ORNL/TM-2001/83 A Stochastic Method for Estimating the Effect of Isotopic Uncertainties in Spent Nuclear Fuel M. D. DeHart DOCUMENT AVAILABILITY Reports produced after January 1, 1996, are generally available free via the U.S. Department of Energy (DOE) Information Bridge. Web site http://www.osti.gov/bridge Reports produced before January 1, 1996, may be purchased by members of the public from the following source. National Technical Information Service 5285 Port Royal Road Springfield, VA 22161 Telephone 703-605-6000 (1-800-553-6847) TDD 703-487-4639 Fax 703-605-6900 E-mail [email protected] Web site http://www.ntis.gov/support/ordernowabout.htm Reports are available to DOE employees, DOE contractors, Energy Technology Data Exchange (ETDE) representatives, and International Nuclear Information System (INIS) representatives from the following source. Office of Scientific and Technical Information P.O. 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The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States government or any agency thereof. ORNL/TM-2001/83 Computational Physics and Engineering Division (10) A Stochastic Method for Estimating the Effect of Isotopic Uncertainties in Spent Nuclear Fuel M. D. DeHart Oak Ridge National Laboratory, P.O. Box 2008, Oak Ridge, TN 37831-6370 Date Published: September 2001 Prepared by the OAK RIDGE NATIONAL LABORATORY Oak Ridge, Tennessee 37831 managed and operated by UT-Battelle, LLC for the U.S. DEPARTMENT OF ENERGY under contract DE-AC05-00OR22725 CONTENTS LIST OF FIGURES.......................................................................................................................v LIST OF TABLES......................................................................................................................vii ACKNOWLEDGMENTS............................................................................................................ix ABSTRACT.................................................................................................................................xi 1. INTRODUCTION................................................................................................................1 2. STATISTICAL BACKGROUND........................................................................................3 3. APPROACH........................................................................................................................7 4. PARALLEL PROCESSING..............................................................................................11 5. RESULTS...........................................................................................................................13 5.1. Convergence..............................................................................................................17 5.2. Distribution of Eigenvalues.......................................................................................19 5.3. Actinide-Only vs. “Full” Burnup Credit...................................................................23 5.4. Conservatism of Bounding Approach.......................................................................26 6. CONCLUSIONS................................................................................................................31 7. REFERENCES...................................................................................................................33 APPENDIX A.............................................................................................................................35 KRONOS Fortran-90 Program Listing..............................................................................37 APPENDIX B: SAMPLE BASELINE INPUT MODELS USED BY KRONOS.....................53 Sample 1: KRONOS KENO Cask model, non-uniform axial profile, actinides only, 20 GWd/MTU..................................................................................................55 Sample 2: KRONOS KENO pin model, non-uniform axial profile, actinides + fission products, 40 GWd/MTU..................................................................................63 iii Sample 3: KRONOS XSDRN pin-cell model, actinides + fission products, 60 GWd/MTU .............................................................................................72 iv LIST OF FIGURES Figure Page 1. Convergence of mean value of k for 60 GWd/MTU cask models...........................................18 2. Convergence of population standard deviation for 60 GWd/MTU cask models.....................19 3. Distribution of k values for Case 1, 20 GWd/MTU.................................................................20 4. Distribution of k values for Case 2, 40 GWd/MTU.................................................................21 5. Distribution of k values for Case 3, 60 GWd/MTU.................................................................22 6. Fission product reactivity worth as a function of burnup.........................................................25 7. Uncertainty due to fission products as a function of burnup....................................................26 8. Probability plot for KENO cask calculations, actinides + fission products.............................27 9. Probability plot for KENO cask calculations, actinides only...................................................28 v vi LIST OF TABLES Table Page 1. Validation results used in uncertainty analyses..........................................................................8 2. Results of KRONOS calculations for various configurations and burnups.............................14 3. Reactivity worth of fission products and associated uncertainties...........................................24 vii viii