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Frequency-dependent Study of Solid Helium-4 Contained in a Rigid Double-torus Torsional Oscillator PDF

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Preview Frequency-dependent Study of Solid Helium-4 Contained in a Rigid Double-torus Torsional Oscillator

Frequency-dependent Study of Solid Helium-4 Contained in a Rigid Double-torus Torsional Oscillator Jaewon Choi,∗ Jaeho Shin, and Eunseong Kim† Department of Physics and Center for Supersolid and Quantum Matter Research, Korea Advanced Institute of Science and Technology (KAIST), 291 Daehak-ro, Yuseong-gu, Daejeon 34141, Republic of Korea (Dated: January 27, 2017) The rigid double-torus torsional oscillator (TO) is constructed to reduce any elastic effects in- 7 herent to complicate TO structures, allowing explicit probing for a genuine supersolid signature. 1 We investigated the frequency- and temperature-dependent response of the rigid double-torus TO 0 containing solid 4He with 0.6 ppb 3He and 300 ppb 3He. We did not find evidence to support the 2 frequency-independentcontributionproposedtobeapropertyofsupersolidhelium. Thefrequency- dependentcontribution which comesfrom thesimpleelastic effect ofsolid helium coupled toTO is n essentiallyresponsiblefortheentireresponse. Themagnitudeoftheperioddropislinearly propor- a J tional to f2, indicating that theresponses observed in this TO are mostly caused bythe overshoot of ‘soft’ solid helium against thewall of thetorus. Dissipation of therigid TO is vastly suppressed 6 compared to those of non-rigid TOs. 2 ] r I. INTRODUCTION frequency-independentresonantperiodchangeaftersub- e tracting the frequency-dependentterm andascribedthis h t to a possible supersolid signature. This interpretation o The resonant period of an ideal torsional oscillator can be questioned since the measurements reported rel- . (TO) is proportional to the square root of its rotational t atively large period drop which can be associated with a inertia √I, and the superfluid decoupling can be de- the non-rigidity of TO. m tected by the reduction of the resonant period. The For this article, we measured the period drop and ac- d- resonant period drop of a TO containing solid helium companieddissipationpeakusingadouble-frequencyTO n was originally interpreted as the appearance of a super- thatwasconstructedtobehighlyrigidtominimizeshear o solid phase1–17. Recently, a number of experimental and modulus effects. The frequency dependence of the rigid c theoretical efforts have indicated that the anomaly in double-frequency TO was investigated in various modes [ the TO response can be explained by the shear modulus of representation. As a result, we elucidate whether or 1 change18–27. The previous finite element method (FEM) not solid helium-4 exhibits true supersolidity. v simulation suggested that the influence on the period of 1 TO due to the change in shear modulus of solid helium 2 was negligible28–30. Nevertheless, the effect can be sig- II. EXPERIMENTAL DETAILS 6 nificantly amplified resulting from non-ideal TO design. 7 Four mechanisms of non-ideal TO response have been 0 KAIST rigid double-torus torsional oscillator (TO) suggested30–33. In order to minimize the contribution of . (Fig. 1) was carefully designed to minimize the various 1 the elastic effect to the resonant period of TO, it should 0 elastic effects caused by: (1) shear-modulus-dependent be meticulously constructed to be rigid. However, most 7 relative motion between TO parts (the glue effect)30,33, of TOsused in the previoussupersolidexperiments were 1 (2) solid helium contained in the torsional rod (the tor- not rigid.30–32. Recently, the Chan group reported that : sion rod hole effect)31, and (3) solid helium layer grown v theresonantperioddropwassubstantiallyreducedwhen Xi therigidityofTOwassystematicallyincreased34–36. The on a thin TO base plate (Maris effect)32. We first assembled every joint in the TO using resonantperioddropofahighlyrigidTOwasonlyafew r stainless-steel screws or hard-soldering to diminish elas- a timesgreaterthanthatduetotheelasticeffectestimated tic effects on the TO period due to the relative motion by FEM simulation. They set the upper bound for the between different parts. The torsion plate and the tor- non-classical rotational inertia (NCRI) to be less than sionrodwererigidly connectedby machiningthe assem- approximately 4 ppm36. bly from a single piece of Be-Cu. The torus-shaped TO However, new evidence of a ‘true’ supersolid signa- cell for solid helium was constructed by hard-soldering ture wassuggestedby Reppyet al.37,38 basedondouble- twopiecesofsemi-circularcopper tubing. The toruswas frequency TO experiments. Superfluidity or the NCRI hard-soldered onto thick copper plate and the combined is independent of frequency while non-superfluidity or structures were fastened down directly on the torsion therelaxationphenomenonresultingfromshearmodulus plate by four screws. change leads to a strong frequency dependence. Accord- Second, we used a thick torsion rod and a very thin ingly, analysis on the frequency dependence can be used fill line to preventthe elastic effect of solidhelium in the to differentiate the superfluid response from the non- fill line. The change of shear modulus of solid helium-4 superfluid response30,38. Reppy et al. observed a small contained in the torsion rod can induce the TO period 2 operated at four resonant frequencies. This is possible due to the configurationofourTO whichconsists oftwo torus-shaped solid helium containers attached to upper and lower stages. This configuration enables modifica- tion of the resonant frequency by loading solid helium into the upper or both tori. We first placed the solid sample in both tori. After collecting the first dataset, the solid helium inside the lower torus was carefully re- moved at low temperature to avoid damaging the solid sample placed in the upper torus. Finite element method (FEM) simulations indicates thata30%changeintheshearmodulusofsolidhelium-4 in the upper torus leads to only a 0.93-ns period drop in FIG. 1. KAISTrigid double-torustorsional oscillator. first(1st)mode (in-phase)anda 1.16-nsdropinthe sec- ond (2nd) mode (out-of-phase). These simulations cor- respond to 2.3 10−5 and 1.9 10−4 respectively in the × × anomaly31. This effect may be responsible for the pe- framework of so-called NCRI fraction. The major con- riod drop observed in the majority of TO experiments. tribution seemingly comes from the overshooteffect, the In order to remove this effect, a 1-mm-diatmeter CuNi relative motion of solid helium with respect to the outer filling capillary was directly installed on top of the TO wall. cell instead of making a hole through a torsion rod. The empty cell has resonant frequencies of 449.57 Hz Third, the TO cell containing solid helium was hard- and 1139.77 Hz for in-phase and out-of-phase modes re- soldered to a 3-mm-thick copper plate and was designed spectively. Two pairs of electrodes attached to the lower sothatsolidheliuminthetorusdidnothaveadirectcon- torus were used to drive and detect the TO response. tactto the baseplate nearthe torsionrod. In acylindri- The additional electrodes installed on the upper plate calTO,solidheliumwasgrowndirectlyonitsbaseplate. enables the detection of the amplitude and phase of the If the thickness of the base plate is not sufficiently thick, upper torus. We confirmed that the phase difference be- then the period drop due to the change in shear modu- tween the two tori was approximately 0 degrees for the lus of solid helium can be significantly amplified32. The in-phase mode and 180 degrees for out-of-phase mode. contribution of solid helium is greater in the proximity Themechanicalqualityfactorwasapproximately1 106 × of the torsionrod andwhen the base plate is thinner. In at 4.2 K for both modes. this study, solid helium confined in a rigid torus channel Bulk solid helium-4 samples containing an impurity onthethickcopperplatewasnotexpectedtoexhibitthe concentration of 0.6 ppb and 300 ppb helium-3 were strong Maris effect. grownby the blocked capillary method. The sample cell was first pressurized to target pressures of 67-82 bar at Finally, we carefully tuned the so-called ‘overshootef- 3.2 K and the mixing chamber was then cooled to the fect’ caused by direct coupling of elastic properties of base temperature. The resonant period shifted accord- solid helium to the TO response. Since solid helium is ing to solid growth in the upper torus: 39,800 ns for the much softer than the wall of the container, it undergoes in-phase mode and 6,040 ns for the out-of-phase mode. additional displacement. The shear modulus change of The large period shift due to solid helium and its solid solidheliumnotmovingin phasewith the confining wall stability in the first mode enables us to distinguish the can induce the period anomaly without non-linear am- change of the resonant period within about 2 ppm reso- plification. The resonant period drop introduced by the lution. This sensitivity is lower than the upper limit of overshoot effect is known to be linearly proportional to NCRI fraction reported by the PSU group (4 ppm)36. the square of the TO frequency. For this experiment, we optimized the overshooteffect so that the system was in a regime where the elastic effect is not too small to be detected and not too big to make the TO softer. In this III. TO PERIOD AND DISSIPATION TO,solid helium was locatedin a torus with a relatively large cross-section (diameter: 5 mm), which allows us The period and dissipation of the TO for both the in- to have large mass loading and high resolution for the phaseandout-of-phasemodesweremeasuredoveratem- so-called NCRI fraction. One can effectively reduce this peraturerangeof20-300mK.Figure2presentsthe reso- effect by confining solid helium in a thick copper torus nantperiodoftherigiddouble-torusTOcontaininghigh- with a small cross-section at the expense of diminishing purity solid helium-4 (0.6 ppb) and commercial-purity the capability of frequency analysis. This fine-tuning al- solid helium-4 (300 ppb) as a function of temperatures lows us to investigate the effect of the shear modulus on atdifferentrimvelocities. The perioddropanomalywas thedouble-frequencyTOandpossiblesupersoliditymore observed for both modes of the rigid double-torus TO. clearly. Compared with the empty cell data (dashed line), the In addition, the KAIST rigid double-torus TO can be perioddropin0.6-ppbsolidsampleappearsinitiallyat80 3 e ng (a) 47.2 m/s (b) 47.7 m/s (c) 52.6 m/s (d) 21.3 m/s ha1.5 87.5 m/s 87.8 m/s 131.3 m/s 52.8 m/s Period C1.0 248387801509...4881. 8 mmmm///sss/s 248196810552...342 7. 2 mmmm//ss/s/s 251154189256..0007.. 68 mmmm//ss//ss 125354240...237 mmm///sss e v0.5 ati el R 0.0 T) -1 Q( 4 x10-7 n 3 o ati 2 p si 1 s Di 0 0.02 0.04 0.06 0.080.1 0.02 0.04 0.06 0.080.1 0.0 0.1 0.2 0.3 0.0 0.1 0.2 0.3 Temperature (K) FIG. 2. Period and dissipation data of the KAIST rigid double-pendulum TO containing solid helium with 0.6-ppb 3He ((a) in-phaseand(b)out-of-phase)and300-ppb3He((c)in-phaseand(d)out-of-phase). Theempty-cellbackgroundwassubtracted in both period and dissipation data. The y-axis of upper panels represent absolute values of period changes, calculated from theempty-cell backgrounds. mK,andbecamesaturatedbelow25mKforbothmodes anonsettemperatureof160mKandreachesamaximum (colored symbols). The magnitude of the period drop is of1.49ns(dP /∆P =3.7 10−5)at40mK.Intheout- − − × suppressed by the increase in the rim velocity of the al- of-phasemode,theonsettemperatureishigherthanthat ternating current (AC) oscillation for both modes. The of the in-phase mode, about 200 mK. The shifted onset suppression of the TO anomaly appears at a rim veloc- temperature at higher frequency modes has been previ- ity of 100 µm/s for both modes. Similar behaviors have ously reported from a double-pendulum TO by Rutgers been observed in numerous previous experiments1,2,8–15, group9 and also in shear modulus measurements in an- including the measurement of the rigid TOs34–36. The other experiment21. The magnitude of the period drop lowonsettemperatureofabout80mK andsharpertem- saturatesto 1.55ns (dP /∆P =2.6 10−4) at 40mK. − − × perature dependence of the TO anomaly were reported The maximum period dropobservedfor both modes has for low helium-3 impurity concentrations18,39. The pe- a similar order of magnitude as those anticipated by the riod values measured at different rim velocities follows FEM simulation. The dissipation in TO amplitude ap- theemptycellbackgroundathightemperaturesforboth pearsoverthesametemperaturerange. Atthelowestrim resonant modes. velocity of 50 µm/s, the dissipation peak was located at The maximum period drop at the lowest rim veloc- approximately 105 mK. ity is 1.43 ns and 1.66 ns for the in-phase (-) and the We investigated seven different solid helium samples. out-of-phase (+) modes respectively, which are a similar The resonant period showed similar order of magnitude order of magnitude to those expected from the contri- drops, approximately 1.3-1.7 ns for both modes. How- bution by the shear modulus (0.93 ns for the in-phase ever, only two solid samples described above show dis- mode and 1.16 ns for the out-of-phase mode with a 30% sipation in the TO response. In addition, the size of shear modulus change). By subtracting the empty-cell these dissipation peaks is approximately 10−7 and is background,wecalculateddP withrespecttothemass orders of magnitude smaller than those from typical ± loading of solid helium ∆P , equivalent to the NCRI TO experiments. These minute dissipation features are ± fraction, dP /∆P =3.5 10−5 for the in-phase mode; consistent with the results from the Chan group who − − dP /∆P =2.5 10−4 for×the out-of-phasemode. Con- showed no clear dissipation features in their rigid TO + + sidering that the×maximum change in shear modulus at experiments35,36. The absence of and/or the significant thelowesttemperaturecanvaryfrom8%18 to86%40,the reduction of dissipations can be connected to a rigidity perioddropcanbereasonablyattributedtothestiffening of the TO. effect of the shear modulus in solid helium. Dissipation inthe TOresponseisalsoobservedforbothmodes. The dissipationpeakappearsaround30mK atwhichthe pe- IV. FREQUENCY-DEPENDENT STUDY riodofthe TOchangesmostdrastically. The dissipation peak is also suppressed by increasing the rim velocity in The frequency dependence of the TO responses is bothmodesagreeingwithpreviousmeasurements1,2,8–15. examined to clarify the origin of the marginal period We observed essentially the same results for the drop. While dP/∆P is independent of the measure- commercial-purity (300 ppb) solid helium-4 sample ex- ment frequency in the supersolid scenario, it is propor- cept for the anomaly found at higher temperatures. In tional to the square of the measurement frequency in thein-phasemode,theanomalousperioddropappearsat the shear-modulus effect scenario30. Reppy et al.37,38 4 provided a simple mathematical methods to decom- pose the period drop observed in their TO experi- 4 (a) (b) ment into both frequency-independent and frequency- 47.2m/s 47.2m/s dependent parts explicitly. The measured period drop -5 10)3 8278.15.8mm/s/s 8278.15.8mm/s/s consists of two tienrdms: (i) the frequency-independent P- (x2 487850..81mm//essxp 487850..81mm//ss tseorlimd[sdiPgn±a/t∆urPe,±a]nd(T(i,i)Vt)h,eregfraerqdueednacsy-adpeputeantdivenetsutperemr- P-/ a(dt P4-7/.2P-m)/s d1 dep [dP /∆P ] (T,V,f), attributed to the elastic over- ± ± shoot effect, where T is temperature and V is rim veloc- 0 ity. The total period drop observed in TO experiments 0.02 0.0 5 0.1 0.2 0.02 0.05 0.1 0.2 can be written as follows: Temperature (K) FIG. 3. (a) Frequency-independent dP−/∆P−ind and (b) dP± exp = dP± ind(T,V)+ dP± dep(T,V,f) frequency-dependentdP−/∆P−dep asafunctionoftempera- (cid:20)∆P (cid:21) (cid:20)∆P (cid:21) (cid:20)∆P (cid:21) ture. The same color-coded pair for each modewas obtained ± ± ± (1) usingthesamerimvelocity. Nodistinguishablevelocityeffect Since the period drop originating from the overshoot isseenindP−/∆P−ind (a),incontrastto(b)demonstrating effect is proportional to f2, the last term can be substi- aclearrim-velocitydependence. dP−/∆P− atthelowestrim velocity 47.2µm/s is shown for comparison. tuted with [dP /∆P ]dep(T,V,f) = a(T,V)f2. Then, ± ± ind both the frequency-independent term [dP /∆P ] − − andthefrequency-dependentterm[dP /∆P ]dep ofthe frequency-independent drop. The frequency-dependent − − in-phase mode are decomposed as follows: TO response can be extrapolated to values less than 4 ppm (0.16 ns) when the stiffening of solid helium is significantly suppressed, indicating that the entire TO dP− ind = f+2 dP− exp f−2 dP+ exp (2) anomalycanbe ascribedto the shearmodulus changeof (cid:20)∆P (cid:21) γ (cid:20)∆P (cid:21) − γ (cid:20)∆P (cid:21) solid helium at low temperatures. − − + Figure 4 shows the low temperature dP/∆P for four resonant modes as a function of frequency. Two solid dP− dep = 1 f+2 dP− exp+ f−2 dP+ exp triangles are measured for solid samples grown in both (cid:20)∆P (cid:21) (cid:18) − γ (cid:19)(cid:20)∆P (cid:21) γ (cid:20)∆P (cid:21) toriand the other two solid circles correspondedto sam- − − + (3) ples grown only in the upper torus. In the log-log plot where γ =f2 f2. of dP/∆P and f2, the data can be linearly fitted to To measu+re−[dP− /∆P ]ind and [dP /∆P ]dep at a the equation log(dP/∆P) = ( 9.74)+(1.003)log(f2). − − − − − certainrimvelocity,thedrivingACvoltagewascarefully Theslopeofequationisnearly1,indicatingthatdP/∆P adjusted to have the same rim velocity for the in-phase is linearly proportional to f2. Converting the log-scale and out-of-phase modes. Accordingly, the same color- axis to a linear one, the y-intercept is equivalent to coded pair of temperature scans for eachmode as shown 2.62 10−7 (-0.3 ppm) which indicates that the mea- − × inFigure3wasobtainedatthesamerimvelocity,despite sured period drop originates from the shear modulus ef- of different driving AC voltages. fect rather than supersolid mass decoupling. The temperature dependence of (a) the frequency- The frequency dependence can be analyzed by other independent and (b) the frequency-dependent term at methods. The ratio between the period shifts of the two various TO rim velocities are plotted in Figure 3. The modes δP+/δP− can distinguish the origin of TO re- datasets identified with the same color in both Figure sponse at low temperature: either supersolidity or shear 3-(a) and 3-(b) are obtained using the same rim veloc- modulus change30. The ratio for the supersolid scenario ity. However, the two figures are significantly different. (δP+/δP−)SS would follow the mass-loading (or miss- No sizable frequency-independent period drop at any ing) change which can be easily obtained by measuring rim velocity can be identified in Figure 3-(a), while the themass-loading-inducedperiodshiftsofbothmodes. In frequency-dependent period response at the rim velocity contrast, the ratio for the shear modulus effect required of47.2µm/sisnearlythesameasthetotalperioddropin an additional frequency-dependent contribution as fol- the measurements. The averagedfrequency-independent lows: period drop is approximately 0 4 ppm, which is simi- lar to the upper limit set in the±rigid TO study36. Ac- (δP /δP ) = f2/f2 (δP /δP ) (4) cordingly, the majority of the period anomaly can be + − SM + − + − SS (cid:0) (cid:1) attributed not to the appearance of supersolidity but The mass-loading ratio (δP /δP ) in our experi- + − SS to the stiffening of the shear modulus of solid helium- ment is measured to be approximately 0.152. The solid 4. Besides, the frequency-dependent term was strongly straight line shown in Figure 5 indicates mass decou- suppressed with increasing TO rim velocity. In con- plingorthe supersolidscenarioestimatedbyFEMsimu- trast,noapparentdrivedependencewasobservedforthe lation and experimental measurements. The effect from 5 3 2.5 SS scenario loaded on both tori 1.5 SM scenario (analytic) 2 loaded on the upper torus SM scenario (FEM) linear fit (slope=1.00325) experiment (0.6ppb) )1.5 -4 x10 ns)1.0 experiment (300ppb) P ( 1 + ( P P/ d 0.5 0.5 0.0 105 2 3 4 5 6 8 106 2 0.0 0.5 1.0 1.5 2 2 Frequency (Hz ) P- (ns) FIG. 4. Log-Log plot of dP/∆P measured in four differ- FIG.5. Plotoftheratiooftheperiodshiftsmeasuredinboth ent frequencies as a function of the TO frequency squared modes. Thedotted line, thesupersolid mass decoupling(SS) for 0.6-ppb 3He (solid triangle) and 300-ppb 3He (solid cir- scenario, is directly calculated by the ratio of mass-loading cles). TheredsolidtrianglesrepresentdP/∆P measuredwith in both modes. Both solid and dashed lines indicate the bothtorifilledwiththesolidheliumsample,whiletheorange shear modulus (SM) scenario estimated by using finite ele- solidcirclesrepresentdP/∆P measuredwithonlyuppertorus ment method (FEM) simulation and an analytical solution, filled. Thegreydashedlineindicatesthelinearlyfittedresult. respectively. The experimental results of solid helium with The y-intercept can be converted to frequency-independent 0.6-ppb 3He (solid triangles) and 300-ppb 3He (solid circles) dP/∆P of -0.3ppm. are consistent with theSM scenario. the shear modulus change of solid helium is estimated analytically (the dashed line) and with FEM simulation [dP /∆P ]ind =1.86 10−3. Theperioddropanddissi- − − (the solidline). The slope of δP+/δP− plot in the shear pation were analyzed b×y the complex response function. modulus scenario is steeper than that in the supersolid The TO response they observed was not in agreement mass-loading scenario due to the additional frequency- with the functional formof simple glassydynamics. The dependentcontribution. The measuredδP /δP values + − authorsconcludedthatadifferentphysicalmechanismis for both 0.6 ppb and 300 ppb solid helium-4 (Figure 5) required for explaining the TO responses. indicate that the ratio δP /δP collapses to the shear + − modulus scenario. The ratios obtained in the previous TheCornellgroupalsodesignedacompoundTOwith studies lie between shear modulus expectations and su- anannularsamplespaceandmeasuredtheTOresponses. persolid expectations, suggesting the possible existence After removing the overshoot effect by frequency anal- of a putative supersolid9,37,38,41. However, we confirmed ysis, they extracted a finite frequency-independent pe- that the TO responses from the KAIST rigid double- riod drop [dP /∆P ]ind = 1 10−4, several orders of − − torusTO originatedfromthe non-supersolidorigin. The × magnitudelargerthanthe elasticcontributionestimated discrepancywithpreviousdouble-frequencyTOobserva- by their FEM simulation. Additional dissipation intro- tions may arise from the rigidity of TO. duced by solid helium was measured to be very small. The height of the dissipation peak was reported to only 5 10−8inbothresonantmodes. Theyproposedthatthe V. DISCUSSIONS × finite frequency-independent period drop could possible be new evidence for supersolidity in bulk solid helium. Recently, Both the Cornell37,38 and London41 groups constructedadouble-frequencyTOtoinvestigatethefre- In our rigid TO, the frequency-independent period quency dependence of the period anomaly. The London dropistwoorthreeordersofmagnitudesmallerthanthe groupmeasuredtheperiodanddissipationofatwo-mode value reportedfrom the Cornelland London group. The TO containing a poly-crystalline solid helium-4 sample. dissipationpeak is notobservedinmostsolidsamplesor They observed a period drop and concomitant dissipa- the size of the dissipationpeak was verysmall ( 10−7). tionfeatures,equivalenttodP /∆P =2.10 10−3and We believe that this discrepancy is presumably∼due to − − dP /∆P =8.04 10−3. Thetorsionrodhole×effectand TOrigidity. IfthetrueNCRI fractionisabout100ppm, + + × Maris effect was removed by analytical calculations. Af- thentheperioddropanomalyshouldhavebeenobserved ter fitting a linear equation to those data in f2-domain, in highly rigid TO experiments at PSU and in our rigid they found a sizable frequency-independent period drop double TO experiments. 6 VI. CONCLUSION be smaller than 4 ppm. WestudiedthefrequencydependenceofTOresponses ACKNOWLEDGMENTS ofsolidhelium-4usingtherigiddouble-torustorsionalos- cillator. Theperioddropanomalyisobservedforbothin- The authors acknowledge Duk Y. Kim at Pennsylva- phaseandout-of-phasemodes. Frequencyanalysisshows nia State University for fruitful discussions and advices thatthefrequency-independentperiodshiftislessthan4 in the early stage of construction of the rigid double- ppm, closeto the upper limit setby the PSU group,and pendulum torsional oscillator. This work is supported thefrequency-dependentcontributionisalmostthesame by the National Research Foundation of Korea through as the TO response. We conclude that the TO response the Creative Research Initiatives. J. Choi would like to at low temperatures is not due to the appearance of su- thank the POSCO TJ Park Foundation for its financial persoliditybutduetothechangeintheshearmodulusof supportandgenerositythroughtheTJParkScienceFel- solid helium. 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