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Basic Studies in the Field of High-Temperature Engineering. PDF

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Nuclear Science Basic Studies in the Field of High-temperature Engineering Second Information Exchange Meeting Paris, France 10-12 October 2001 Co-organised by the Japan Atomic Energy Research Institute (JAERI) NUCLEAR ENERGY AGENCY ORGANISATION FOR ECONOMIC CO-OPERATION AND DEVELOPMENT ORGANISATION FOR ECONOMIC CO-OPERATION AND DEVELOPMENT Pursuant to Article 1 of the Convention signed in Paris on 14th December 1960, and which came into force on 30th September 1961, the Organisation for Economic Co-operation and Development (OECD) shall promote policies designed: − to achieve the highest sustainable economic growth and employment and a rising standard of living in Member countries, while maintaining financial stability, and thus to contribute to the development of the world economy; − to contribute to sound economic expansion in Member as well as non-member countries in the process of economic development; and − to contribute to the expansion of world trade on a multilateral, non-discriminatory basis in accordance with international obligations. The original Member countries of the OECD are Austria, Belgium, Canada, Denmark, France, Germany, Greece, Iceland, Ireland, Italy, Luxembourg, the Netherlands, Norway, Portugal, Spain, Sweden, Switzerland, Turkey, the United Kingdom and the United States. The following countries became Members subsequently through accession at the dates indicated hereafter: Japan (28th April 1964), Finland (28th January 1969), Australia (7th June 1971), New Zealand (29th May 1973), Mexico (18th May 1994), the Czech Republic (21st December 1995), Hungary (7th May 1996), Poland (22nd November 1996) and the Republic of Korea (12th December 1996). The Commission of the European Communities takes part in the work of the OECD (Article 13 of the OECD Convention). NUCLEAR ENERGY AGENCY The OECD Nuclear Energy Agency (NEA) was established on 1st February 1958 under the name of the OEEC European Nuclear Energy Agency. It received its present designation on 20th April 1972, when Japan became its first non-European full Member. NEA membership today consists of 27 OECD Member countries: Australia, Austria, Belgium, Canada, Czech Republic, Denmark, Finland, France, Germany, Greece, Hungary, Iceland, Ireland, Italy, Japan, Luxembourg, Mexico, the Netherlands, Norway, Portugal, Republic of Korea, Spain, Sweden, Switzerland, Turkey, the United Kingdom and the United States. The Commission of the European Communities also takes part in the work of the Agency. The mission of the NEA is: − to assist its Member countries in maintaining and further developing, through international co-operation, the scientific, technological and legal bases required for a safe, environmentally friendly and economical use of nuclear energy for peaceful purposes, as well as − to provide authoritative assessments and to forge common understandings on key issues, as input to government decisions on nuclear energy policy and to broader OECD policy analyses in areas such as energy and sustainable development. Specific areas of competence of the NEA include safety and regulation of nuclear activities, radioactive waste management, radiological protection, nuclear science, economic and technical analyses of the nuclear fuel cycle, nuclear law and liability, and public information. The NEA Data Bank provides nuclear data and computer program services for participating countries. In these and related tasks, the NEA works in close collaboration with the International Atomic Energy Agency in Vienna, with which it has a Co-operation Agreement, as well as with other international organisations in the nuclear field. © OECD 2002 Permission to reproduce a portion of this work for non-commercial purposes or classroom use should be obtained through the Centre français d’exploitation du droit de copie (CCF), 20, rue des Grands-Augustins, 75006 Paris, France, Tel. (33-1) 44 07 47 70, Fax (33-1) 46 34 67 19, for every country except the United States. In the United States permission should be obtained through the Copyright Clearance Center, Customer Service, (508)750-8400, 222 Rosewood Drive, Danvers, MA 01923, USA, or CCC Online: http://www.copyright.com/. All other applications for permission to reproduce or translate all or part of this book should be made to OECD Publications, 2, rue André-Pascal, 75775 Paris Cedex 16, France. FOREWORD In the field of basic research on materials pertinent to high-temperature and neutron irradiation tests, great international interest exists concerning the study of irradiation effects, notably on advanced ceramic and metallic materials and on the development of in-core instrumentation. For this reason, the Nuclear Science Committee (NSC) of the OECD Nuclear Energy Agency (NEA), along with the Japan Atomic Energy Research Institute (JAERI), organised the Second Information Exchange Meeting on Basic Studies in the Field of High-temperature Engineering. The meeting was held in Paris on 10-12 October 2001, and attended by 43 participants from eight countries and two international organisations. A total of 28 papers were presented, including 26 orally, dealing with recent progress in the following research domains: • overviews of high-temperature engineering research in each country and organisation; • improvement in material properties by high-temperature irradiation; • development of in-core material characterisation methods and irradiation facilities; • basic studies on the behaviour of irradiated graphite/carbon and ceramic materials including their composites under both operation and storage conditions; • basic studies on high-temperature, gas-cooled reactor (HTGR) fuel fabrication and performance. The final session was dedicated to discussing possible co-operative works to be undertaken within the framework of the OECD/NEA Nuclear Science Committee. It was recommended that a further information exchange meeting, dealing with possible international collaboration as well as some of the topics addressed here, should be planned to be held in Oarai, Japan in 2003. 3 TABLE OF CONTENTS Foreword............................................................................................................................................ 3 Executive Summary............................................................................................................................ 9 OPENING SESSION....................................................................................................................... 11 C. Kessler Welcome Address..................................................................................................... 13 S. Ishino Opening Address...................................................................................................... 15 SESSION I Overviews of High-temperature Engineering Research in Each Country and Organisation..................................................................................... 17 Chair: W. von Lensa J. Martín-Bermejo, M. Hugon, G. Van Goethem Research Activities on High-temperature Gas-cooled Reactors (HTRs) in the 5th EURATOM RTD Framework Programme................................................ 19 J. Kendall, M. Methnani Update on IAEA High-temperature Gas-cooled Reactor Activities......................... 31 Y. Sudo, T. Hoshiya, M. Ishihara, T. Shibata, S. Ishino, T. Terai, T. Oku, Y. Motohashi, S. Tagawa, Y. Katsumura, M. Yamawaki, T. Shikama, C. Mori, H. Itoh, S. Shiozawa Present Status of the Innovative Basic Research on High-temperature Engineering using the HTTR.................................................................................... 39 J.C. Kuijper, A.I. van Heek, J.B.M. de Haas, R. Conrad, M. Burghartz, J.L. Kloosterman Present Status in the Netherlands of Research Relevant to High Temperature Gas-cooled Reactor Design................................................................. 51 D. Hittner, F. Carré, J. Roualt Current Status of High-temperature Engineering Research in France...................... 69 K. Kugeler, P-W. Phlippen, M. Kugeler, H. Hohn Overview of High-temperature Reactor Engineering and Research......................... 77 A.J. Wickham, I.M. Coe, P.J. Bramah, T.J. Abram The Contribution of UK Organisations in the Development of New High-temperature Reactors....................................................................................... 91 5 SESSION II Improvement in Material Properties by High-temperature Irradiation........... 101 Chairs: T. Shikama, B. Marsden H. Kurishita Improvement in Ductility of Refractory Metals by Neutron Irradiation.................. 103 M. Ishihara, T. Shibata, S. Baba, T. Hoshiya, C. Wan, Y. Motohashi Effects of Superplastic Deformation on Thermal and Mechanical Properties of 3Y-TZP Ceramics (Review)................................................................ 113 C.H. Wu Development of an Innovative Carbon-based Ceramic Material: Application in High-temperature, Neutron and Hydrogen Environment................. 125 T. Nitawaki, Y. Kato A Carbon Dioxide Partial Condensation Cycle for High-temperature Reactors....................................................................................... 133 SESSION III Development of In-core Material Characterisation Methods and Irradiation Facility.......................................................................................... 143 Chairs: C. Vitanza, M. Yamawaki T. Shibata, T. Kikuchi, S. Miyamoto, K. Ogura, Y. Ishigaki Development of the I-I Type Irradiation Equipment for the HTTR......................... 145 T. Shikama, M. Narui, T. Kakuta, M. Ishitsuka, K. Hayashi, T. Sagawa, T. Hoshiya Application of Optical Diagnostics in High-temperature Gas-cooled Systems.................................................................................................. 153 C. Mori, A. Uritani, T. Kakuta, M. Katagiri, T. Shikama, M. Nakazawa, T. Iguchi, J. Kawarabayashi, I. Kimura, H. Kobayashi, S. Hayashi Measurement Method of In-core Neutron and Gamma-ray Distributions with Scintillator Optical Fibre Detector and Self-powered Detector.............................................................................................. 161 C. Vitanza Development of In-core Test Capabilities for Material Characterisation................. 167 G-N. Luo, T. Terai, M. Yamawaki, K. Yamaguchi Application of Work Function Measuring Technique to Monitoring/ Characterisation of Material Surfaces under Irradiation........................................... 177 M. Narui, T. Shikama, M. Yamasaki, H. Matsui Development of High-temperature Irradiation Techniques Utilising the Japan Materials Testing Reactor.......................................................... 191 6 SESSION IV Basic Studies on Behaviour of Irradiated Graphite/Carbon and Ceramic Materials Including their Composites under both Operation and Storage Conditions.......................................................................................... 201 Chairs: B. McEnaney, A. Wickham D. Buckthorpe, R. Couturier, B. van der Schaaf, B. Riou, H. Rantala, R. Moormann, F. Alonso, B-C. Friedrich Investigation of High-temperature Reactor (HTR) Materials................................... 203 W.R. Taylor, M.D. Warner, G.B. Neighbour, B. McEnaney, S.E. Clift Radially Keyed Graphite Moderator Cores: An Investigation into the Stability of Finite Element Models.............................................................. 215 M. Ishihara, T. Shibata, T. Takahashi, S. Baba, T. Hoshiya Understanding of Mechanical Properties of Graphite on the Basis of Mesoscopic Microstructure (Review)......................................................... 225 R. Moormann, H-K. Hinssen Advanced Graphite Oxidation Models..................................................................... 243 B.J. Marsden, S.D. Preston Irradiation Creep in Graphite – A Review................................................................ 255 G.B. Neighbour, P.J. Hacker An Analysis of Irradiation Creep in Nuclear Graphites............................................ 269 B. McEnaney, A.J. Wickham, M. Dubourg Planning for Disposal of Irradiated Graphite: Issues for the New Generation of HTRs.................................................................................................. 281 P.J. Hacker, B. McEnaney, A.J. Wickham, G. Haag Status of IAEA International Database on Irradiated Graphite Properties with Respect to HTR Engineering Issues................................................ 293 SESSION V Basic Studies on HTGR Fuel Fabrication and Performance.............................. 305 Chairs: J. Kuijper, R. Moormann L. Thomé, A. Gentils, F. Garrido, J. Jagielski Evidence of Dramatic Fission Product Release from Irradiated Nuclear Ceramics...................................................................................................... 307 A. Chernikov, V. Eremeev, V. Ivanov Method of Reactor Tests of HTGR Fuel Elements at an Impulse Loading.............. 315 D. Petti, G. Miller, J. Maki, D. Varacalle, J. Buongiorno Gas Reactor TRISO-coated Particle Fuel Modelling Activities at the Idaho National Engineering and Environmental Laboratory.......................... 323 7 Session Summaries........................................................................................................................... 339 Chair: Y. Sudo Recommendations.............................................................................................................................. 349 List of Participants.............................................................................................................................. 351 8 EXECUTIVE SUMMARY Co-organised by the OECD Nuclear Energy Agency and Japan Atomic Energy Research Institute, the Second Information Exchange Meeting on Basic Studies in the Field of High-temperature Engineering was a great success. It was held in Paris on 10-12 October, 2001, and its main topics were: • The exchange of information with regard to the latest activities for studying high-temperature irradiation-induced damage/effects in advanced materials and fuels. • The discussion of the possibility of co-operative studies in the field of high-temperature engineering using the HTTR and other research reactors for irradiation research programmes in the framework of international co-operation organised by the OECD/NEA/NSC. • The development of a framework of possible international co-operative activities concerning topics of interest. • The proposal/recommendation of possible co-operative works to be undertaken within a framework or under the auspices of the OECD/NEA/NSC. Forty-three participants gathered together from eight countries and two international organisations. Twenty-eight papers were submitted, of which 26 were oral presentations dealing with recent progress and national/international programmes in the field of high-temperature engineering. The papers were presented in five sessions as follows: • Session I: Overviews of high-temperature engineering research in each country and organisation (six papers). • Session II: Improvement in material properties by high-temperature irradiation(four papers). • Session III: Development of in-core material characterisation methods and irradiation facilities (six papers). • Session IV: Basic studies on the behaviour of irradiated graphite/carbon and ceramic materials including their composites under both operation and storage conditions(eight papers). • Session V: Basic studies on HTGR fuel fabrication and performance(two papers). In Session I, the current status of high-temperature engineering research in the EC, Japan, the Netherlands, France, Germany and the United Kingdom were summarised. In Session II, examples of improvement in material properties through high-temperature irradiation, the effects of superplastic deformation on thermal and mechanical properties of 3Y-TZP ceramics and the development of an innovative carbon-based ceramic material and carbon dioxide partial condensation cycle were presented. 9

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