ATMOSPHERIC TURBULENCE AND AIR POLLUTION MODELLING ATMOSPHERIC SCIENCES LIBRARY Editorial Advisory Board R. A. Anthes Nationsl Center for Atmospheric Research (U.S.A.) A. Berger Universite Catholique Louvain (Belgium) P. J. Crutzen Max-Planck-Institut fur Chemie (F.R.G.) H.-W. Georgii Universitit Frankfurt (F.R.G.) P. V. Hobbs University of Washington, Seattle (U.S.A.) A. Hollingsworth European Centre for Medium Range Weather Forecasts, Reading (England) G. E. Hunt University College London (England) K. Ya. Kondratyev Main Geophysical Observatory, Moscow (U.S.S.R.) T. N. Krishnamurti The Florida State University, Tallahassee (U.S.A.) J. Latham University of Manchester Institute of Science and Technology (England) D. K. Lilly National Center for Atmospheric Research (U.S.A.) J.London University of Colorado, Boulder (U.S.A.) A. H. Dort National Oceanic and Atmospheric Administration (U.S.A.) I. Drlanski National Oceanic and A tmospheric Administration (U.S.A.) H. R. Pruppacher Johannes Gutenberg Universitit, Mainz (F.R.G.) N. J. Rosenberg University of Nebraska, Lincoln (U.S.A.) C. J. E. Schuurmans Rijksuniversiteit Utrecht (The Netherlands) H. Tennekes Koninklijk Nederlands Meteorologisch Instituut, de Bilt (The Netherlands) S.A. Twomey The University of Arizona (U.S.A.) T. M. L. Wigley University of East Anglia (England) J. C. Wijngaard National Center for Atmospheric Research (U.S.A.) V. E. Zuev Institute for Atmospheric Optics, Tomsk (U.S.S.R.) Atmospheric Turbulence and Air Pollution Modelling A Course held in The Hague, 21-25 September, 1981 edited by F. T. M. NIEUWSTADT and H. VAN DOP Royal Netherlands Meteorological Institute, de Bilt D. Reidel Publishing Company A MEMBER OF THE KLUWER ACADEMIC PUBLISHERS GROUP " Dordrecht I Boston I Lancaster library of Congress Cataloging in Publication Data Main entry under title: Atmospheric turbulence and air pollution modelling. (Atmospheric sciences library) Bibliography: p. Includes indexes. 1. Atmospheric turbulence-Mathematical models-Addresses, essays, lectures. 2. Boundary layer (Meteorology)-Mathematical models-Addresses, essays, lectures. 3. Atmospheric diffusion-Mathematical models-Addresses, essays, lectures. 4. Air-Pollution-Meteorological aspects-Mathematical models-Addresses, essays, lectures. I. Nieuwstadt, F. T. M. (Frans T. M.), 1946- . II. Dop, H. van (Han van), 1944- . III. Series. QC880.4.T8A85 551.5'17 82-3758 ISBN-13: 978-90-277-1807-5 e-ISBN-13: 978-94-010-9112-1 DOl: 10.1007/978-94-010-9112-1 AACR2 Published by D. Reidel Publishing Company P.O. Box 17, 3300 AA Dordrecht, Holland Sold and distributed in the U.S.A. and Canada by Kluwer Academic Publishers, 190 Old Derby Street, Hingham, MA 02043, U.S.A. In all other countries, sold and distributed by Kluwer Academic Publishers Group, P.O. Box 322, 3300 AH Dordrecht, Holland Reprinted with corrections. All Rights Reserved © 1982,1984 by D. Reidel Publishing Company, Dordrecht, Holland No part of the material protected by this copyright notice may be reproduced or utilized in any form or by any means, electronic or mechanical, including photocopying, recording or by any information storage and retrieval system, without written permission from the copyright owner CONTENTS PREFACE xi SYMBOLS AND NOTATION xv ACKNOWLEDGEMENTS xxi 1. EQUATIONS AND CONCEPTS - J.A. BUSINGER 1 1.1. INTRODUCTION 1 1.2. GOVERNING EQUATIONS 2 The Equations of Continuity 2 The Equation of State 3 Potential Temperature 4 The Equations of Motion 5 Conservation of Enthalpy 6 Conservation of Transferable Scalar Quantities 8 1.3. EQUATIONS OF THE MEAN FLOW 8 1.4. DISCUSSION OF THE BOUSSINESQ APPROXIMATIONS AND THE CONSERVATION OF ENTHALPY EQUATION 13 1.5. SUMMARY OF THE BOUSSINESQ SET OF EQUATICNS 15 1.6. THE CLOSURE PROBLEM, FIRST-ORDER CLOSURE 16 1 .7. SECOND-ORDER VARIANCE AND COVARIANCE EQUATIONS 19 1.8. THE TURBULENT KINETIC ENERGY BALANCE; TEMPERATURE VARIANCE BALANCE 22 APPENDIX A. REQUIREMENTS FOR A DIVERGENCE-FREE VELOCITY FIELD 26 vi CONTENTS APPENDIX B. THE MAGNITUDE OF PRESSURE FLUCTUATIONS 30 APPENDIX C. THE ENTHALPY EQUATION FOR mIST AIR 30 APPENDIX D. THE EKMAN SPIRAL 33 2. SIMILARITY RELATIONS, SCALING LAWS AND SPECTRAL DYNAMICS - H. TENNEKES 37 2.1. INTRODUCTION 37 2.2. SIMILARITY 39 ROSSBY~NUMBER The Surface Layer 42 The Process of Matching 43 The Constant-Stress Layer 46 The Von Karman Constant 47 2.3. DIABATIC EXTENSION OF ROSSBY-NUMBER SIMILARITY 47 2.4. MONIN-OBUKHOV SIMILARITY IN THE SURFACE LAYER 50 2.5. SCALING OF TURBULENCE QUANTITIES IN THE SURFACE LAYER 53 2.6. SCALING OF TURBULENCE OUTSIDE THE SURFACE LAYER 56 2.7. CORRELATION FUNCTIONS AND SPECTRA 60 2.8. INERTIAL SUBRANGES 64 3. BOUNDARY-LAYER MODELING - J.C. WYNGAARD 69 3.1. THE CALCULATION OF BOUNDARY-LAYER STRUCTURE 69 3.2. ENSEMBLE-AVERAGE MODELS 72 First-Order or Eddy-Diffusivity (K) Closure 72 Second-Order Closure 77 3.3. VOLUME-AVERAGE MODELS 97 Large-Eddy Models 98 Other Volume-Average Models 105 CONTENTS vii 4. OBSERVED CHARACTERISTICS OF THE ATMOSPHERIC BOUNDARY LAYER - S.J. CAUGHEY 107 4.1. INTRODUCTION 107 4.2. CONVECTIVE BOUNDARY LAYER 110 Boundary-Layer Development 110 Spectra of the Velocity Components 114 SpectI'1B of Temperature 119 Cospectra of Heat Flux and Stress 121 Entrainment 127 Variances, Dissipation Rates and Structure Parameters 131 Turbulent Kinetic Energy Budget 137 4.3. STABLE BOUNDARY LAYER 139 General Characteristics of the SBL 139 Waves and Turbulence 143 Turbulence Spectra in the Stable Surface Layer 148 Turbulence Behavior through the SBL Depth 150 Depth of the SBL 156 4.4. CONCLUDING REMARKS 156 5. DIFFUSION IN THE CONVECTIVE BOUNDARY LAYER - R.G. LAMB 159 5.1. INTRODUCTION 159 5.2. FORMULATION OF A LAGRANGIAN DIFFUSION HODEL 166 5.3. NUMERICAL SIMULATIONS OF NON-BUOYANT MATERIAL DIFFUSION AND COMPARISONS WITH OBSERVATIONS 175 Results 176 Comparison of the Model Results with Observations 183 5.4. THE STRUCTURE OF TURBULENCE IN THE CONVECTIVE BOUNDARY LAYER 191 5.5. FORMULAS FOR APPLICATION 197 5.6. DISPERSION OF BUOYANT EMISSIONS IN A CONVECTIVE BOUNDARY LAYER 206 viii CONTENTS 6. DIFFUSION IN THE STABLE BOUNDARY LAYER - J.C.R. HUNT 231 6.1. INTRODUCTION 231 6.2. BASIC IDEAS ABOUT MOLECULAR AND FLUID ELEMENT MOTION AND PROBABILITY DISTRIBUTIONS 232 6.3. TURBULENT DIFFUSION IN IDEALIZED FLOWS 236 Marked Fluid Elements in Unstratified Turbulence Away from Boundaries 236 Unidirectional shear flow 238 Straining flow 243 Flux gradient relations - when are they likely to go wrong? 244 Diffusion in Stably-Stratified Turbulence 247 6.4. TURBULENCE DIFFUSION IN THE STABLY-STRATIFIED ATMOSPHERIC BOUNDARY LAYER 253 Some Properties of the Stably Stratified Atmospheric Boundary Layer 253 Mean velocity profile 254 Mean temperature profile 254 Vertical turbulence and heat flux 254 Horizontal components of turbulence 255 Turbulence at heights of 50 to 300 m 256 Diffusivities and temperature fluctuations 256 Elevated Source above the Surface Layer 258 Sources in the Surface Layer 260 < Elevated sources in the surface layer (t TL) 260 > Elevated sources in the surface layer (t TL) 262 Comparison of vertical diffusion from ground-level and elevated sources 269 6.5. CONCLUDING REMARKS 271 Concentration Distributions 271 Complex Atmospheric Conditions 272 Topography 272 7. APPLICATIONS IN AIR POLLUTION MODELING - S.R. HANNA 275 7.1. INTRODUCTION 275 CONTENTS ix 7.2. STATISTICAL MODELS OF DIFFUSION 277 Taylor's Statistical Theory 277 Monte Carlo Diffusion Models 280 Model description 280 Turbulent energy and Lagrangian time scales in the unstable PBL 282 Turbulent energy and Lagrangian time scales in the stable PBL 283 Turbulent energy and Lagrangian time scales in the neutral PBL 284 Results of application of the Monte Carlo model 285 The Langevin Horizontal Diffusion Model 286 7.3. IMPROVEMENTS TO THE GAUSSIAN MODEL 288 Wind Speed in the Gaussian Plume Model 288 Plume Rise Calculations 289 Estimation of Gy and Gz using Ge and Ge 290 Determination of Stability Class 291 Revisions of Pasquill-Gifford (P-G) Sigma Curves 292 7.4. K-DIFFUSION MODELS 295 Analytical Solutions to the Diffusion Equation 295 Numerical Solutions to the Diffusion Equation 297 7.5. PROGRESS IN THE SIMILARITY THEORY OF DIFFUSION 300 7.6. RECENT SPECIAL APPLICATIONS 303 Skewness of'Vertical Turbulent Velocity 304 Natural Variability of Pollutant Concentrations 306 Representativeness of Wind-Speed Observations 307 8. REPORT FROM THE PANEL DISCUSSION - L. KRISTENSEN 311 9. REFERENCES 323 AUTHORS INDEX 343 SUBJECT INDEX 350 PREFACE The study of turbulence in the atmosphere has seen considerable progress in the last decade. To put it briefly: boundary-layer meteorology, the branch of atmospheric science that concentrates on turbulence in the lower atmosphere, has moved from the surface layer into the boundary layer itself. The progress has been made on all fronts: theoretical, numerical and observational. On the other hand, air pollution modeling has not seen such a rapid evolution. It has not benefited as much as it should have from the increasing knowledge in the field of atmospheric turbulence. Air pollution modeling is still in many ways based on observations and theories of the surface layer only. This book aims to bring the reader up to date on recent advances in boundary-layer meteorology and to pave the path for applications in air pollution dispersion problems. The text originates from the material presented during a short course on Atmospheric Turbulence and Air Pollution Modeling held in The Hague during September 1981. This course was sponsored and organized by the Royal Netherlands Meteorological Institute, xi