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Encyclopedia of Physical Science and Technology - Classical Physics PDF

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P1: FYK Revised Pages Qu: 00, 00, 00, 00 Encyclopedia of Physical Science and Technology EN001-05 May 25, 2001 16:7 Acoustic Chaos Werner Lauterborn Universita¨t Go¨ttingen I. The Problem of Acoustic Cavitation Noise II. The Period-Doubling Noise Sequence III. A Fractal Noise Attractor IV. Lyapunov Analysis V. Period-Doubling Bubble Oscillations VI. Theory of Driven Bubbles VII. Other Systems VIII. Philosophical Implications GLOSSARY a dynamic system. A point in phase space characterizes a specific state of the system. Bifurcation Qualitative change in the behavior of a sys- Strange attractor In dissipative systems, the motion tem, when a parameter (temperature, pressure, etc.) is tends to certain limits forms (attractors). When the mo- altered (e.g., period-doubling bifurcation); related to tion comes to rest, this attractor is called a fixed point. phase change in thermodynamics. Chaotic motions run on a strange attractor, which has Cavitation Rupture of liquids when subject to tension ei- involved properties (e.g., a fractal dimension). ther in flow fields (hydraulic cavitation) or by an acous- tic wave (acoustic cavitation). Chaos Behavior (motion) with all signs of statistics de- THE PAST FEW years have seen a remarkable develop- spite an underlying deterministic law (often, determin- ment in physics, which may be described as the upsurge istic chaos). of “chaos.” Chaos is a term scientists have adapted from Fractal Object (set of points) that does not have a smooth common language to describe the motion or behavior of structure with an integer dimension (e.g., three dimen- a system (physical or biological) that, although governed sional). Instead, a fractal (noninteger) dimension must by an underlying deterministic law, is irregular and, in the be ascribed to them. long term, unpredictable. Period doubling Special way of obtaining chaotic (irreg- Chaotic motion seems to appear in any sufficiently ular) motion; the period of a periodic motion doubles complex dynamical system. Acoustics, that part of repeatedly until in the limit of infinite doubling aperi- physics that descibes the vibration of usually larger en- odic motion is obtained. sembles of molecules in gases, liquids, and solids, makes Phase space Space spanned by the dependent variables of no exception. As a main necessary ingredient of chaotic 117 P1: FYK Revised Pages Encyclopedia of Physical Science and Technology EN001-05 May 8, 2001 14:48 118 Acoustic Chaos dynamics is nonlinearity, acoustic chaos is closely related to ask what physical mechanisms are known to convert a to nonlinear oscillations and waves in gases, liquids, single frequency to a broadband spectrum? This could not and solids. It is the science of never-repeating sound be answered before chaos theory was developed. However, waves. This property it shares with noise, a term having although chaos theory is now well established, a physical its origin in acoustics and formerly attributed to every (intuitive) understanding is still lacking. sound signal with a broadband Fourier spectrum. But Fourier analysis is especially adapted to linear oscillatory systems. The standard interpretation of the lines in a II. THE PERIOD-DOUBLING Fourier spectrum is that each line corresponds to a (linear) NOISE SEQUENCE mode of vibration and a degree of freedom of the system. However, as examples from chaos physics show, a broad- To investigate the sound emission from acoustic cavita- band spectrum can already be obtained with just three tion the experimental arrangement as depicted in Fig. 1 (nonlinear) degrees of freedom (that is, three dependent is used. To irradiate the liquid (water) a piezoceramic variables). Chaos physics thus develops a totally new cylinder (PZT-4) of 76-mm length, 76-mm inner diameter, view of the noise problem. It is a deterministic view, and 5-mm wall thickness is used. When driven at its main but it is still an open question how far the new approach resonance, 23.56 kHz, a high-intensity acoustic field is will reach in explaining still unsolved noise problems generated in the interior and cavitation is easily achieved. (e.g., the 1/ f -noise spectrum encountered so often). The The noise is picked up by a broadband hydrophone and detailed relationship between chaos and noise is still an digitized at rates up to 60 MHz after suitable lowpass area of active research. An example, where the properties filtering (for correct analog-to-digital conversion for later of acoustic noise could be related to chaotic dynamics, is processing) and strong filtering of the driving frequency, given below for the case of acoustic cavitation noise. which would otherwise dominate the noise output. The Acoustic chaos appears in an experiment when a liq- experiment is fully computer controlled. The amplitude of uid is irradiated with sound of high intensity. The liquid the driving sound field can be made an arbitrary function then ruptures to form bubbles or cavities (almost empty of time via a programmable synthesizer. In most cases, bubbles). The phenomenon is known as acoustic cavita- linear ramp functions are applied to study the buildup of tion and is accompanied by intense noise emission—the noise when the driving pressure amplitude in the liquid is acoustic cavitation noise. It has its origin in the bubbles set increased. into oscillation in the sound field. Bubbles are nonlinear From the data stored in the memory of the transient oscillators, and it can be shown both experimentally and recorder, power spectra are calculated via the fast-Fourier- theoretically that they exhibit chaotic oscillations after a transform algorithm from usually 4096 samples out of the series of period doublings. The acoustic emission from 128 × 1024 samples stored. This yields about 1000 short- these bubbles is then a chaotic sound wave (i.e., irregular time spectra when the 4096 samples are shifted by 128 and never repeats). This is acoustic chaos. samples from one spectrum to the next. Figure 2 shows four power spectra from one such experiment. Each diagram gives the excitation level at I. THE PROBLEM OF ACOUSTIC CAVITATION NOISE The projection of high-intensity sound into liquids has been investigated since the application of sound to locate objects under water became used. It was soon noticed that at too high an intensity the liquid may rupture, giving rise to acoustic cavitation. This phenomenon is accompanied by broadband noise emission, which is detrimental to the useful operation of, for instance, a sonar device. The noise emission presents an interesting physical problem that may be formulated in the following way. A sound wave of a single frequency (a pure tone) is trans- formed into a broadband sound spectrum, consisting of an (almost) infinite number of neighboring frequencies. What is the physical mechanism that causes this transfor- FIGURE 1 Experimental arrangement for measurements on mation? The question may even be shifted in its emphasis acoustic cavitation noise (chaotic sound). P1: FYK Revised Pages Encyclopedia of Physical Science and Technology EN001-05 May 8, 2001 14:48 Acoustic Chaos 119 FIGURE 2 Power spectra of acoustic cavitation noise at different excitation levels (related to the pressure amplitudes of the driving sound wave). (From Lauterborn, W. (1986). Phys. Today 39, S-4.) the transducer in volts, the time since the experiment systems has been found to show period doubling, among (irradiating the liquid with a linear ramp of increasing them driven nonlinear oscillators. A peculiar feature excitation) has started in milliseconds, and the power of the period-doubling bifurcation is that it occurs in spectrum at this time. At the beginning of the experiment, sequences; that is, when one period-doubling bifurcation at low sound intensity, only the driving frequency f0 shows has occurred, it is likely that further period doubling will up. In the upper left diagram of Fig. 2 the third harmonic, occur upon altering a parameter of the system, and so on, 3 f0, is present. When comparing both lines it should often in an infinite series. Acoustic cavitation has been one be remembered that the driving frequency is strongly of the first experimental examples known to exhibit this damped by filtering. In the lower left-hand diagram, many series. In Fig. 2, the upper right-hand diagram shows the 1 more lines are present. Of special interest is the spectral noise spectrum after further period doubling to f0. The 4 1 1 1 line at 2 f0 (and their harmonics). A well-known feature of doubling sequence can be observed via 8 f0 and 16 f0 up 1 nonlinear systems is that they produce higher harmonics. to f 0 (not shown here). It is obvious that the spectrum is 32 Not yet widely known is that subharmonics can also be rapidly “filled” with lines and gets more and more dense. produced by some nonlinear systems. These then seem The limit of the infinite series yields an aperiodic motion, to spontaneously divide the applied frequency f0 to a densely packed power spectrum (not homogeneously), yield, for example, exactly half that frequency (or exactly that is, broadband noise (but characteristically colored by one-third). This phenomenon has become known as a lines). One such noise spectrum is shown in Fig. 2 (lower period-doubling (-tripling) bifurcation. A large class of right-hand diagram). Thus, at least one way of turning P1: FYK Revised Pages Encyclopedia of Physical Science and Technology EN001-05 May 8, 2001 14:48 120 Acoustic Chaos a pure tone into broadband noise has been found—via successive period doubling. This finding has a deeper implication. If a system be- comes aperiodic through the phenomenon of repeated pe- riod doubling, then this is a strong indication that the ir- regularity attained in this way is of simple deterministic origin. This implies that acoustic cavitation noise is not a basically statistical phenomenon but a deterministic one. It also implies that a description of the system with usual sta- tistical means may not be appropriate and that a successful description by some deterministic theory may be feasible. III. A FRACTAL NOISE ATTRACTOR In Section II the sound signal has been treated by Fourier analysis. Fourier analysis is a decomposition of a signal into a sum of simple waves (normal modes) and is said to give the degrees of freedom of the described system. Chaos theory shows that this interpretation must be abandoned. Broadband noise, for instance, is usually thought to be due to a high (nearly infinite) number of degrees of freedom that superposed yield noise. Chaotic systems, however, have the ability to produce noise with only a few (nonlin- ear) degrees of freedom, that is, with only a few dependent variables. Also, it has been found that continuous systems FIGURE 3 Strange attractor of acoustic cavitation noise obtained with only three dependent variables are capable of chaotic by phase–space analysis of experimental data (a time series of pressure values sampled at 1 MHz). The attractor is rotated to motions and thus, producing noise. Chaos theory has de- visualize its three-dimensional structure. (Courtesy of J. Holzfuss. veloped new methods to cope with this problem. One of From Lauterborn, W. (1986). In “Frontiers in Physical Acoustics” these is phase-space analysis, which in conjunction with (D. Sette, ed.), pp. 124–144, North Holland, Amsterdam.) fractal dimension estimation is capable of yielding the in- trinsic degrees of freedom of the system. This method has been applied to inspect acoustic cavitation noise. The an- object. This suggests that the dynamical system produc- swer it may give is the dimension of the dynamical system ing the noise has only a few nonlinear degrees of freedom. producing acoustic cavitation noise. See SERIES. The flat appearance of the attractor in a three-dimensional The sampled noise data are first used to construct a phase space (Fig. 3) suggests that only three essential de- noise attractor in a suitable phase space. Then the (frac- grees are needed for the system. This is confirmed by a tal) dimension of the attractor is determined. The pro- fractal dimension analysis, which yields a dimension of cedure to construct an attractor in a space of chosen di- d = 2.5 for this attractor. Unfortunately, a method has not mension n simply consists in combining n samples (not yet been conceived of how to construct the equations of necessarily consecutive ones) to an n-tuple, whose en- motion from the data. tries are interpreted as the coordinate values of a point in n-dimensional Euclidian space. An example of a noise at- tractor constructed in this way is given in Fig. 3. The attrac- IV. LYAPUNOV ANALYSIS tor has been obtained from a time series of pressure values {p(kts); t = 1, . . . , 4096; ts = 1 µsec} taken at a sampling Chaotic systems exhibit what is called sensitive depen- frequency of fs = 1/ts = 1 MHz by forming the three- dence on initial conditions. This expression has been intro- tuples [p(kts), p(kts + T ), p(kts + 2T )], k = 1, . . . , 4086, duced to denote the property of a chaotic system that small with T = 5 µsec. The frequency of the driving sound field differences in the initial conditions, however small, are has been 23.56 kHz. The attractor in Fig. 3 is shown from persistently magnified because of the dynamics of the sys- different views to demonstrate its nearly flat structure. It is tem. This property is captured mathematically by the no- most remarkable that not an unstructured cluster of points tion of Lyapunov exponents and Lyapunov spectra. Their is obtained as is expected for noise, but a quite well-defined definition can be illustrated by the deformation of a small P1: FYK Revised Pages Encyclopedia of Physical Science and Technology EN001-05 May 8, 2001 14:48 Acoustic Chaos 121 In dissipative systems, the final motion takes place on attractors. Besides the fractal dimension, as discussed in the previous section, the Lyapunov spectrum may serve to characterize these attractors. When at least one Lyapunov exponent is greater than zero, the attractor is said to be chaotic. Progress in the field of nonlinear dynamics has made possible the calculation of the Lyapunov spectrum from a time series. It could be shown that acoustic cavita- tion in the region of broadband noise emission is charac- FIGURE 4 Idea for defining Lyapunov exponents. A small sphere terized by one positive Lyapunov exponent. in phase space is deformed to an ellipsoid, indicating expansion or contraction of neighboring trajectories. V. PERIOD-DOUBLING BUBBLE sphere of initial conditions along a fiducial trajectory (see OSCILLATIONS Fig. 4). The expansion or contraction is used to define the Lyapunov exponents λi , i = 1, 2, . . . , m, where m is the Thus far, only the acoustic signal has been investigated. dimension of the phase space of the system. When, on the An optic inspection of the liquid inside the piezoelectric average, for example, r1(t) is larger than r1(0), then λ1 > 0 cylinder (see Fig. 1) reveals that a highly structured cloud and there is a persistent magnification in the system. The of bubbles or cavities is present (Fig. 5) oscillating and set {λi , i = 1, . . . , m}, whereby the λi usually are ordered moving in the sound field. It is obviously these bubbles λ1 ≥ λ2 ≥ · · · ≥ λm, is called the Lyapunov spectrum. that produce the noise. If this is the case, the bubbles must FIGURE 5 Acoustic cavitation bubble field in water inside a cylin- FIGURE 6 Reconstructed images from (a) a holographic series drical piezoelectric transducer of about 7 cm in diameter. Two taken at 23.100 holograms per second of bubbles inside a piezo- planes in depth are shown about 5 mm apart. The pictures are ob- electric cylinder driven at 23.100 Hz and (b) the corresponding tained by photographs from the reconstructed three-dimensional power spectrum of the noise emitted. Two period-doublings have image of a hologram taken with a ruby laser. taken place. P1: FYK Revised Pages Encyclopedia of Physical Science and Technology EN001-05 May 8, 2001 14:48 122 Acoustic Chaos FIGURE 7 Period-doubling route to chaos for a driven bubble oscillator. Left column: radius-time solution curves; middle left column: trajectories in phase space; middle right column: Poincare´ section plots: right column: power spectra. Rn is the radius of the bubble at rest, Ps and v are the pressure amplitude and frequency of the driving sound field, respectively. (From Lauterborn, W., and Parlitz, U. (1988). J. Acoust. Soc. Am. 84, 1975.) P1: FYK Revised Pages Encyclopedia of Physical Science and Technology EN001-05 May 8, 2001 14:48 Acoustic Chaos 123 FIGURE 7 (Continued ) P1: FYK Revised Pages Encyclopedia of Physical Science and Technology EN001-05 May 8, 2001 14:48 124 Acoustic Chaos move chaotically and should show the period-doubling The third column shows so-called Poincare´ section plots. sequence encountered in the noise output. This has been Here, only the dots after the lapse of one full period of confirmed by holographic investigations where once per the driving sound field are plotted in the radius–velocity period of the driving sound field a hologram of the bub- plane of the bubble motion. Period doubling is seen most ble field has been taken. Holograms have been taken be- easily here and also the evolution of a strange (or chaotic) cause the bubbles move in three dimensions, and it is attractor. The rightmost column gives the power spectra difficult to photograph them at high resolution when an of the radial bubble motion. The filling of the spectrum extended depth of view is needed. In one experiment the with successive lines in between the old lines is evident, driving frequency was 23,100 Hz, which means 23,100 as is the ultimate filling when the chaotic motion is holograms per second have been taken. The total num- reached. ber of holograms, however, was limited to a few hundred. A compact way to show the period-doubling route to Figure 6a gives an example of a series of photographs chaos is by plotting the radius of the bubble as a func- taken from a holographic series. In this case, two period- tion of a parameter of the system that can be varied, e.g., doubling bifurcations have already taken place since the the frequency of the driving sound field. Figure 8a gives oscillations only repeat after four cycles of the driving an example for a bubble of radius at rest of Rn = 10 µm, sound wave. The first period doubling is strongly visible; driven by a sound field of frequency ν between 390 kHz the second one can only be seen by careful inspection. and 510 kHz at a pressure amplitude of Ps = 290 kPa. Figure 6b gives the noise power spectrum taken simulta- The period-doubling cascade to chaos is clearly visible. neously with the holograms. The acoustic measurements In the chaotic region, “windows” of periodicity show show both period doublings more clearly than the optical 1 measurement (documented in Fig. 6a) as the 4 f0 ( f0 = 23.1 kHz) spectral line is strongly present together with its harmonics. VI. THEORY OF DRIVEN BUBBLES A theory has not yet been developed that can account for the dynamics of a bubble field as shown in Fig. 5. The most advanced theory is only able to describe the motion of a single spherical bubble in a sound field. Even with suitable neglections the model is a highly nonlinear ordinary differential equation of second order for the radius R of the bubble as a function of time. With a sinusoidal driving term (sound wave) the phase space is three dimensional, just sufficient for a dynamical system to show irregular (chaotic) motion. The model is an example of a driven nonlinear oscillator for which chaotic solutions in certain parameter regions are by now standard. However, period doubling and irregular motion were found in the late 1960s in numerical calculations when chaos theory was not yet available and thus the interpretation of the results difficult. The surprising fact is that already this simple model of a purely spherically oscillating bubble set into oscillation by a sound wave yields successive period doubling up to chaotic oscillations. Figure 7 demonstrates the period- doubling route to chaos in four ways. The leftmost column gives the radius of the bubble in the sound field as a func- tion of time, where the dot on the curve indicates the lapse of a full period of the driving sound field. The next column FIGURE 8 (a) A period-doubling cascade as seen in the bifurca- shows the corresponding trajectories in the plane spanned tion diagram. (b) The corresponding largest Lyapunov exponent by the radius of the bubble and its velocity. The dots again λ max. (c) The winding number w. (From Parlitz, U. et al. (1990). mark the lapse of a full period of the driving sound field. J. Acoust. Soc. Am. 88, 1061.) P1: FYK Revised Pages Encyclopedia of Physical Science and Technology EN001-05 May 8, 2001 14:48 Acoustic Chaos 125 up as regularly experienced with other chaotic systems. VII. OTHER SYSTEMS In Fig. 8b the largest Lyapunov exponent λmax is plot- ted. It is seen that λmax > 0 when the chaotic region is Are there other systems in acoustics with chaotic dynam- reached. Figure 8c gives a further characterization of the ics? The answer is surely yes, although the subtleties of system by the winding number w. The winding number chaotic dynamics make it difficult to easily locate them. describes the winding of a neighboring trajectory around When looking for chaotic acoustic systems, the ques- the given one per period of the bubble oscillation. It can tion arises as to what ingredients an oscillatory system, as be seen that this quantity changes quite regularly in the an acoustic one, must possess to be susceptible to chaos. period-doubling sequence, and rules can be given for this The full answer is not yet known, but some understanding change. is emerging. A necessary, but unfortunately not sufficient, The driven bubble system shows resonances at vari- ingredient is nonlinearity. Next, period doubling is known ous frequencies that can be labeled by the ratio of the to be a precursor of chaos. It is a peculiar fact that, when linear resonance frequency of the bubble to the driving one period doubling has occurred, another one is likely to frequency of the sound wave. Figure 9 gives an example appear, and indeed a whole series with slight alterations of of the complicated response characteristic of a driven bub- parameters. Further, the appearance of oscillations when ble. At somewhat higher driving than given in the figure a parameter is altered points to an intrinsic instability of a the oscillations start to become chaotic. A chaotic bubble system and thus to the possibility of becoming a chaotic attractor is shown in Fig. 10. To better reveal its structure, one. After all, two distinct classes can be formulated: (1) it is not the total trajectory that is plotted but only the periodically driven passive nonlinear systems (oscillators) points in the velocity–radius plane of the bubble wall at a and (2) self-excited systems (oscillators). Passive means fixed phase of the driving. These points hop around on the that in the absence of any external driving the system attractor in an irregular fashion. These chaotic bubble os- stays at rest as, for instance, a pendulum does. But a cillations must be considered as the source of the chaotic pendulum has the potential to oscillate chaotically when sound output observed in acoustic cavitation. being driven periodically, for instance by a sinusoidally FIGURE 9 Frequency response curves (resonance curves) for a bubble in water with a radius at rest of Rn = 10 µm for different sound pressure amplitudes pA of 0.4, 0.5, 0.6, 0.7, and 0.8 bar. (From Lauterborn, W. (1976). J. Acoust. Soc. Am. 59, 283.) P1: FYK Revised Pages Encyclopedia of Physical Science and Technology EN001-05 May 8, 2001 14:48 126 Acoustic Chaos as it is a three-dimensional (space), nonlinear, dynamical (time) system; that is, it requires three space coordinates and one time coordinate to be followed. This is at the border of present-day technology both numerically and experimentally. The latest measurements have singled out mode competition as the mechanism underlying the com- plex dynamics. Figure 11 gives two examples of oscilla- tory patterns: a periodic hexagonal structure (Fig. 11a) and a FIGURE 10 A numerically calculated strange bubble attractor (Ps = 300 kPa, v = 600 kHz). (Courtesy of U. Parlitz.) varying torque. This is easily shown experimentally by the repeated period doubling that soon appears at higher periodic driving. Self-excited systems develop sustained oscillations from seemingly constant exterior conditions. One example is the Rayleigh-Be´nard convection, where a liquid layer is heated from below in a gravitational field. The system goes chaotic at a high enough temperature difference between the bottom and surface of the liquid layer. Self-excited systems may also be driven, giving an important subclass of this type. The simplest model in this class is the driven van der Pol oscillator. A real physical system of this category is the weather (the atmosphere). It is periodically driven by solar radiation with the low period of 24 hr, and it is a self-excited system, as already constant heating by the sun may lead to b Rayleigh-Be´nard convection as observed on a faster time scale. The first reported period-doubled oscillation from a pe- riodically driven passive system dates back to Faraday in 1831. Starting with the investigation of sound-emitting, vi- brating surfaces with the help of Chladni figures, Faraday used water instead of sand, resulting in vibrating a layer of liquid vertically. He was very astonished about the re- sult: regular spatial patterns of a different kinds appeared and, above all, these patterns were oscillating at half the frequency of the vertical motion of the plate. Photography was not yet invented to catch the motion, but Faraday may well have seen chaotic motion without knowing it. It is in- teresting to note that there is a connection to the oscillation of bubbles as considered before. Besides purely spherical oscillations, bubbles are susceptible to surface oscillations as are drops of liquid. The Faraday case of a vibrating flat surface of a liquid may be considered as the limiting case of either a bubble of larger and larger size or a drop of FIGURE 11 Two patterns appearing on the surface of a liq- larger and larger size, when the surface is bent around up uid layer vibrated vertically in a cylindrical container: (a) regular or down. Today, the Faraday patterns and Faraday oscil- hexagonal pattern at low amplitude, and (b) pattern when ap- lations can be observed better, albeit still with difficulties proaching chaotic vibration. (Courtesy of Ch. Merkwirth.)

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