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Four-junction superconducting circuit Yueyin Qiu,1,2 Wei Xiong,1,2 Xiao-Ling He,3 Tie-Fu Li,4,2 and J. Q. You2 1Department of Physics, Fudan University, Shanghai 200433,China 2Beijing Computational Science Research Center, Beijing 100193, China 3School of Science, Zhejiang University of Science and Technology, Hangzhou, Zhejiang 310023, China 4Institute of Microelectronics, Department of Microelectronics and Nanoelectronics and Tsinghua National Laboratory of Information Science and Technology, Tsinghua University, Beijing 100084, China (Dated: August 4, 2016) We develop a theory for the quantum circuit consisting of a superconducting loop interrupted by four Josephson junctions and pierced by a magnetic flux (either static or time-dependent). In 6 addition to the similarity with the typical three-junction flux qubit in the double-well regime, we 1 demonstrate the difference of the four-junction circuit from its three-junction analogue, including 0 its advantages over the latter. Moreover, the four-junction circuit in the single-well regime is also 2 investigated. Our theory provides a tool to explore the physical properties of this four-junction superconductingcircuit. g u A SuperconductingquantumcircuitsbasedonJosephson son junctions in the four-junction circuit. We find that 3 junctions exhibit macroscopic quantum coherence and the four-junction circuit with only one smaller junction can be used as qubits for quantum information process- has a broader parameter range to achieve a flux qubit ] ing (see, e.g., Refs. [1–9]). Behaving as artificial atoms, inthedouble-wellregimethanthethree-junctioncircuit. h these circuits can also be utilized to demonstrate novel Moreover,forthefour-junctioncircuitwithtwoidentical p - atomic-physics and quantum-optics phenomena, includ- smaller junctions, the circuitcan be used as a qubit bet- t ing those that are difficult to observe or even do not oc- ter than the three-junction circuit, because it becomes n a cur in natural atomic systems [10]. As a rough distinc- more robust against the state leakage from the qubit u tion,therearethreetypesofsuperconductingqubits,i.e., subspace to the third level. This can be a useful advan- q charge[1,2],flux[4,11]andphasequbits[5,6,12]. Inthe tage of the four-junction circuit over the three-junction [ charge qubit, where the charge degree of freedom domi- circuit when used as a qubit. Also, we study the four- 2 nates, two discrete Cooper-pair states are coupled via a junction circuit in the single-well regime, which was not v Josephson coupling energy [1, 2]. In contrast, the phase exploited before. Our theory can provide a useful tool 2 degree of freedom dominates in both flux [11] and phase to explore the physical properties of this four-junction 7 qubits [5, 6]. superconducting circuit. 0 The typical flux qubit is composed of a superconduct- 0 ing loop interrupted by three Josephson junctions [11]. 0 . Similar to other types of superconducting qubits, it ex- 2 Results hibits good quantum coherence and can be tuned ex- 0 6 ternally. Recent experimental measurements [9] showed Four-junctionsuperconductingcircuit. (1)Theto- 1 thatthedecoherencetimeofthethree-junctionfluxqubit tal Hamiltonian. Let us considera superconducting loop : canbelongerthan40µs. Duetotheconvenienceinsam- interrupted by four Josephson junctions and pierced by v ple fabrication (i.e., the double-layer structure fabrica- a magnetic flux [see Fig. 1(a)], where the first and sec- i X tion by the shadowevaporationtechnique [13]), a super- ond junctions have identical Josephson coupling energy r conducting loopinterruptedby four Josephsonjunctions EJ and capacitance C (i.e., EJi =EJ and Ci =C, with a was also used as the flux qubit. The experiments [14] i=1,2),whilethethirdandfourthjunctionsarereduced showedthatthis four-junctionflux qubitbehavessimilar as E = αE , E = βE , C = αC, and C = βC, J3 J J4 J 3 4 to the three-junction flux qubit. Also, two four-junction with 0 < α,β < 1. The phase drops ϕ (i = 1,2,3,4) i flux qubits were interacting experimentally via a cou- through these four Josephson junctions are constrained pler [15], similar to the interqubit coupling mediated by by the fluxoid quantization a high-excitation-energy quantum object [16]. The the- ory of the three-junction flux circuit with a static flux ϕ +ϕ +ϕ +ϕ +2πf (t)=0, (1) bias was well developed [17], but a theory for the four- 1 2 3 4 tot junctioncircuitlacksbecauseaddingoneJosephsonjunc- tionmoretothesuperconductingloopmakestheproblem where ftot(t) = Φtot(t)/Φ0, with Φtot(t) being the to- more complex. tal magnetic flux in the loop (which includes the exter- Inthispaper,wedevelopatheoryforthefour-junction nally applied flux, either static or time-dependent, and circuitwitheitherastaticortime-dependentfluxbias. In the inductance-induced flux owing to the persistent cur- additiontothe similaritywiththe three-junctioncircuit, rentintheloop)andΦ0 =h/2ebeing the fluxquantum. we demonstrate the difference from the three-junction The kinetic energy of the four-junction circuit is the circuitduetothedifferentsizesofthetwosmallerJoseph- electrostaticenergy[18]storedinthejunctioncapacitors, 2 (a) φ E (b) where 1 J 2πβ ξ =f f , b= , φ2EJ Φtot(t) φ4βEJ φ1EJ Φtot(t) φ2EJ tot− e −α+β+2αβ α+β λ± b± = | − | , (5) 2(α+β)2+4β2 4(β+α)λ±+2λ2± φ αE φ αE − 3 J 3 J q (1+α+3β) 1+(α β)2+8β2+2(β α) λ± = ± − − , FIG. 1: (color online) Schematic diagram of the considered 2 p superconducting circuits. (a) Superconducting loop inter- with f =Φ /Φ being the reduced static magnetic flux rupted by four Josephson junctions and pierced by a total e e 0 applied to the superconducting loop. The electrostatic magnetic flux, Φ (t), which includes the externally applied tot energy can then be converted to a quadratic form flux and the inductance-induced flux. Here two of the four T junctions have identical Josephson coupling energy EJ and 2 C Φ csoanpaccoituapnlicnegCe.neArgmyoαngEJotahnedr tcwapoajcuintacnticoenαs,Co,naenhdasthJeosoetphher- T = 2 2π0 (ϕ˙2+Γ+ϕ˙2++Γ−ϕ˙2−+Γξξ˙2), (6) (cid:18) (cid:19) hasJosephsoncouplingenergyβEJ andcapacitanceβC,with where 0<α,β <1. (b) Superconducting loop interrupted by three Josephson junctions and pierced by a total magnetic flux 4β2 2β2(α+β) Φpltiontg(te),newrghyerEeJtwaondjucnacptaiocnitsanhcaeveC,idwenhtiliecatlhJeotsheiprhdsoonnechoaus- Γ± =2b2±(cid:20)1+2β− α+β−λ± + (α+β−λ±)2(cid:21), Josephson coupling energy αEJ and capacitance αC, with Γξ = 2α2+4βα2+α+β+4αβ b2 (7) 0<α<1. In both (a) and (b),each red component denotes the thin insulator layer of a Josephson junction, and an ar- (cid:0)+4πβ(1+2α)b+4π2β. (cid:1) rowalongtheloopdenotestheassigneddirectionofthephase The total Josephson coupling energy of the four- dropacrossthecorrespondingJosephson junction. Notethat junction circuit is each phase drop can be chosen along either the clockwise or counter-clockwise direction, but once the direction is fixed, 4 thephase drop is positive along it. U = E (1 cosϕ ) Ji i − i=1 X =E [2+α+β cosϕ cosϕ J 1 2 − − αcosϕ βcos(ϕ +ϕ +ϕ +2πf )] which can be written as − 3− 1 2 3 tot ϕ =EJ 2+α+β cos +b+ϕ++b−ϕ−+αbξ − √2 4 (cid:20) (cid:18) (cid:19) 1 = C V2, (2) ϕ T 2Xi=1 i i −cos(cid:18)−√2 +b+ϕ++b−ϕ−+αbξ(cid:19) 2βb+ 2βb− αcos ϕ+ ϕ−+bξ where Vi =(Φ0/2π)ϕ˙i is the voltage acrossthe ith junc- − (cid:18)−α+β−λ+ − α+β−λ− (cid:19) tion. Using the the fluxoid quantization condition in 2(α λ+)b+ 2(α λ−)b− βcos − ϕ++ − ϕ− Eq. (1), we can rewrite the kinetic energy as − (cid:18) α+β−λ+ α+β−λ− +(2αb+b+2π)ξ+2πf . (8) e C Φ 2 (cid:19)(cid:21) = 0 ϕ˙2+ϕ˙2+αϕ˙2 (3) T 2 2π 1 2 3 Also,thereis the inductive energydue to the inductance (cid:18) (cid:19) (cid:26) L of the superconducting loop [19]: 2 +β ϕ˙ +ϕ˙ +ϕ˙ +2πf˙ . 1 2 3 tot Φ2 h i (cid:27) UL = 0(ftot fext)2, (9) 2L − where the reduced externally-applied magnetic flux f We introduce a phase transformation ext cangenerallybe written asa sumofthe static andtime- dependent fluxes, i.e., f = f + f (t), with f (t) ext e a a ≡ ϕ Φ (t)/Φ being the reduced time-dependent magnetic ϕ1 = √2 +b+ϕ++b−ϕ−+αbξ, fieald app0lied to the four-junction loop. When including ϕ this inductive energy, the total potential energy of the ϕ2 =−√2 +b+ϕ++b−ϕ−+αbξ, (4) four-junction circuit is written as 2βb+ 2βb− Φ2 ϕ3 =−α+β λ+ϕ+− α+β λ−ϕ−+bξ, U =U(ϕ,ϕ+,ϕ−,ξ)+ 2L0(ξ−fa)2. (10) − − 3 The Lagrangianof the four-junction circuit is i.e., a harmonic oscillator driven by a time-dependent magnetic flux f (t). The angular frequency of this har- a = monic oscillator is L T −U = C2 Φ2π0 2(ϕ˙2+Γ+ϕ˙2++Γ−ϕ˙2−+Γξξ˙2) ωosc = 1 . (17) (cid:18) (cid:19) ΓξCL Φ2 U(ϕ,ϕ+,ϕ−,ξ) 0(ξ fa)2. (11) Withtheparametersachievpedinexperimentsfortheflux − − 2L − qubit [14, 20], α 0.7, C 8 fF, and L 10 pH. More- ∼ ∼ ∼ where we assign ϕ, ϕ±, and ξ as the canonical coor- over, β α, so ωosc/2π 1 103 GHz. For the four- ∼ ∼ × dinates. The corresponding canonical momenta P = junctionfluxqubit,theenergygap∆betweenthelowest ∂ /∂ϕ˙, P± =∂ /∂ϕ˙±, and Pξ =∂ /∂ξ˙ are two levels is typically ∆ 1-10 GHz [14, 15], which is L L L much smaller than ω /2∼π 1 103 GHz. Usually, osc Φ0 2 the time-dependent magnetic∼flux×fa(t) applied to the P =C ϕ˙, four-junction loop is a microwave wave with ω /2π 1- 2π a (cid:18) (cid:19) 10 GHz, which is also much smaller than ω /2π.∼Be- P± =C Φ0 2Γ±ϕ˙±, (12) cause ∆ ≪ ωosc/2π and the flux fa(t) is aolssco very off 2π resonance from the harmonic oscillator (i.e., ω ω ), (cid:18) (cid:19) a ≪ osc 2 the oscillator is nearly kept in the ground state at a low Φ Pξ =C 0 Γξξ˙. temperature. Then, using the adiabatic approximation 2π (cid:18) (cid:19) to eliminate the degree of freedom of the oscillator, the Hamiltonian of the four-junction circuit can be reduced Therefore,theHamiltonianofthefour-junctioncircuitis to given by P2 P2 H = P ϕ˙ H =4EC P2+ + + − +U(ϕ,ϕ+,ϕ−,ξ). (18) i i−L (cid:18) Γ+ Γ−(cid:19) i X P2 P2 P2 Also,bothLandthepersistentcurrentI ofthesupercon- = 4E P2+ + + − + ξ ducting loop are small, so that IL/Φ 10−3 [17]. This C 0 Γ+ Γ− Γξ! inductance-induced flux is much smalle∼r than the exter- +U(ϕ,ϕ+,ϕ−,ξ)+ Φ20(ξ fa)2, (13) nthaellytoatpapllflieudxmfagnceatnicafllusoxbfeextap=prfoex+imfaat(etl)y. Twhrietrteefnoraes, 2L − tot f f +f (t). tot e a ≃ where E = e2/(2C) is the single-particle charging en- Below we first study the static-flux case, i.e., only a C ergy of the Josephson junction. In comparison with the static magnetic flux is applied to the four-junction loop. previous work in Ref. [17] for the three-junctions flux In this case, ftot fe, so ξ 0. The phase transforma- ≃ ≃ qubit,anewdegreeoffreedomξisincludedintheHamil- tion in Eq. (4) becomes tonian, so that the Hamiltonian can also apply to the ϕ case when the superconducting loop contains a time- ϕ1 = +b+ϕ++b−ϕ−, √2 dependent magnetic flux. ϕ (2) The reduced Hamiltonian. The total Hamiltonian ϕ2 =−√2 +b+ϕ++b−ϕ−, (19) of the four-junction circuit can be rewritten as 2βb+ 2βb− ϕ3 = ϕ+ ϕ−, P2 P2 −α+β−λ+ − α+β−λ− H =4EC(cid:18)P2+ Γ++ + Γ−−(cid:19)+U(ϕ,ϕ+,ϕ−,ξ)+Hosc, and the Hamiltonian of the four-junction circuit in (14) Eq. (18) is further reduced to where P2 P2 Hosc = 4ΓECPξ2+ 2ΦL20(ξ−fa)2, (15) H0 =4EC(cid:18)P2+ Γ++ + Γ−−(cid:19)+U(ϕ,ϕ+,ϕ−), (20) ξ with U(ϕ,ϕ+,ϕ−) U(ϕ,ϕ+,ϕ−,ξ)ξ=0. ≡ | Quantum mechanically, the canonical momenta can be Figure 2 shows the contour plots of the potential wrii~t∂te/n∂ϕaξsiPn t=he−cia~n∂o/n∂icϕa,l-Pco±or=din−ait~e∂r/e∂pϕre±s,enatnadtioPnξ. = sUu(bϕs,pϕa+ce,ϕs−pa)nn≡edUb(yϕ1ϕ,ϕ12a,nϕd3)ϕi2nfothrefetw=o-d1i/m2e,nwsihonerael −Note that the Hamiltonian Hosc in Eq. (15) can be ϕi (i=1,2,3) are related to ϕ and ϕ± by Eq. (19). For rewritten as a three-junction flux qubit, α is usually in the range of 1/2 < α < 1. When 0 < α < 1/2, each double well in H = 4ECP2+ Φ20ξ2 Φ20ξf (t), (16) the potential is reduced to a single well [17], so the flux osc Γ ξ 2L − L a qubit in the double-well regime is converted to a flux ξ 4 (a) 2 (b)2 (c) 2 5.8 5.6 5.3 4.8 4.6 4.3 1 1 1 3.8 3.6 3.3 (cid:652) 2.8 2.6 2.3 (cid:21) 0 0 0 (cid:307)/2 1.8 1.6 1.3 -1 -1 -1 -2 -2 -2 -2 -1 0 1 2 -2 -1 0 1 2 -2 -1 0 1 2 (cid:307)1/(cid:21)(cid:652) (cid:307)1/(cid:21)(cid:652) (cid:307)1/(cid:21)(cid:652) FIG.2: (coloronline)ContourplotsofthepotentialU(ϕ1,ϕ2,ϕ3)atϕ3 =0andfe =1/2,where(a)α=1,β=0.8,(b)α=1, β =0.6, and (c) α=1, β =0.3. qubitinthesingle-wellregime. Forthefour-junctioncir- where K is a reciprocal lattice vector. Substituting cuit, there are wider ranges of parameters to achieve a Eq.(24)intoEq.(22),wethenobtainanequationsimilar flux qubit. For instance, in the case of three identical tothecentralequationinthetheoryofenergybands[21]. Josephson junctions (i.e., α = 1 and 0 < β < 1), when Numerically solving this equation, we can obtainthe en- β >1/3,thepotentialU(ϕ ,ϕ ,ϕ )hastwoenergymin- ergy spectrum and eigenstates of the Hamiltonian H . 1 2 3 0 ima in the unit cell of three-dimensional periodic lattice For the three-junction flux qubit, an approximate ∗ at ϕ =ϕ =ϕ = ϕ mod 2π, where tight-binding solution was obtained in Ref. [17] by pro- 1 2 3 ± jectingtheSchr¨odingerequationontothequbitsubspace, ∗ 3β 1 where the needed tunneling matrix elements were esti- ϕ =arcsin − . (21) s 4β ! mated using the WKB method. For the four-junction case,suchanapproximatetight-bindingsolutioncanalso A flux qubit in the double-well potential can then be be derived, but it is difficult to calculate the tunneling achieved in the parameter range of 1/3 < β < 1, which matrix elements via the WKB method, because a three- is broader than the range of 1/2 < α < 1 for the three- dimensionalpotentialisinvolvedinthefour-junctioncir- junctionfluxqubit. Figures2(a)and2(b)showasection cuit. Thus, we resortto the numerical approachto solve of U(ϕ1,ϕ2,ϕ3) at ϕ3 =0. Corresponding to the above- the Schr¨odinger equation in Eq. (22). With this numeri- mentionedtwominima,afigure-eight-shapeddoublewell cal approach,we can obtain the results for both the flux exists in each unit cell of the periodic lattice in the two- qubit and the three-level system. dimensional subspace. When β <1/3, each figure-eight- Figure 3 shows the energy levels of the four-junction shaped double well in the ϕ3 = 0 section of the poten- circuit versus the reduced static flux fe, in compari- tial is reduced to a single well [see Fig. 2(c)], with only son with the three-junction circuit. In the case of four- one minimum in the unit cell at ϕ1 = ϕ2 = 0 mod 2π. junction circuit, when the lowest two or three levels are Thiscorrespondstoafluxqubitinthesingle-wellregime considered,the energy spectrum with α=1 and β =0.6 achieved in the four-junction superconducting circuit. is similar to the energy spectrum with α = 0.7 in the case of three-junction circuit [comparing Fig. 3(c) with Energy spectrum. The energy spectrum and eigen- Fig. 3(a)]. Because the lowest two levels are well sepa- states of the four-junction circuit are determined by ratedfromotherlevels,boththree-andfour-junctioncir- H Ψ(ϕ)=EΨ(ϕ), (22) cuits can be utilized as quantum two-level systems (i.e., 0 flux qubits). In this case, the flux qubit can be modeled where ϕ (ϕ,ϕ+,ϕ−) = (ϕ1,ϕ2,ϕ3) is a three- as ≡ dimensional vector in the phase space. Equation (22) 1 isjustlikethequantummechanicalproblemofaparticle H = (εσ +∆σ ), (25) 0 z x moving in a three-dimensional periodic potential U(ϕ). 2 Thus, the solution of it has the Bloch-wave form where the tunneling amplitude ∆ correspondsto the en- Ψ(ϕ)=eik·ϕu(ϕ), (23) ergy difference between the two lowest-energy levels at f =1/2,andε=2I Φ (f 1/2)is the biasenergydue e p 0 e where k is a wavevector and u(ϕ) is a periodic function − totheexternalflux,withI beingthemaximalpersistent p in the phases of ϕ (i = 1,2,3). Also, Ψ(ϕ) should be i currentcirculatinginthe loop. Herethemaximalpersis- periodic in the phases of ϕ . To ensure this, the wave- i tent current I can be approximately calculated as [17] p function Ψ(ϕ) is constrained by k=0. Then, Ψ(ϕ) can I Φ−1∂E /∂f at a value of f considerably away be written as p ≈ | 0 0 e| e fromf =1/2,whereE istheenergyleveloftheground e 0 Ψ(ϕ)=u(ϕ)= aKeiK·ϕ, (24) state of the system. The Pauli operators σz and σx are representedusingthetwo(i.e.,theclockwiseandcounter- K X 5 FIG.3: (coloronline) Energyspectraof thesuperconductingcircuitsversusthereducedstaticfluxfe. (a)α=0.7and(b)0.4 inthecaseofthree-junctioncircuit;(c)α=1andβ=0.6,(d)α=1andβ =0.3,(e)α=β=0.6,(f)α=β =0.3,(g)α=0.5 and β =0.6, and (h) α=0.2 and β =0.3 in the case of four-junction circuit. In this figure and the following one, we choose EJ =50EC . clockwise)persistent-currentstates. Moreover,similarto system. However, our calculations on transition matrix the three-junction circuit, the four-junction circuit can elementsindicate thatthe circuitcanstillbe better used also be used as a quantum three-level system (qutrit) as a qubit, because only the transition matrix element owing to the considerable separation of the third energy between the ground and first excited states is apprecia- levelfromotherhigherlevelsaswell. Whenreducingthe bly large (see the next section). smallest junction to, e.g., β = 0.3 in the four-junction In addition, we further consider the case of two differ- circuit [see Fig. 3(d)], only the lowest two levels are well ent smallerJosephsonjunctions (i.e., α=β) in the four- separated from other levels, similar to the case of three- 6 junctioncircuit. Inthe double-wellregime[seeFig.3(g), junction circuit in Fig. 3(b) where α = 0.4. Now the where α = 0.5 and β = 0.6], the energy levels look sim- double-well potential has been convertedto a single well ilar to those in Fig. 3(e) and the lowest two levels can (see Fig. 2), so the circuit behaves as a flux qubit in still be used as a qubit. Also, this qubit is less sensitive the single-well regime. Compared to the flux qubits in to the influence of the external magnetic field around Figs. 3(a) and 3(c), the energy levels in Figs. 3(b) and the degeneracypoint,becausethe energylevelsaremore 3(d) are less sensitive to the external flux f , so the ob- e flat than those in Fig. 3(e). In the single-well regime tained flux qubits in the single-well regime are more ro- [see Fig. 3(h), where α = 0.2 and β = 0.3], the low- bust against the flux noise. However,because the small- est three levels are well separatedfrom the higher levels. estJosephsonjunctionintheloopisfurtherreduced,the Moreover, in addition to the transition matrix element charge noise may become important [22]. To suppress between the ground and first excited states, the transi- this charge noise, one can shunt a large capacitance to tionmatrixelementbetweenthe firstandsecondexcited the smallest junction to improve the quantum coherence states is also larger (see the section below). Therefore, of the qubit [9, 22, 23]. in the single-well regime, the four-junction circuit in the Furthermore, let us consider the four-junction cir- caseofα=β canbebetterusedasaquantumthree-level 6 cuit with two identical smaller Josephson junctions. In system. ThisisdifferentfromthecasesinFigs.3(b),3(d) Fig. 3(e) where α = β = 0.6, the lowest two levels are and 3(f). also well separated from other levels, but the third level is not so separated from higher levels. Thus, from the Transition matrix elements. Now we consider the energy-level point of view, this four-junction circuit can time-dependent case with f (t) f + f (t), i.e., in tot e a ≃ be better used as a flux qubit than a three-level system. additiontoastaticfluxf ,atime-dependentfluxf (t) e a ≡ In Fig. 3(f) where α = β = 0.3, the lowest three levels Φ (t)/Φ isalsoappliedtothefour-junctionloop. Inthis a 0 are well separated from other levels. It seems that the case, ξ f (t) when ignoringthe very smallinductance- a ≃ four-junction circuit can be better used as a three-level induced flux. For a small enough time-dependent flux, 6 only the first-order perturbation due to ξ needs to be Here we consider a microwave field with frequency considered in Eq. (18). Then, the Hamiltonian of the ω applied to the superconducting loop. The time- a four-junction circuit in Eq. (18) can be expressed as dependent magnetic flux in the loop can be written as Φ (t)=Φ(0)cosω t. Then, with the current I available, ′ a a a H =H +H (t), (26) 0 the magnetic-dipole transition matrix elements are cal- culated by with H given in Eq. (20) and 0 t = iIΦ(0) j , (32) ′ ϕ ij h | a | i H (t)=fa(t)EJ αbsin +b+ϕ++b−ϕ− √2 where i and j are eigenstates of the Hamiltonian H (cid:20) (cid:18) (cid:19) | i | i 0 ϕ in Eq. (20). +αbsin −√2 +b+ϕ++b−ϕ− Figure 4 shows the transition matrix elements |t01|, (cid:18) (cid:19) t , and t of the three- and four-junction circuits as 02 12 αbsin 2βb+ ϕ++ 2βb− ϕ− |a fu|nction|of|the reduced static flux fe, where the sub- − (cid:18)α+β−λ+ α+β−λ− (cid:19) scripts0,1 and2 correspondto the groundstate|0i, the 2(α λ )b first excited state 1 , and the second excited state 2 +(2αb+b+2π)βsin − + +ϕ | i | i α+β λ + ofthe system, respectively. Similar to the three-junction (cid:18) − + circuit in Fig. 4(a) where α = 0.7, the four-junction cir- 2(α λ−)b− + − ϕ−+2πfe . (27) cuit with α = 1 and β = 0.6 (i.e., there is only one α+β−λ− (cid:19)(cid:21) smaller Josephson junction in the circuit) behaves as a Thetime-dependentperturbationH′(t)canberewritten ladder-type (namely, Ξ-type [24]) three-level system at f =1/2,and a cyclic-type (∆-type [25]) three-levelsys- as e tematf =1/2[seeFig.4(c)]. FortheΞ-typethree-level e 6 H′(t)= IΦa(t), (28) system achieved when fe = 1/2, the transition between − the ground state 0 and the second excited state 2 is | i | i where notallowed,whichis analogousto anaturalatom. How- ever, for the ∆-type three-level system at f = 1/2, all I =−EΦJ0(cid:20)αbsin(cid:18)√ϕ2 +b+ϕ++b−ϕ−(cid:19) dtriaffnesrietniotnfsroammoannga|t0uir,al|1aitoamndic|2syisaterema[l2lo5w].eed6W. hTenhisthies ϕ smallest Josephson junction is further reduced, t is +αbsin −√2 +b+ϕ++b−ϕ− greatly suppressed. Now both three- and four-ju|n0c2t|ion (cid:18) (cid:19) circuits behave more like a Ξ-type three-level system in 2βb+ 2βb− −αbsin(cid:18)α+β−λ+ϕ++ α+β−λ−ϕ−(cid:19) theAws hfoolre trhegeiofnouorf-jfuenschtioownnciinrcFuiigts.w4i(tbh) tawnod 4id(de)n.tical +(2αb+b+2π)βsin 2(α−λ+)b+ϕ+ smaller Josephson junctions (α=β), while |t01| remains α+β λ appreciably large, the transition between 0 and 2 as (cid:18) − + | i | i + 2α(α+−βλ−λ)−b−ϕ−+2πfe (29) dwueclledas(tih.ee.,tr|at0n2s|it≈ion0baetnwdee|tn12|1|i≈an0d)|2ini atrheegwrehaotlley rree-- − (cid:19)(cid:21) gion of f shown in Figs. 4(e) and 4(f). Now, in either e is the current in the superconducting loop. Because double- or single-well regime, the four-junction circuit can be well used as a qubit, because the state leakage (2αb+b+2π)β = αb from the qubit subspace to the third level is suppressed. − 2παβ Thisisanapparentadvantageofthefour-junctioncircuit = , (30) −α+β+2αβ over the three-junction circuit when used as a qubit. WhenthetwosmallerJosephsonjunctionsinthefour- we can express the current I as junction circuit become different (i.e., α = β), in ad- 6 dition to t , both t and t become nonzero ex- 01 02 12 αβ 2πE | | | | | | I = J [sinϕ +sinϕ +sinϕ cept for the degeneracy point [see Figs. 4(g) and 4(h)]. 1 2 3 α+β+2αβ (cid:18) Φ0 (cid:19) This circuit behaves very different from the circuit with sin(ϕ +ϕ +ϕ +2πf )] twoidenticalsmallerjunctions[comparingFig.4(g)with 1 2 3 e − 1 Fig. 4(e), and comparing Fig. 4(h) with Fig. 4(f)], but = (αβI +αβI +βI +αI ), (31) 1 2 3 4 it is similar to the three-junction circuit and the four- α+β+2αβ junction circuit with only one smaller junction [compar- where I = I sinϕ , with i = 1,2 and I = 2πE /Φ , ing Fig. 4(g) with Figs. 4(a) and 4(c), and comparing i c 1 c J 0 I =αI sinϕ , andI =βI sinϕ areJosephsonsuper- Fig. 4(h) with Figs. 4(b) and 4(d)]. However, when the 3 c 3 4 c 4 currents through the four junctions. The phase drops ϕ distributionoftheenergylevelsisalsotakenintoaccount i (i=1,2,3) are related to ϕ and ϕ± by Eq. (19), and ϕ4 (see Fig. 3), the four-junction circuit with α= β can be 6 is constraintby the fluxoidquantizationconditioninthe better used as a quantum three-level system (qutrit) in static-flux case, i.e., ϕ +ϕ +ϕ +ϕ +2πf =0. the single-well regime. This is very different from the 1 2 3 4 e 7 0.6 0.6 0.6 0.6 (a) |t | (c) (e) (g) 01 |t | 02 0.4 |t | 0.4 0.4 0.4 12 0.2 0.2 0.2 0.2 s nt e m ele 0.0 0.0 0.0 0.0 x atri 0.48 0.49 0.50 0.51 0.52 0.48 0.49 0.50 0.51 0.52 0.48 0.49 0.50 0.51 0.52 0.48 0.49 0.50 0.51 0.5.2 m sition 0.3 (b) 0.3 (d) 0.3 (f) 0.3 (h) n a Tr 0.2 0.2 0.2 0.2 0.1 0.1 0.1 0.1 0.0 0.0 0.0 0.0 0.48 0.49 0.50 0.51 0.52 0.48 0.49 0.50 0.51 0.52 0.48 0.49 0.50 0.51 0.52 0.48 0.49 0.50 0.51 0.52 fe fe fe fe FIG.4: (coloronline)Transition matrixelements|t01|,|t02|and|t12|ofthesuperconductingcircuits(inunitsofIcΦ(a0))versus the reduced static flux fe. (a) α=0.7 and (b) 0.4 in the case of three-junction circuit; (c) α=1 and β =0.6, (d) α=1 and β =0.3, (e) α=β =0.6, (f) α=β =0.3, (g) α=0.5 and β =0.6, and (h) α=0.2 and β =0.3 in the case of four-junction circuit. three-junction circuit and the four-junction circuit with regimes. In addition to the similarity with the three- only one smaller junction, which can be better used as a junction circuit, we show the difference of the four- qubit in the single-well regime. Therefore, as compared junction circuit from its three-junction analogue. Also, tothethree-junctioncircuit,thefour-junctioncircuitcan we demonstrate its advantages over the three-junction provide more choices to achieve different quantum sys- circuit. Owing to the one additional Josephson junction tems. inthecircuit,thephysicalpropertiesofthefour-junction circuitbecomericherthanthoseofthethree-junctioncir- cuit. For instance, in the case of four-junction circuit withonlyonesmallerJosephsonjunction,thecircuithas Summary a broader parameter range to achieve a flux qubit in the We have developed a theory for the four-junction super- double-well regime than the three-junction circuit does. conducting loop pierced by an externally applied mag- Moreover, in the case of four-junction circuit with two netic flux. When the loop inductance is considered, the identical smaller junctions, the circuit can be used as derived Hamiltonian of this four-junction circuit can be a qubit better than the three-junction circuit in both written as the sum of two parts, one of which is the double- and single-well regimes. This is because among Hamiltonian of a harmonic oscillator with a very large the lowest three eigenstates of the four-junction circuit, frequency. This makes it feasible to employ the adia- only the transition matrix element between the ground batic approximation to eliminate the degree of freedom and first excited states is appreciably large, while other oftheharmonicoscillatorinthetotalHamiltonian. Also, two elements become zero. These properties of the four- this theory can be used to study the case when the ap- junction circuit can suppress the state leakage from the pliedmagnetic-fluxbiasbecomestime-dependent. Inthe qubit subspace to the second excited state, and the cir- case of static flux bias, the total Hamiltonian of the cuitwiththeseparametersisthusexpectedtohavebetter four-junction circuit is reduced to the Hamiltonian of quantum coherence when used as a qubit. the superconducting qubit. When the flux bias is time- dependent,thetotalHamiltonianofthefour-junctioncir- cuit can be reduced to the Hamiltonian of the supercon- Methods ducting qubit plus a perturbation related to the applied time-dependent flux. Then, we can calculate the energy Three-junction circuit with a time-dependent spectrumandthe transitionmatrixelements ofthe four- magnetic flux. To compare with our four-junction re- junction superconducting circuit. sults, we also consider a three-junction superconducting In conclusion, we have studied the four-junction su- loop pierced by a time-dependent total magnetic flux perconducting circuit in both double- and single-well Φ (t) [see Fig. 1(b)], because no explicit derivation ex- tot 8 ists in the literature for this time-dependent case. The Because L is small in a three-junction flux qubit [17], directions of the phase drops ϕ (i = 1,2,3) through we canignorethe flux generatedby the loopinductance. i the three Josephson junctions are chosen as in Ref. [17], Thus, when only a static flux is applied to the loop, which are constrained by the following fluxoid quantiza- f (t) f , i.e., ξ 0. The phase transformation in tot e ≃ ≃ tion condition: Eq. (34) becomes ϕ1−ϕ2+ϕ3+2πftot(t)=0, (33) ϕ = ϕ1+ϕ2, ϕ = ϕ1−ϕ2, (40) p m 2 2 where f (t) = Φ (t)/Φ . Here we assume that two tot tot 0 larger junctions have identical capacitance C and cou- andthe Hamiltonianof the circuitin Eq.(39)is reduced pling energy E , while the smaller junction has capaci- J to tance αC and coupling energy αE , with 0<α<1. J Similar to the four-junction circuit, we introduce a 2E phase transformation H0 =2ECPp2+ (1+C2α)Pm2 +EJ[2+α (41) ϕp = ϕ1+ϕ2, −2cosϕpcosϕm−αcos(2ϕm+2πfe)], 2 ϕ ϕ 2πα 1 2 whichisthe Hamiltonianofthe three-junctionfluxqubit ϕ = − + ξ, (34) m 2 1+2α derived in Ref. [17]. For the time-dependent case with f (t) f +f (t), where ξ ftot(t) fe, with fe = Φe/Φ0 being the re- tot ≃ e a ≡ − ξ f (t), where f (t) Φ (t)/Φ is the reduced time- duced static magnetic flux applied to the superconduct- ≃ a a ≡ a 0 dependent magnetic flux applied to the three-junction ing loop. The Hamiltonian of the three-junction circuit loop. When the time-dependent magnetic flux is small can be derived as enough, only the first-order perturbation due to ξ needs H =2E P2+ 2EC P2 +U(ϕ ,ϕ ,ξ)+H , (35) to be considered, and the Hamiltonian of the circuit in C p (1+2α) m p m osc Eq. (39) can be expressed as where EC =e2/(2C), H =H +H′(t), (42) 0 2πα U =EJ 2+α−2cosϕpcos ϕm− 1+2αξ with H0 given in Eq. (41) and H′(t)=−IΦa(t), where (cid:26) (cid:18) (cid:19) 2π −αcos 2ϕm+ 1+2αξ+2πfe , (36) I = 2πα EJ [2cosϕpsinϕm sin(2ϕm+2πfe)] (cid:18) (cid:19)(cid:27) 1+2αΦ0 − (43) and is the current in the three-junction loop [26]. Using E (1+2α) Φ2 Eq. (40) and the fluxoid quantization condition in the H = C P2+ 0(ξ f )2. (37) osc π2α ξ 2L − a static-flux case (i.e., ϕ1 ϕ2+ϕ3+2πfe = 0), the cur- − rent I can also be rewritten as Quantum mechanically, the canonical momenta can be written as P = i~∂/∂ϕ , P = i~∂/∂ϕ , and P = p p m m ξ α 2πE −iT~∂h/e∂aϕnξguinlarthfre−ecqauneonnciycaolf-cthooerhdainr−matoenriecporsecsiellnattaotriogniv.en I = 1+2α(cid:18) Φ0J(cid:19)[sinϕ1−sinϕ2 sin(ϕ ϕ +2πf )] in Eq. (37) is 1 2 e − − 1 = (αI αI +I ), (44) 1+2α 1+2α 1− 2 3 ω = . (38) osc αCL r where I is the Josephson supercurrent through each i Using the parameters achieved in experiments [14, 20], junction. Moreover, as in Eq. (32), the magnetic- we have α 0.7, C 8 fF, and L 10 pH, so one dipole transitionmatrix elements are calculatedby t = has ωosc/2π∼∼ 103 GH∼z, which is muc∼h larger than the iIΦ(a0) j ,where i and j areeigenstatesoftheHaimjil- energygap∆ 1-10GHzofthethree-junctionfluxqubit h | | i | i | i (see, e.g., Ref.∼[4]). If the time-dependent magnetic flux tonian H0 in Eq. (41). is the usually applied microwave field, the oscillator can indeed be regardedas being in the groundstate at a low temperature,asanalyzedforthe four-junctionfluxqubit Acknowledgement in the main text. Then, the Hamiltonian of the three- This work is supported by the NSAF Grant No. junction circuit can be reduced to U1330201, the National Natural Science Foundation of China Grant No. 91121015, and the National Basic Re- 2E H =2E P2+ C P2 +U(ϕ ,ϕ ,ξ). (39) search Programof China Grant No. 2014CB921401. C p (1+2α) m p m 9 [1] Nakamura,Y.,Pashkin,Y.A.&Tsai,J.S.Coherentcon- (2005). trol of macroscopic quantum states in a single-Cooper- [15] Niskanen, A. O. et al. Quantum coherent tunable cou- pair box.Nature 398, 786-788 (1999). pling of superconducting qubits. Science 316, 723-726 [2] Bouchiat, V. et al. Quantum coherence with a single (2007). Cooper pair. Phys. Scr. T76, 165-170 (1998). [16] Ashhab, S. et al. Interqubit coupling mediated by a [3] Vion, D. et al. 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