COHERENCE AND ULTRASHORT PULSE LASER EMISSION Edited by Dr. F. J. Duarte Coherence and Ultrashort Pulse Laser Emission Edited by Dr. F. J. Duarte Published by InTech Janeza Trdine 9, 51000 Rijeka, Croatia Copyright © 2010 InTech All chapters are Open Access articles distributed under the Creative Commons Non Commercial Share Alike Attribution 3.0 license, which permits to copy, distribute, transmit, and adapt the work in any medium, so long as the original work is properly cited. After this work has been published by InTech, authors have the right to republish it, in whole or part, in any publication of which they are the author, and to make other personal use of the work. Any republication, referencing or personal use of the work must explicitly identify the original source. Statements and opinions expressed in the chapters are these of the individual contributors and not necessarily those of the editors or publisher. No responsibility is accepted for the accuracy of information contained in the published articles. The publisher assumes no responsibility for any damage or injury to persons or property arising out of the use of any materials, instructions, methods or ideas contained in the book. Publishing Process Manager Jelena Marusic Technical Editor Teodora Smiljanic Cover Designer Martina Sirotic Image Copyright Kostyantyn Ivanyshen, 2010. Used under license from Shutterstock.com First published December, 2010 Printed in India A free online edition of this book is available at www.intechopen.com Additional hard copies can be obtained from [email protected] Coherence and Ultrashort Pulse Laser Emission, Edited by Dr. F. J. Duarte p. cm. ISBN 978-953-307-242-5 free online editions of InTech Books and Journals can be found at www.intechopen.com Contents Preface IX Part 1 Coherence and Quantum Phenomena 1 Chapter 1 Electrically-Pumped Organic-Semiconductor Coherent Emission: A Review 3 F. J. Duarte Chapter 2 Coherence of XUV Laser Sources 23 Sebastian Roling and Helmut Zacharias Chapter 3 Laser Technology for Compact, Narrow-bandwidth Gamma-ray Sources 49 Miroslav Shverdin, Felicie Albert, David Gibson, Mike Messerly, Fred Hartemann, Craig Siders, Chris Barty Chapter 4 Quantum Manipulations of Single Trapped-Ions Beyond the Lamb-Dicke Limit 75 M. Zhang and L. F.Wei Chapter 5 Coherent Optical Phonons in Bismuth Crystal 95 Davide Boschetto and Antoine Rousse Chapter 6 Quantum Interference Signal from an Inhomogeneously Broadened System Excited by an Optically Phase-Controlled Laser-Pulse Pair 115 Shin-ichiro Sato and Takayuki Kiba Chapter 7 Quantum Control of Laser-driven Chiral Molecular Motors 133 Masahiro Yamaki, Sheng H. Lin, Kunihiko Hoki and Yuichi Fujimura Chapter 8 Energy Approach to Atoms in a Laser Field and Quantum Dynamics with Laser Pulses of Different Shape 159 Alexander V. Glushkov, Ol’ga Yu. Khetselius, Andrey A. Svinarenko and George P. Prepelitsa VI Contents Part 2 Ultrashort Laser Pulse Emission and Applications 187 Chapter 9 Second Harmonic Generation under Strong Influence of Dispersion and Cubic Nonlinearity Effects 189 Sergey Mironov, Vladimir Lozhkarev, Vladislav Ginzburg, Ivan Yakovlev, Grigory Luchinin, Efim Khazanov, Alexander Sergeev, and Gerard Mourou Chapter 10 Temporal Stretching of Short Pulses 205 Rajeev Khare and Paritosh K. Shukla Chapter 11 Ultrafast Laser Pulse Synchronization 227 Heping Zeng, Ming Yan and Wenxue Li Chapter 12 Carrier-Envelope Phase Stabilization of Grating Based High-Power Ultrafast Laser 261 Shouyuan Chen, Yi Wu, Kun Zhao and Zenghu Chang Chapter 13 The Generation and Characterisation of Ultrashort Mid-Infrared Pulses 281 J. Biegert, P.K.Bates and O.Chalus Chapter 14 Contrast Improvement of Relativistic Few-Cycle Light Pulses 305 Lsázló Veisz Chapter 15 Modeling the Interaction of a Single-Cycle Laser Pulse With a Bound Electron Without Ionization 331 Ufuk Parali and Dennis R. Alexander Chapter 16 Ultrashort, Strongly Focused Laser Pulses in Free Space 355 Alexandre April Chapter 17 Interaction of Short Laser Pulses with Gases and Ionized Gases 383 Stephan Wieneke, Stephan Brückner and Wolfgang Viöl Chapter 18 Characterisation and Manipulation of Proton Beams Accelerated by Ultra-Short and High-Contrast Laser Pulses 403 Sargis Ter-Avetisyan, Mathias Schnürer and Peter V Nickles Chapter 19 Picosecond Laser Pulse Distortion by Propagation through a Turbulent Atmosphere 435 Josef Blazej, Ivan Prochazka and Lukas Kral Contents VII Chapter 20 Comparison between Finite-Difference Time-Domain Method and Experimental Results for Femtosecond Laser Pulse Propagation 449 Shinki Nakamura Chapter 21 Non Perturbative Time-Dependent Density Functional Theory, TDDFT: Study of Ionization and Harmonic Generation in Linear Di-(N ) and Tri-(CO , OCS, CS ) 2 2 2 Atomic Molecules with Ultrashort Intense Laser Pulses-Orientational Effects 493 Emmanuel Penka Fowe and André Dieter Bandrauk Chapter 22 Femtosecond Fabrication of Waveguides in Ion-Doped Laser Crystals 519 Andrey Okhrimchuk Chapter 23 Heat Absorption, Transport and Phase Transformation in Noble Metals Excited by Femtosecond Laser Pulses 543 Wai-Lun Chan and Robert S. Averback Chapter 24 Probing Ultrafast Dynamics of Polarization Clusters in BaTiO by Pulsed Soft X-Ray Laser Speckle Technique 561 3 Kai Ji and Keiichiro Nasu Chapter 25 Two-Photon Polymerization of Inorganic-Organic Hybrid Polymers as Scalable Technology Using Ultra-Short Laser Pulses 583 Houbertz, Ruth, Steenhusen, Sönke, Stichel, Thomas, and Sextl, Gerhard Chapter 26 Several Diffractive Optical Elements Fabricated by Femtosecond Laser Pulses Writing Directly 609 Zhongyi Guo, Lingling Ran, Shiliang Qu and Shutian Liu Chapter 27 Sub-Wavelength Patterning of Self-Assembled Organic Monolayers via Nonlinear Processing with Femtosecond Laser Pulses 629 Nils Hartmann Chapter 28 Applications of Short Laser Pulses 645 S. Mehdi Sharifi and Abdossamad Talebpour Chapter 29 Ultrashort Laser Pulses Applications 663 Ricardo Elgul Samad, Lilia Coronato Courrol, Sonia Licia Baldochi and Nilson Dias Vieira Junior Preface In an optimized pulsed laser source, the coherence of its emission (or linewidth) is intimately related to the duration of the emission pulse, by one of the most beautiful expressions of quantum optics ΔνΔt ≈ 1 which is an alternative version of Heisenberg’s uncertainty principle ΔpΔx ≈ h In this volume, recent contributions on coherence provide a useful perspective on the diversity of various coherent sources of emission and coherent related phenomena of current interest. These papers provide a preamble for a larger collection of contribu- tions on ultrashort pulse laser generation and ultrashort pulse laser phenomena. Pa- pers on ultrashort pulse phenomena include works on few cycle pulses, high-power generation, propagation in various media, and a variety of applications of current in- terest. Undoubtedly, Coherence and Ultrashort Pulse Emission off ers a rich and practical perspective on this rapidly evolving fi eld. F. J. Duarte Rochester New York, USA