. Petit, O. Marchand, F. Barré, P. Giordano EXPERIMENTAL RIA STUDIES (Session 2) Status of RIA related fuel safety research at JAEA .............................................................................. 45 T. Sugiyama, H. Sasajima, M. Amaya, F. Nagase New techniques for the testing of cladding material under RIA conditions.......................................... 55 H.K. Yueh, R.J. Comstock, V. Grigoriev, J. Karlsson, W. Lees, Y.P. Lin, D. Lutz, D. Mitchell, D. Schrire Current status of RIA study in the Republic of Korea .......................................................................... 67 S.-K. Kim, J.-G. Bang, D.-H. Kim, Y.-S. Yang, Y.-H. Koo The cladding fracture behaviour under biaxial stress conditions .......................................................... 77 T. Fukuda, T. Mihara, M. Amaya, T. Sugiyama, F. Nagase Fracture behaviour of hydrided cladding tubes with radial incipient crack in periphery ...................... 85 T. Mihara, T. Fukuda, Y. Udagawa, T. Sugiyama, F. Nagase ANALYTICAL RIA STUDIES (Session 3) Recent RIA and LOCA analyses performed at Technical Research Centre Finland (VTT) using fuel performance codes SCANAIR and FRAPTRAN-GENFLO ............................................ 97 A. Arffman Assessment of steady state uncertainties impact on RIA modelling ................................................... 117 A. Huguet, L.E. Herranz RCCA ejection fault studies: Application of a burnup threshold for the evaluation of the radiological releases ........................................................................................................................ 131 C. Bernaudat, J. Guion, N. Waeckela Present status of the verifications and model development of FEMAXI and RANNS codes in JAEA ................................................................................................................................. 141 M. Suzuki, Y. Udagawa, T. Sugiyama, F. Nagase RCCA ejection fault studies: Application of a burnup threshold for the evaluation of the radiological releases ........................................................................................................................ 153 Y. Udagawa, T. Sugiyama, M. Suzuki, F. Nagase LOCA R&D (Session 4) LOCA: An operator’s view on German licensing practice ................................................................. 163 A. Wensauer IRSN R&D studies on fuel behaviour under LOCA conditions ......................................................... 179 M. Petit, C. Grandjean, N. Trégourès, F. Barré, P. Giordano Investigation of the RU-43LV fuel behaviour under LOCA conditions in CANDU reactor .............. 191 G. Horhoianu EXPERIMENTAL LOCA STUDIES (Session 5) High burnup fuel behaviour under LOCA conditions as observed in Halden reactor experiments ..................................................................................................................................... 207 E. Kolstad, W. Wiesenack, B. Oberländer, T. Tverberg Results of integral, high burnup, fuelled LOCA tests and companion testing with as-fabricated and pre-hydrided cladding ......................................................................................... 219 P. Askeljung, M. Billone, M. Flanagan Behaviour of high burnup fuel during LOCA; key observations and test plan at JAEA .................... 229 F. Nagase, T. Chuto UJP LOCA oxidation criteria “K” and “O ” ....................................................................................... 241 Β M. Négyesi, L. Novotný, J. Kabátová, S. Linhart, V. Klouček, J. Lorinčík, V. Vrtílkováb Quantification of the chemical elements partitioning within pre-hydrided Zircaloy-4 after high temperature steam oxidation as a function of the final cooling scenario (LOCA conditions) and consequences on the (local) materials hardening ..................................... 253 J.C. Brachet, D. Hamon, J.L. Béchade, P. Forget, C. Toffolon-Masclet, C. Raepsaet, J.P. Mardon, B. Sebbari ANALYTICAL LOCA STUDIES (Session 6) Evaluation and analysis of high burnup fuel behaviour under LOCA conditions ............................... 269 Y. Yun, M.A. Zimmermann The RAPTA-5.2: Code for modelling of VVER type fuel rod behavior under design basis accidents conditions ............................................................................................................... 279 P.V. Fedotov, A.A. Goncharov, A.V. Kumachev, O.A. Nechaeva, V.V. Novikov, A.V. Salatov, Y.V. Pimenov, Y.N. Dolgov Assessment of fuel behaviour under large break LOCA condition for Indian pressurized heavy water reactor ......................................................................................................................... 289 A. Dixit, S.K. Yadav, N. Kumar, T.A. Khan, M. Singhal, N. Mohan, P.K. Malhotra, S.G. Ghadge, U. Chandra Matare coupled codes package validation and assessment of potential clad ballooning behaviour for limiting ATWS and LBLOCA fault sequences in support of development of the SIZEWELL ‘B’ PWR safety case with an increased fuel internal pressure limit and M5TM clad fuel ................................................................................................................................. 301 R. Page, S. Jenkins Radiological consequences for CHASHMA NPP Unit 2 due to large break LOCA without ECCS and CSS ................................................................................................................................ 327 S.A.A. Rizvi, M.A. Ahmed, Q. Hasnain, A. Minhaj POWER RAMP AND SEVERE ACCIDENT (Session 7) Status of power transient test program on LWR fuels using JMTR .................................................... 349 J. Ogiyanagi, S. Hanawa, F. Nagase Fission gas release from high burnup fuel during normal and power ramp conditions ...................... 357 M. Amaya, J. Nakamura, F. Nagase Investigation of VVER 1000 core degradation during SBO accident scenario in case of pressurizer SV stuck in open position ............................................................................................. 367 P. Groudev, A. Stefanova, R.Gencheva List of Abbreviations ........................................................................................................................... 379 List of Participants .............................................................................................................................. 383 SUMMARY SESSION 1: R&D PROGRAMME ON FUEL BEHAVIOUR UNDER TRANSIENTS Chairpersons: T. Fuketa (JAEA) and M. Flanagan (NRC) 1. BACKGROUND The presentations of this session highlight research activities at two of the major nuclear test reactor facilities, CABRI reactor and the Nuclear Safety Research Reactor (NSRR), operating in the world today. 2. SUMMARIES AND COMMENTS F. Nagase of the Japan Atomic Energy Agency (JAEA) in Japan presented an overview of the fuel safety research activity at the JAEA. F. Nagase explained that JAEA’s research activities span reactivity initiated accidents (RIAs), loss of coolant accidents (LOCAs), fuel behaviour code development and verification, as well as fundamental studies of specific phenomena. The JAEA studies in the Nuclear Safety Research Reactor (NSRR), simulating RIA events, have produced a fundamental understanding of pellet cladding mechanical interaction (PCMI) failure for RIA events and semi-integral quench tests have confirmed the adequacy of the Japanese LOCA regulatory limits for the high burnup of fuel. Fundamental studies on oxidation behaviour and crack propagation in hydrided cladding have been critical for evaluating and interpreting the results of both the LOCA and RIA studies. The knowledge from the transient testing and the fundamental studies has been successfully integrated into fuel behaviour codes to produce improved modelling capabilities. In the future, JAEA research programs will continue to use these demonstrated experimental approaches to study advanced cladding and fuel materials. Recently, a new emphasis has emerged on fuel and cladding response in severe accidents and beyond design basis accidents. M. Petit of the Institut de Radioprotection et de Sûreté Nucléaire (IRSN) in France presented an overview of research being conducted at IRSN to study fuel behaviour under RIA conditions. M. Petit presented that the experiments in the sodium loop of the CABRI reactor led to a fundamental understanding of the PCMI failure mode of RIA transients and the findings indicated a need to revise RIA criteria. Now, a new program will be conducted in a water loop in the CABRI reactor which will illuminate both the PCMI and departure from nucleate boiling (DNB) phase of a postulated RIA transient. A test matrix was presented for the new program with a total of 10 tests. Two tests in sodium have already been completed. Many of these planned tests are specifically designed to complement the experimental databases of the CABRI sodium loop tests and the NSRR RIA tests. 3. PROBLEMS, CHALLENGES AND PERSPECTIVES Even with these 12 planned tests, it is clear some aspects of fuel behaviour under RIA conditions will still remain largely unaddressed. Despite many years of research and operating experience of light water reactors, research questions still remain in order to characterize the fuel and cladding behaviour in response to accident conditions in a detailed way. At the same time, there are fewer and fewer facilities capable of simulating RIA, LOCA and transient conditions. Combining test reactor studies with fundamental studies further increases the contribution of test reactor findings to the understanding of fuel and cladding response to 1 transient conditions. With many countries facing decreased financial resources, international collaboration is becoming increasingly necessary to run large scale test programs and fundamental understanding of the complex phenomena of nuclear fuel and cladding is necessary to direct the limited resources to generate the maximum benefit. The JAEA and IRSN research programs provide critical coordination of large scale test programs and fundamental research which has resolved, and will continue to resolve critical questions for safe operation of nuclear power plants. 4. RECOMMENDATIONS FOR FUTURE WORK An extension in the test program is therefore proposed to address aspects such as the performance of fuel as intermediate burnups, where large uncertainty and disagreement between expert interpretation remains. 1. Encouragement of partnerships and synthesis of research program findings from various international programs. 2. Combining test reactor studies with fundamental studies further increases the contribution of test reactor findings to the understanding of fuel and cladding response to transient conditions and should be supported. SESSION 2: EXPERIMENTAL RIA STUDIES Chairpersons: M. Petit (IRSN) and T. Sugiyama (JAEA) 1. BACKGROUND The behaviour of nuclear reactor fuels during off-normal and postulated accident conditions such as RIA are a matter of investigations. In order to define adequate criteria for fuel design effects and for burnup related effects, the fuel response to RIA transients is being studied experimentally and analytically. Considerable experimental evidence has been gathered in recent years covering a variety of materials and conditions. 2. SUMMARIES AND COMMENTS In the session 2, entitled “Experimental RIA Studies”, 5 papers were presented. The first paper by T. Sugiyama, JAEA, Japan, showed an overview of the 14 RIA experiments performed in the NSRR reactor during the Advanced LWR Fuel Performance and Safety (ALPS) programme on high burnup light water reactor (LWR) fuel. Both low and high initial temperature tests were conducted. The paper discussed the outcome of the experiments in terms of PCMI failure criterion. Also addressed was the influence of the initial temperature on PCMI failure. In conclusion the fuels to be tested in the phase 2 of ALPS (that were received in January 2011) were presented. The second paper by K. Yueh, Electric Power Research Institute (EPRI), United States of America (USA), discussed the results of 2 new mechanical tests performed by Studsvik, Sweden on behalf of EPRI. The first type of tests on Zr-2 with radial hydrides — called rapid heating and load test — showed that even brief exposure at high temperature enhances the ductility of the hydrided cladding samples. There appears to be an abrupt recovery between 70–100°C, comparable to a brittle to ductile transition, followed by a more gradual ductility improvement when temperature increases. The second type of test, called modified burst test, consists of a loading of a cladding sample by the use of a tube 2
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