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Chemical Dynamics at Low Temperatures PDF

387 Pages·1994·12.98 MB·English
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‘CHEMICAL DYNAMICS AT LOW TEMPERATURES ADSNCES IN CHESGCAL PHYSICS Cont Batszauers, Kobenian Unicenter FyeceKominy Inn, Kemi Taurens, reaver Duce Tense Colawbia Lora equa al Clarity, New You, New “Youu U5. (6 Coan, Trane a Fea “gies Manson" Chivers Mosier Cetak, Eevon seu: sod Eaglocebg Company. Aapencals, New Tests, US 8 en Prong Ue fan Fries bat, Tae Liss: Crago, Che itkies, US. evinnn Ti Keinas, Uneersty of Tn, Torts, Ont. Cet ‘Shiau Kravwnzy Bevautent of Chey. Hav Unecaly, Ceibelgs Mavasaurs USA. Ye LRonornssen, Deporte of Pte, Meson Sloe Caversy. Wo Kt. Tnutate of Bile, Phpy, Rusia AerSsoy af Se2ace Paso ‘Moxo% Fepoo. Fusia Reoy Mnacus, Derarinen! oF Chomisty Cadfomia Inte sf Teckasbey Pinion. Cora, U9 Gnnncioe Mint, Leben Lie de Rati, aca tay Sie, Bi ‘lan Belson ‘A. Bacar, Conte de Reshetthes Pan, Fal, Dowsing Cuevas, Tales, YY, Fann, Sere se Phaove Theor, Coune Eley Nace ce ‘Sesh, Gesmevrele, Peace Pr Seacin, Inne Cbe Mhorez che Chemie nl StH. ive Tecan Stasis, Oly Sue Unbenity, Desuraces of Camis, Columbus, ‘Gas USA. Kygomags Toss. Dopaeasat uf Mein Faeuly of Seence, Unive ot Kove, Rests, lapse CHEMICAL DYNAMICS AT LOW TEMPERATURES VICTOR A. AENDERSKIL ghee Foe ao toy a Ca tay of amg Esai Star SEHD INTRODUCTION Frese of us can ane Lager keep 4p sith the toed ut scienbts tertare ven in apecinzed suatelds Any attempt te Uo mere ame padky educated Wik respect fof. ege domein a sance his tbe appear oF ‘lug. at windnilk. Yee tho svtthose of ales crema <ilfetent fusiget into ner, postal. general coneops vo whale a eves. end the dose somein educeted persists mL EL scicatts, This oves ‘Adianees in Chenstal Plucis. it deveted t Alping the tele oblsin general information abn ¥ oie vaiey of pi in ekanial phys Feld slick we ialemret serv usrls. Our tiene is 40 hace expert present vnmprehennive analysts of subjess ol ineres std Ip encewiage the expression of nu idual point view We lupe Wi ts pica ta the Preventation of an overeiow of 4 subject wil 30th atimate ewe reset and seve at ptsilind Weaning est for Bogranets i 4 Gel ues Pace Sresae 8. Keck PREFACE, ‘Coomical dynamics ar lew temperatures is ccna dh ele ears reactors thac cannouat petentel energy battiers separating Betas Fin predues inthe dere of teas acuvauow “Il Gest expects outa fvitenoe of this tspe ot veaslions say abteiied un tho eaily 197s an CL slid site courerson of roe resitas. ‘These invetiyations lecely demonstrated that there is © sufciently starp tears from Arrhenivedike.esponsntl ompersture uspenleace, sturacteisti Ul Uhernal arian, ta mach weaker povar-bke operate slepemlenes dro fo ihe lus-lempetae bt Ie eile constant fh prineiye, the oeplimition ul Ibi phsnomenon was known 9 bs associate ih lenuglng throvgh 3 samme Only ler 4 substan boy OF experiment dsc wees acevrlaled mere adeuate aaah ove.upel faut eliidéted the mulddimersisual chatter vf amucling amd Ube ets of uontannelirg intra: and ineerrclelas vise end mles Same idess have Poca conideced iadedendendy in he yuan Uconmeenslale thours. sich har Pest eiplied mainly to gnephase Fctums paaceeng a8 the region Doles the anecgetie thrid. The supersonie je cue technique. ip corabiation with hieh-ssolutioa Tuatecularspecruntopy, has rsveled numerous snaps 22 raltidimtst- ual tieling in dook.ed moloelee and diner, “Theis ere t mnmaber if speci sues corsning the advaaees in each ef cheve sjate eres of overt, bev deve is us% 4 need Lor 4 Snvey of ihe oative field The jun oumaleration of auulisquensienal ‘anneling an fis mimssuution ia che isinas Branches uf cherie fhysics can pevvide thecetcine with a. quide on 4 Mage set of sot imicleed peels ta whish medeta quar mechanical metho em he arplisd, Fxpetimenatine teed infortation 30a" the deep, angles Ibetteen rwaeling hence asin, paee wea wanna flee Ia, st frst sgh, ght ceecryrelate, Oe gol ty tt adrays hath a tose ‘ieee sigh setae Th sacle of the everen sola sil the ch DF mat, In the fst chupter. tho history of the devslepment of chem) stynamige st lowe lamperotar & yorisjed Ike fumaelation of general ‘prem sl the min apynoaamations sed ts sul them dee green. The Secon chapler censilers speviie Lestnves of tannekng ehecn4al ty raniss The resol ave proseitel wathuvt denvation, The fed shaper onan consists description of sasdinnreiona ewnnsting in eke ath incegeal fervaligns, The snnve texdtinucl consideration st the ste pucoten inthe WE apprcainatin i givin Append & This chapter SS uesyued us aewexeuer to the sled 3 ie anti tevey «heme Fenevias, The fourth anf chapters ave devoted Ws aes, problette lf rwo- ans mulidasnsioual tungeing. Reasers win £2 aot Interested in theovoucal agpects tam skip those fo Chepters. bucoate Chepter 2 ‘online tho ban anlormataon necesary foc und.amanding Chapters iavwhich peronen’ experimen a evils are presented We are qratslal 7% L. Goldens, who wes the iilaler of the snvesligation this ek, W. HL Miler. N- Mkt, and B. Crubar tor weld) avis. sai Nelped us ix seleviun of ‘macrick. und our colaborains, P. Gnnsvich, E. Yi, Misuchko. ard T_1. Tagee. J. tar ‘upon and dscosiows, One of 32 (VA. i grate to ths Nabil Seeise Tonwltivn Ive sappert ual 0 ihe Gaiversity of LURK Inssitalicy wh le is solu wap en g writen Flas, we ave ied ter Aung Tapig snd leaner Brndeshi fay hie skill esksauce the preparation sf the manus enegioke ae Views A, Raters Fem aia 2. Makarae So Boke Oop Bk Charles A. Wight CONTENTS Terman 1 eon Tanna Action 4B TUsseLIse Is Ossonsession se Moves as ‘gansta “LtsseLine o Cuuvton. Desewtes ne Ter Parsrere of 4 Hear Ravi i Hypnocns Trewern 1s “Teserine Rerarion wy ‘Vrensrios: Rovaniow Tustesis Sertanavenr® oF Mouuut ces ane ovens oA Hieawy Panter Teasstra 39 Covers 3 Reruuscrs aa Atal ise Somes wis CHEMICAL. DYNAMICS AT LOW TEMPERATURES. ADWANCES IN CHEMICAL PHYSICS INTRODUCTION CON UNS La. AISTORICAT. BACKGROUND Evety cheingal reeetin islnse th ssarrengenaemt of chemical Bones. Und ordinary cccunscanes, hs eetarane and products ate slable om the une ile of thoi brawn frscuoncis. In this tespes! thee represent Suisislstioniey sratss, aml the section isl anvoiated wih sommunnbng an energy omer thal divdes them, The shits of he reaelane unser thermal vumhtions implies thatthe pupwhion dt them among theieenongy Levels close ty eatin. Foe his to take lice, the hamer aga! su) he greater dn both the tNeraal energy fa the energy Teel spy: that os Aly Yefig BEET ‘Under these conditions the ze constant is detetraned hy the setscally aveziged resetive fue fim the inkl be the line sale “Ths quintessential expresnen of shige chemicil kiuslws i8 the Amiens HD) k 089i Bhs 12) “The vate cian nt exptesion 230 he tntereta ookey 8 some sh-raterins aren frquney tiple yn Beltomarn tector, which Fearesents the prehailty of accupving the initial sees Cet is jst abe the rope the Bain, Tre Atri lew pedis that even ta Ue est Darier sil saisy'ng 54 (1-1) the vate Gomstent varshes 2 solizoly Tow: pens, For mance, even “op 2 veae asl xeaca Sah Ms, L2kgal:mol, FM et ac 30K, The Tae constant Grants th lh oe at TINK, Such a law value ul & suple.sly presludes he possibly of wcusuniag cy couvensie a a Leorateny ane wale

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