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Coherence and Correlation in Atomic Collisions PDF

697 Pages·1980·17.82 MB·English
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Coherence and Correlation in Atomic Collisions PHYSICS OF ATOMS AND MOLECULES Series Editors: P. G. Burke, The Queen's University ofB elfast, Northern Ireland and Daresbury Laboratory, Science Research Council, Warrington, England and H. Kleinpoppen, Institute of Atomic Physic8, University of Stirling, Scotland Editorial Advisory Board: R.B. Bernstein (New York, U.S.A.) W. Hanle (Giessen, Germany) J.C. Cohen-Tannoudji (Paris, France) W.E. Lamb, Jr. (Tucson, U.S.A.) R.W. Crompton (Canbe"a, Australia) P.-O. Lowdin (Gainesville, U.S.A.) J.N. Dodd (Dunedin, New Zealand) M.R.C. McDowell (London,U.K.) G.F. Drukarev (Leningrad, U.S.S.R.) K.Takayanagi(Tokyo,Japan) 1976: ELECTRON AND PHOTON INTERACTIONS WITH ATOMS Edited by H. Kleinpoppen and M.R.C. McDowell 1978: PROGRESS IN ATOMIC SPECTROSCOPY, Parts A and B Edited by W. Hanle and H. Kleinpoppen 1979: ATOM-MOLECULE COLLISION THEORY: A Guide for the Experimentalist Edited by Richard B. Bernstein 1980: COHERENCE AND CORRELATION IN ATOMIC COLLISIONS Edited by H. Kleinpoppen and J.F. Williams 1n preparation: THEORY OF ELECTRON-ATOM COLLISIONS By P.G. Burke and c.J. Joachain VARIATIONAL MEmODS IN ELECTRON-ATOM SCATTERING THEORY By R. K. Nesbet DENSITY MATRIX FORMALISM AND APPLICATIONS IN PHYSICS By K. B. Blum A Continuation Order Plan is available for this series. A continuation order will bring delivery of each new volume immediately upon publication. Volumes are billed only upon actual shipment. For further information please contact the publisher. Coherence and Correlation in Atomic Collisions Edited by H. Kleinpoppen Institute of Atomic Physics University of Stirling Stirling, Scotland and lEWilliams Department ofP ure and Applied Physics Queen's University Belfast, Northern Ireland Plenum Press . New York and London Library of Congress Cataloging in Publication Data Main entry under title: Coherence and correlation in atomic collisions. (physics of atoms and molecules) Includes index. 1. Coherence (Nuclear physics) - Congresses. 2. Angular correlations (Nuclear physics) - Congresses. 3. Collisions (Nuclear physics) - Congresses. I. Klein poppen, Hans. II. Williams, J. F. QC794.6.C58C66 539.7'54 79-15977 ISBN-13: 978-1-4613-2999-2 e-ISBN-13: 978-1-4613-2997-8 DOl: 10.1007/978-1-4613-2997-8 © 1980 Plenum Press, New York A Division of Plenum Publishing Corporation 227 West 17th Street, New York, N.Y. 10011 Softcover reprint of the hardcover 1st edition 1980 All rights reserved No part of this book may be reproduced, stored in a retrieval system, or transmitted, in any form or by any means, electronic, mechanical, photocopying, microfilming, recording, or otherwise, without written permission from the publisher To Sir Harrie Massey, Sec. R.S. GeG9 Suzuki Riddell Aydinol Matsuzawa Sandner McGregor Andersen Ramat Hultberg Hils Koschmieder Eminyan Rubin Malcolm M. Campbell ~~ H. M. M. M. W. 1. N. G. S. D. H. M. K. 1. D. 0~ 86. 87. 88. 89. 90. 91. 92. 93. 94. 95. 96. 97. 98. 99. 00. 1 9 e n ~ n ~~GG@9 e@G) K. Jung A. Ugbabe E. Weigold A. Dixon J. W. van der Water W. Eissner W. Jitschin G. Sinapius G. Stefani F. H. M. Faisal S. Harper K. Taulbjerg S. Hara J. S. Briggs R. Schuch H. F. M. HeidemaG. Nienhuis ege, London. 88 89 G @Q 69. 70. 71. 72. 73. 74. 75. 76. 77. 78. 79. 80. 81. 82. 83. 84. 8i. sity Coll 6 er ge 2 4 gC0g H. A. Schuessler R. J. Celotta M. S. Lubell B. J aduszliwer P. Curry Kocbach L. T. R. Twomey A. Sellin 1. D. Madison E. H. Pederson E. Reichert R. Dang G. F. Hanne U. Heinzmann T. Andersen D; Roy J. van Eck Astronomy, Univ Q 4 )G 52. 53. 54. 55. 56. 57. 58. 59. 60. 61. 62. 63. 64. 65. 66. 67. 68. cs and 9 40 G hysi Joo~@e787€V G (jff<ii) @ 000G) K. H. Schartner 35. R. Helbing 36. K. J. Ross 37. G. C. King 38. J. Comer 39. R. G. Keesing 40. B. Miiller 41. R. Browning 42. A. E. Kingston 43. N. S. Scott 44. 45. A. M. Ermolaev V. Kempter 46. N. H. Tolk 47. J. F. Williams 48. M. R. H. Rudge 49. C. Bottcher 50. S. H. Al-Shamma 51. ographic Unit, Dept. of P i ot f Q Ph ;)ee~G ®@ G3) Q00 H. O. Lutz S. Datz P. Weiss W. R. Newell D. F. Register R. J. Tweed H. G. Berry H. Kleinpoppen J. Delwiche W. Nakel R. Camilloni D. Caldwell N. Malik H. Klar B. Fastrup A. Niehaus R. Morgenstern Photograph by: ;~ 0 8. 9. 0. 1. 2. 3. 4. 5. 6. 7. 8. 9. 0. 1. 2. 3. 4. r 11222222222233333 Q ni Q~ E. Trefftz D. Golden J. W. McConkey K. Blum R. K. Nesbet V. Hertel 1. H. Ehrhardt B. Bederson Sir Harrie Massey E. McCarthy 1. D. H. Jaecks W. Raith J. Kessler U. Fano P. S. Farago F. H. Read A. Giardini-Guido 1. 2. 3. 4. 5. 6. 7. 8. 9. 0. I. 2. 3. 4. 5. 6. 7. 1I111111 The International Workshop on COHERENCE AND CORRELATION IN ATOMIC COLLISIONS was given financial support by Edwards High Vacuum I.B.M. United Kingdom Ltd. Intertechnique Ltd. Ortec Ltd. Plenum Press Spectra-Physics Ltd. University College, London University of Bielefeld University of Stirling Scientific Advisory Committee of the International Workshop P.S. Farago, D. E. Golden, H. Kelinpoppen, J. Macek, I.E. McCarthy, M.R.C. McDowell, W.R. Newell, A. Niehaus, A. Schannann, J.F. Williams Local and Programme Committee of the International Workshop H. Kleinpoppen (Chainnan), H.O. Lutz, I. McGregor, W.R. Newell (Secretary), J.F. Williams Contents Introduction. . . . . . . . . . . . . xiii H. Kleinpoppen and J. F. Williams 1. Theory of (e,2e) Experiments I. E. McCarthy 2. Impulsive (e,2e) Experiments: A Tool to Test Different Ionization Theories and Electronic Structure of Atoms and Molecules . . . . . . . . .. 13 A. Giardini-Guidoni, R. Camilloni, and G. Stefani 3. Low-Energy Electron Impact Ionization with Completely Determined Kinematics 41 H. Ehrhardt, K. Jung, and E. Schubert 4. Coincidence Investigations of Electron-Hydrogen Collisions 59 Erich Weigold 5. Correlation in Multiple Escape near Threshold. 67 H. Klar 6. Interference Effects in the Multiphoton Ionization of Atoms 79 K. C. Mathur 7. Correlation in Electron-Atom Excitation 85 D. E. Golden and N. C. Steph 8. Angular Correlation Parameters for Excitation of the 2'P State of Helium and the 2p State of Atomic Hydrogen . . . . . . . . . . . .. 97 M. T. Hollywood, A. Crowe, and J. F. Williams 9. New Aspects in Electron-Photon Coincidence Experiments 109 H. Kleinpoppen and I. McGregor 10. The Possibility of a Complete Determination of Scattering Amplitudes for S -+ D Excitation by Electron-Photon Coincidence Measurements . 121 Gerard Nienhuis II. Threshold and Pseudothreshold Excitation of Molecules by Electron Impact 133 K. Blum ix x Contents 12. Polarization Correlation Measurements in Ar and HI . 145 J. W. McConkey and 1. C. Malcolm 13. Effect of Optical Potentials on Angular Correlation Parameters 167 D. H. Madison 14. The Calculation of Orientation and Alignment Parameters for the Electron Impact Excitation of the 31P State of He in the First-Order Many-Body Theory. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 179 G. D. Meneses and Gy. Csanak 15. Electron-Photon Correlations in Bremsstrahlung Processes. 187 Werner Nakel 16. Angular Distribution and Polarization of x-Ray Radiation by Electron Impact on Free Atoms . . . . . . . . . . . . . . . . . . . . . . . . . . 205 M. Aydinol, R. Hippler, 1. McGregor, and H. Kleinpoppen 17. Energy Dependence of the Alignment in Inner-Shell Ionization by Electron Impact. . . . . . . . . . . . . . . . . . . . . . . . . . 215 W. Sandner, M. Weber, and W. Mehlhorn 18. Identification of States Excited by Collision: Current State of Theory . . . 223 U. Fano 19. Angular Correlation between Autoionization Electron and Scattered Ion in Slow He+-He Collision. . . . . . . . . . . . . . . . . . . . . . . 229 R. Morgenstern and A. Niehaus 20. Coherence Effects in Postcollision Interactions in Electron Impact Experiments 243 Frank H. Read and John Comer 21. Collision-Stimulated Autoionization 257 V. I. Matveev and E. S. Parilis 22. Electronic Correlation in Electron-Atom Scattering . 269 R. K. Nesbet 23. Observation of the Postcollision Interaction in the Scattered-Electron Spectra of Helium ............... . 271 D. Roy 24. Excitation of Autoionizing States in Noble Gases by Fast Electrons 283 V. V. Balashov, A. N. Grum-Grzhimailo, N. M. Kabachnik, A. 1. Magunov, and S. 1. Strakhova 25. The Postcollision Interaction as a Manifestation of Many-Electron Correlations 297 M. Ya. Amusia, M. Yu. Kuchiev, and S. A. Sheinerman 26. Coincidence Studies of Inner-Shell Excitation in Ion-Atom Collisions 315 H. O. Lutz, N. Luz, S. Sackmann, W. Jitschin, and R. Hippler Contents xi 27. Coherent Production of Positrons in Heavy-Ion Collisions 331 J. Reinhardt, B. Muller, and W. Greiner 28. Alignment of Core-Excited Autoionizing Be+ Projectiles Excited in Single Gas Collisions. . . . . . . . . . . . . . . . . . . . . . . . . 361 P. Bisgaard, R. Bruch, P. Dahl, and M. Rndbro 29. Interference Effects in K-Shell Vacancy Sharing. 369 R. Schuch, G. Nolte, W. Lichtenberg, and H. Schmidt-Bocking 30. Coherent Excitation of Ionic States by Correlated Collisions in a Crystal Lattice 373 S. Datz 31. Alignment, Orientation, and the Beam-Foil Interaction 387 R. M. Schectman, L. J. Curtis, and H. G. Berry 32. Polarized-Photon, Scattered-Ion Coincidence Study of Mg+ Collisions with He, Ne, and Ar ......................... 395 N. Andersen, T. Andersen, C. L. Cocke, and E. Horsdal Pedersen 33. Coherence Effects in Heavy-Ion-Atom Collisions 403 C. Bottcher 34. Excitation of Cd(53P1) and Cd(51P1) in Na+-Cd Collisions: Optical Polarization and Population of Magnetic Sublevels. . . . . . . . . . . . . . . . 413 Vincenzo Aquilanti, Piergiorgio Casavecchia, and Gaia Grossi 35. Spin Polarization in lon-Atom Collisions Studied with Ion Storage Techniques 423 Hans A. Schuessler 36. Scattering Experiments with Laser-Excited Atoms 437 R. Duren 37. Orbital Angular Momentum State Coherence in Charge Transfer to the n = 2 Hydrogen Levels by Fast Protons in Gases . . . . . . . . . . 447 L. Liljeby, S. Mannervik, S. Hultberg, and I. A. Sellin 38. Photon-Scattered Atom Coincidence Study with Vector Polarization Analysis for K-Noble-Gas Collisions . . . . . . . . . . . . . . . . 457 L. Zehnle, E. Clemens, P. J. Martin, W. Schauble, and V. Kempter 39. Alignment and Orientation Measurements in He+-He and He+-H. Collisions 473 D. H. Jaecks, F. Eriksen, and L. Fornari 40. Simultaneous Electron-Photon Excitation of Atoms ........... 479 F. H. M. Faisal 41. Energy and Angular Momentum Exchanges between Two Electrons in a Coulomb Field. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 493 H. G. M. Heideman 42. Oscillatory Structure of Excitation Functions in Atomic Collisions . 509 D. Hasselkamp, A. Scharmann, and K.-H. Schartner

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H. KLEINPOPPEN AND J. F. WILLIAMS It has only very recently become possible to study angular correlations and coherence effects in different areas of atomic collision processes: These investigations have provided us with an analysis of experimental data in terms of scattering amplitudes and their ph
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