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Four-body correlations in nuclei M. Sambataroa and N. Sandulescub aIstituto Nazionale di Fisica Nucleare - Sezione di Catania, Via S. Sofia 64, I-95123 Catania, Italy bNational Institute of Physics and Nuclear Engineering, P.O. Box MG-6, Magurele, Bucharest, Romania Low-energyspectraof4nnucleiaredescribedwithhighaccuracyintermsoffour-bodycorrelated structures (“quartets”). The states of all N ≥Z nuclei belonging to the A=24 isobaric chain are representedasasuperposition oftwo-quartetstates,withquartetsbeingcharacterizedbyisospinT and angular momentum J. These quartets are assumed to be those describing the lowest states in 20Ne(Tz=0),20F(Tz=1) and20O(Tz=2). Wefindthatthespectrumof theself-conjugate nucleus 24MgcanbewellreproducedintermsofT=0quartetsonlyandthat,amongthese,theJ=0quartet 5 plays by far the leading role in the structure of the ground state. The same conclusion is drawn 1 in the case of the three-quartet N = Z nucleus 28Si. As an application of the quartet formalism 0 to nuclei not confined to the sd shell, we provide a description of the low-lying spectrum of the 2 proton-rich92Pd. Theresultsachievedindicatethat,in4nnuclei,four-bodydegreesoffreedomare more important and more general than usually expected. n a PACSnumbers: 21.10.-k,21.60.Cs,21.60.Gx J 6 1 Innuclear physics,four-bodycorrelatedstructuresare Microscopic quartet models have a long history in nu- usually associated with α-clustering. α-clustering is clear structure. They have been employed to treat the ] h known to be a relevant phenomenon in light N =Z nu- proton-neutron (pn) interaction, in particular the pn t - clei especially at excitation energies close to the α emis- pairing, and to investigate the quartet condensation in l c sion threshold. A common theoretical approach to α- N = Z nuclei [3–8]. However, their complexity has al- u clustering is represented by the α-cluster model [1]. Ac- ways represented a hindrance to their development. Re- n cording to this model, the nucleus consists of a N = Z cently,asimpleapproachhasbeenproposedwhichisable [ core to which some α clusters are appended. These clus- to describe accurately the ground state of the isovector 1 ters are tightly bound and spatially localized structures pairingHamiltonianas acondensate ofquartets builtby v of two neutrons and two protons. The α-cluster model two neutrons and two protons coupled to total isospin 7 exhibitsastrikingcontrastwiththestandardshellmodel T = 0 and, for spherically symmetric mean fields, to 1 picture in which protons and neutrons are described in- total angular momentum J=0 [9]. This quartet model 0 4 steadasweaklyinteractingquasiparticlesinamean-field. conserves exactly the particle number, the isospin and 0 However, these two pictures are expected to coexist at the Pauli principle and can be applied for any number . low excitation energies where, due to the Pauli block- of quartets. Later on a more general description of the 1 0 ing which acts stronger than in the states close to the α ground state of N = Z nuclei as a product of distinct 5 emission threshold (e.g., see the case of the Hoyle state quartets has been proposed and applied to a description 1 [2]),theα-clusteringisexpectedtomanifestitselfmainly of both isovector (T = 1, J = 0) and isoscalar (T = 0, : v as four-body correlations in the configuration space. It J =1) pairing correlations [10, 11]. i is thus commonly supposed that correlated four-body X Of course, pairing is only a part (although a crucial structures (“quartets”) play a major role in the ground r one)ofthenuclearinteraction. Itisreasonabletoexpect a and excited sates of N = Z nuclei. However, to our thatarealisticdescriptionofself-conjugatenucleishould knowledge, this supposition has never been supported involve not only T =0, J =0 quartets. In the following by compelling calculations. In this letter, by using a we will show how the approach of Refs. [10, 11] has simple microscopic quartet model, we will show how the been extended to include quartets with arbitrary values low-energy spectra of 4n nuclei can be indeed described of isospin and angular momentum and to treat realistic in terms of quartets with an accuracy comparable with interactions of shell model type. state-of-the-art shell model calculations. We shall prove thatthisisthecasenotonlyforself-conjugatenucleibut One of the motivations of the present work has been also for 4n nuclei with N 6= Z. For the latter nuclei the thatofidentifying thequartetswhichcontributemostto low-lying states will be expressed in terms of quartets the structure of the low-lyingstates in even-evenN =Z built not only by two protons and two neutrons but also nuclei and, in particular, of investigating the role played by one protonandthree neutrons aswellas by four neu- by T = 0, J = 0 quartets in the ground state of these trons. This fact indicates that the four-body degrees of nuclei. Our analysis will be mainly confined to sd-shell freedom are important also for configurations which are nuclei. WewillbeginbyfixingasetofT =0,1,2quartets different from the α-like ones. and then use these quartets for a description of the low- lying states of 24Mg. To such a purpose, we will carry 2 out configurationinteraction calculations in spaces built 16O andthe nuclei which havetherefore been considered in terms of these quartets. By progressively restricting for the definition of the quartets are 20Ne , 20F and 10 10 9 11 thissetofquartetswewillidentifythemostrelevantones 20O . The lowest states of these nuclei are character- 8 12 forthe low-lyingstatesofthisnucleusand,inparticular, ized by T =0, 1 and 2, respectively. Each of these states for the ground state. A confirmation of the conclusions therefore identifies a quartet with given T,J (and a pro- reached for 24Mg will then be searched in the case of jectionT =(N−Z)/2). Wehavecarriedoutshellmodel z 28Si. HavingdefinedasetofT =0,1,2quartets,alarge calculations for these three nuclei and selected the quar- variety of nuclear systems become, in principle, within tetsassociatedwiththeloweststates. Moreprecisely,we reach in addition to self-conjugate nuclei. These include have retained the lowest 6 states in 20Ne (0 ≤J ≤6), 5 both even-even and odd-odd 4n nuclei. In the second statesin20F(1≤J ≤5)and9statesin20O(0≤J ≤4). part of the paper, we will provide a description of the For all calculations in the sd shell we have employed the whole isobaric chain of A=24 nuclei with N >Z in the USDBinteraction[12]whichgivesaprettygooddescrip- formalismofthesequartets. Finally,asanapplicationof tion of the above nuclei. The quartets so selected have the formalism to nuclei not confined to the sd shell, we then been employed in all the configuration interaction will discuss the case of the proton-rich 92Pd. calculations relative to the sd shell. Westartbybrieflyillustratingourapproach. Wework inasphericallysymmetricmeanfieldandlabelthesingle- particle states by i≡{n ,l ,j }, where the standard no- i i i tation for the orbital quantum numbers is used. The quartet creation operator is defined as 10 24Mg Q+α,JM,TTz = i1jX1J1T1i2jX2J2T2Ci(1αj)1J1T1,i2j2J2T2 51++62++ 12 12 10++625+++ ×h[a+i1a+j1]J1T1[a+i2a+j2]J2T2iJMTTz, MeV) 5 4230+++++ 4234++++ 4 where a+i creates a fermion in the single particle state i E ( + andJ(T)andM(T )denote,respectively,thetotalangu- + 2 z 2 lar momentum(isospin) and the relative projections. No 0 0+ 0+ restrictionsonthe intermediatecouplingsJ1T1 andJ2T2 55.69 55.69 55.17 54.91 are introduced in the calculations. In order to generate EXP SM QM QM(T=0) thespectraof4nnucleiweperformconfigurationinterac- tion calculations in spaces built in terms of selected sets of the above quartets. For these calculations we adopt a static definition of the quartets, i.e. after selecting the quartets (according to a criterion specified below) FIG. 1: The low-energy spectrum of 24Mg obtained in we keep them “frozen” in all calculations. This way of the quartet model (QM) compared to the experimental data constructing the quartets is substantially different from (EXP)andtotheshellmodel(SM)results. Thespectrumin- that of Refs.[10, 11] where we have instead adopted a dicated as QM(T=0) corresponds to a calculation done only dynamical definitionofthe T =0, J =0 quartets. That with T=0 quartets. In this figure as well as in all the re- maining ones relative to nuclei in the sd shell, experimental is to say, in these works,quartets have been constructed levelsandSMresultshavebeenextractedfromRef. [13]. The independently for each nucleus (via an iterative varia- number below each spectrum gives the ground state correla- tionalprocedure)andnoconnectionwhatsoevercouldbe tion energy, namely the difference between the total ground found among quartets of different nuclei. In the present state energy and theenergy in the absence of interaction. work, owing to the fact that various T,J quartets are being considered, this way of proceeding would become prohibitively cumbersome. However, for comparison, we We start our analysis by examining the self-conjugate willalsocarryoutananalysisofthegroundstatesofself- nucleus 24Mg. In Fig. 1, we compare the experimental conjugate nuclei by applying the same variationalproce- spectrum of this nucleus with that resulting from a shell dure of Refs. [10, 11]. model (SM) calculationand with the spectrum obtained The criterion adopted for the selection of the quartets inthequartetmodel(QM)whenalltheselectedT=0,1, has been that of choosing, as representative of the quar- 2quartets aretakeninto account. The quartetapproach tets with a given isospin T, those describing the lowest isseentoreproducewellboththeSMgroundstatecorre- levels with that isospin in nuclei with four active par- lation energy and the SM excited states up to an energy ticles outside the inert core of reference. For applica- of about 9 MeV. The SM is in turn able to fit well the tions within the sd shell, the inert core is representedby experimental levels. 3 HavingverifiedthattheselectedsetsofT=0,1,2quar- ergy. The best description of the ground state of 24Mg tets aresufficient to describe the low-energyspectrumof as a product of two T =0, J =0 quartets is expected to 24Mg,itbecomesofinteresttoinvestigatetheroleofthe be obtained by letting these quartets to be distinct from different quartets. We begin by focusing on isospin. In one another and by constructing them variationally. An Fig. 1, on the right hand side, we show the theoretical effective way to do that is provided by the procedure spectrum obtained in the quartet formalism when only adopted in Refs. [10, 11]. By applying this procedure T=0 quartets are retained. One can see that this spec- one is able to generate a ground state correlationenergy trum does not exhibit relevant differences with respect which exhausts 95.6% of the exact value. This calcula- to the full QM calculation. This provides a clear evi- tion therefore further enhances the role of T = 0, J = 0 dence of the marginal role played by the T=1 and T=2 quartets in this ground state and also suggests that the quartets in the structure of these states. As a next step, minimum set of T=0, J=0,2,4 quartets emerged from we concentrate on the ground state by employing only the aboveanalysismightbe further reducedwith amore T =0 quartets. In Fig. 2, we show how the error in the effective choice of the quartets. correlationenergyofthisstate,relativetotheSMresult, We havesearchedforaconfirmationofthe resultsjust varies by reducing, one quartet at a time and starting discussedbyexamininganotherself-conjugatenucleusin from the highest one in energy, the set of T=0 quartets. the sd shell: 28Si. We find that for this isotope the set The correlation energy remains basically unchanged up of T=0, J=0,2,4 quartets already exhaust almost 99% to the point where only the lowest J=0,2,4 quartets are of the correlation energy. Also in this case, the T = left. From this point on further reductions in the set 0, J = 0 quartet is found to play a leading role being of quartets lead to significant variations in the energy. able to account by itself for 93.4% of the total energy. Thus, these calculations indicate that the T=0 quartets This percentage increases to 98.2% when the quartets with J=0,2,4 play a major role in the ground state of are determined variationally. 24Mg. Among these quartets, the T=0, J=0 quartet is So far we have examined only self-conjugate nuclei. by far the one which contributes most to the correlation The rangeofnucleiwhichareaccessibleintermsofaset energy since, as it can be seen in Fig. 2, an approxima- ofT=0,1,2quartetsis,however,muchbroader. Limiting tionintermsofonlythisquartetaccountsforabout94% ourselves to the case of 8 active particles (two quartets) of the total energy. outside the 16O core, the whole isobaric chain of nuclei withA=24iswithinreach. Wehaveinvestigatedtowhat extent the spectra of these nuclei can be described in terms ofthe fullset ofT=0,1,2quartets employedin the case of 24Mg. The results are shown in Fig. 3 where 8 we compare the low-energy spectra of 24Na , 24Ne , 11 13 10 14 24F and 24O obtained in the quartet model with the 9 15 8 16 1: T=0, J=0(2), 2(2), 4, 6 SM results and with the experimental data. As one can 2: T=0, J=0(2), 2(2), 4 6 see, for all these nuclei the quartet formalism generates 3: T=0, J=0(2), 2, 4 4: T=0, J=0, 2, 4 spectra which agree well with the SM ones. It is worth ) 5: T=0, J=0, 2 stressingthatfor the nucleishowninFig. 3 the quartets % 6: T=0, J=0 ( 4 are built not only by two protons and two neutrons, as Ε ∆ in the case of N =Z nuclei, but also by one proton and threeneutronsandbyfourneutrons. Thecaseofquartets built by four like-particles had been already discussed 2 24Mg in Ref. [14] in relation with a treatment of the pairing Hamiltonian. In order to verify that the results presented so far are 0 1 2 3 4 5 6 not specific to sd-shell nuclei, we have carriedout a sim- ilar analysis for the proton-rich nucleus 92Pd . Calcu- 46 46 lations have been done in a space spanned by the p , 1/2 g orbitals using the F-FIT interaction by Johnstone FIG. 2: Relative errors (with respect to the SM value) in 9/2 thegroundstatecorrelation energyof24Mgcalculated inthe and Skouras [15]. In Fig. 4, one sees the low-lying yrast QM approach with the quartetsindicated in thefigure. spectrum that is obtained in the QM approach by em- ploying only T = 0 quartets. These quartets are those associatedwith the lowestlevels of 96Cd (7 levels with 48 48 In this connection, a few considerations are needed. 0≤ J ≤ 8) and include also a negative parity level with The static formulation of the quartets adopted in this J =5. TheQMyrastspectrumisseentoagreewellwith workisbyconstructionnotthemostperformingonesince the experimental one [16] as well as with the SM spec- itdoesnotguaranteeaminimuminthe groundstate en- trum generatedwithin the same model space by Herndl- 4 24Na 24Ne 11 13 10 14 ++ E (MeV)231 123++343+5++2+3+++ 215343++3+++3+++++2+ E (MeV)5 20++422+++ 343+++ 32423+++4+++02++ 21++ 21++ 0 4+ 4+ 0 0+ 0+ 46.23 46.29 45.44 40.26 40.32 40.05 EXP SM QM EXP SM QM 24F 24O 555+ 9 15 4++ 10 2+ 8 16 2+ 3 11+322432++++ 023+++15+ 243+++0+ 0+324+++ V) 00+ 4+ V) 1+ 1+ Me 1++ 4 1+ Me 5 2+ 2+ ( ( E E 2+ 2+ 0 3+ 3+ + + 0 0 0 23.56 23.47 23.35 9.93 9.82 9.82 EXP SM QM EXP SM QM FIG. 3: The spectra of A=24 nuclei generated by the QM approach compared with the experimental data and the SM predictions. See thecaption of Fig. 1 for further details. Brown[17]. Asinthecasesofthesdshellnucleianalyzed the valence shell. For all these nuclei, as well as for the above, the T =0, J =0 quartet is found to play a lead- proton-richnucleus92Pd,thequartetformalismhaspro- ing role in the ground state, accounting for almost 99% videdadescriptionofthelow-energyspectracomparable of the correlation energy. More details about the struc- in accuracy with that of shell model calculations. This ture of 92Pd in the quartet model will be presented in a fact confirms the importance of quartet degrees of free- separate study. dom in any type of 4n nuclei and validates the present quartet formalism as the appropriate tool for treating By summarizing, in this work we have presented an them. analysisof4nnucleiinaformalismofquartets,i.e.,four- body correlatedstructures characterizedby total isospin Asaconcludingremark,wenoticethatthedescription T andtotalangularmomentumJ. Theanalysishascon- of 4n self-conjugate nuclei in terms of T=0 quartets of cerned the whole isobaric chain of A = 24 nuclei, there- lowangularmomenta(J=0,2,4)whichhasemergedfrom fore ranging from even-evento odd-odd nuclei as well as thepresentanalysisexhibitsastrikinganalogywiththat fromself-conjugatenucleitonucleiwithonlyneutronsin of nuclear collective spectra in a formalism of S (J=0), 5 AcknowledgmentsThisworkwassupportedbytheRo- manianMinistryofEducationandResearchthroughthe grant Idei nr 57. 92Pd 46 46 4 + V)3 6++ 685+_4_ 685+++_4_ [[21]] AKPr..oTIgko.ehTdsaah,keoiT,rH..P.MhHayorsru.imuScuohrpii,p,PlR..5.S2Tc,ha1umc(ka1g,9aa7kn2id),.Gan.dRoHp.kTe,aPnahkyas., Me2 4+ 4+ 44+ Rev. Lett.87, 192501 (2001). ( [3] B.H.FlowersandM.Vujicic,Nucl.Phys.49,586(1963). E 1 2+ 2+ 2+ [4] A. Arima and V. Gillet, Ann.of Phys. 66, 117 (1971). [5] J. Eichler and M. Yamamura, Nucl. Phys. A 182, 33 0 0+ 0+ 0+ (1972). EXP QM H-B [6] M. Hasegawa, S. Tazaki, and R. Okamoto, Nucl. Phys. A592, 45 (1995). [7] J. Dobes and S. Pittel, Phys. Rev.C 57, 688 (1998). [8] R. A. Senk’ov and V. Zelevinsky, Phys. At. Nucl. 74, 1267 (2011). [9] N. Sandulescu, D. Negrea, J. Dukelsky, C. W. Johnson, Phys. Rev. C 85,061303(R) (2012); N. Sandulescu, D. FIG. 4: The low-energy yrast spectrum of 92Pd obtained Negrea, C. W. Johnson, Phys. Rev. C 86, 041302 (R) in the QM approach compared to the experimental data [16] (2012); D. Negrea and N. Sandulescu, Phys. Rev. C90, and the shell model calculation (H-B)of Ref. [17]. 024322 (2014). [10] M. Sambataro and N. Sandulescu, Phys. Rev. C 88, 061303(R) (2013). [11] M.Sambataro,N.Sandulescu,andC.W.Johnson,Phys. D (J=2) and G (J=4) pairs (e.g., see Ref.[19]; for a Lett. B740, 137 (2015). more general shell-model like formalism based on collec- [12] B.A.BrownandW.A.Richter,Phys.Rev.C74,034315 tive pairsseeRef. [18]). Suchananalogyencouragesthe (2006). [13] www.nscl.msu.edu/ brown/resources/resources.html. extensiontoquartetsofbosonmappingtechniquesdevel- [14] M.SambataroandN.Sandulescu,J.Phys.G:Nucl.Part. oped for a microscopic analysis of the Interacting Boson Phys. 40, 055107 (2013). Model (IBM) [20]. Thus, if the s (J =0) and d (J = 2) [15] I.P.JohnstoneandL.D.Skouras,Eur.Phys.J.A11,125 IBMbosonsareinterpretedastheimagesof,respectively, (2001). the T = 0, J = 0 and T = 0, J = 2 quartets, and to [16] B. Cederval et al, Nature469, 68 (2011). the extent that the description of the fermionic Hamil- [17] H.HerndlandB.A.Brown,Nucl.Phys.A627,35(1997). tonian in the space of these quartets can be transferred [18] R. J. Liotta and C. Pomar, Nucl. Phys. A 362, 137 (1981). ontothatofatwo-bodyhermitiansdbosonHamiltonian, [19] F. Catara, A. Insolia, M. Sambataro, E. Maglione, and with its parameters eventually absorbing the contribu- A. Vitturi, Phys.Rev.C32, 634 (1985). tion of other T = 0 quartets (if any), then the use of [20] F. Iachello and A. Arima, The Interacting Boson Model IBM-type Hamiltonians for the treatment of even-even (Cambridge University Press, 1987). self-conjugate nuclei finds a microscopic justification in [21] J. Dukelsky, P. Federman, R. P. J. Perazzo, and H. M. ouranalysis. Toourknowledge,inliteraturethere exists Sofia, Phys.Lett. B 115, 359 (1982). only one (old) example of such an use which was carried out, however,on a pure phenomenological basis [21].

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