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SUPPLEMENT TO ATMOSPHERIC ENVIRONMENT Volume 33 1999 Volume Contents, Author Index and Subject Index © PERGAMON ATMOSPHERIC ENVIRONMENT SCOPE The subject matter of papers published in Atmospheric Environment covers all aspects of the interaction of people and ecosystems with their atmospheric environment. This includes scientific, administrative, eco- nomic and political aspects of these interactions. The main aim of Atmospheric Environment is to provide a scientific understanding of the consequences of natural and human-induced perturbations on the Earth’s atmosphere. Areas covered include but are not limited to air pollution research and its applications, air quality and its effects, dispersion and transport, deposition, biospheric-atmospheric exchange, global atmospheric chemistry, radiation and climate. Novel results based on experiments, theory and modelling of the atmosphere, extending from the local to global scales, are included. 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Atmospheric Environment (ISSN 1352-2310) is published (semi monthly with extra issues in February, April, June, August, October and December) by Elsevier Science Ltd., The Boulevard, Langford Lane, Kidlington, Oxford OX5 1GB, UK. The US subscription price is $3561.00 per year. POSTMASTER: Send address corrections to: Atmospheric Environment, Elsevier Science, Customer Support Department, PO Box 945, New York, NY 10159-0945. Distributed in the USA by Mercury Airfreight International, 365 Blair Road, Avenel, NJ 07001. Disclaimer: Whilst every effort is made by the Publishers and Editorial Board to see that no inaccurate or misleading data, opinion or statement appear in this Journal, they wish to make it clear that the data and opinions appearing in the articles and advertisements herein are the sole responsibility of the contributor or advertiser concerned. Accordingly, the Publishers, the Editorial Board and Editors and their respective employees, officers and agents accept no responsibility or liability whatsoever for the consequences of any such inaccurate or misleading data, opinion or statement. CONTENTS OF VOLUME 33 Number 1 G.C.K. Lam, D.Y.C. Leung, Street-level concentrations of nitrogen dioxide and suspended M. Niewiadomski, S.W. Pang, particulate matter in Hong Kong A.W.F. Lee and P.K.K. Louie J.P. Kunsch Critical velocity and range of a fire-gas plume in a ventilated tunnel I.V. Patroescu, I. Barnes, FT-IR product study of the OH-initiated oxidation of DMS in K.H. Becker and N. Mihalopoulos the presence of NO, D.M. Holland, P.P. Principe and Trends in atmospheric sulfur and nitrogen species in the eastern J.E. Sickles, II United States for 1989-1995 R.H. Grant and Ka-Lam Wong Ozone profiles over a suburban neighborhood R.C. Musselman and W.J. Massman Ozone flux to vegetation and its relationship to plant response and ambient air quality standards T. Salthammer, A. Schwarz and Emission of reactive compounds and secondary products from F. Fuhrmann wood-based furniture coatings H. Kaupp and M.S. McLachlan Atmospheric particle size distributions of polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs) and polycyclic aromatic hydrocarbons (PAHs) and their implications for wet and dry deposition R. Vecchi and G. Valli Ozone assessment in the southern part of the Alps N. Moschonas, D. Danalatos The effect of O, and NO, on the ring retaining products of the and S. Glavas reaction of toluene with hydroxyl radicals K. Koeltzsch On the relationship between the Lagrangian and Eulerian time scale J.L. Collett, Jr., K.J. Hoag, Spatial and temporal variations in San Joaquin Valley fog D.E. Sherman, A. Bator and chemistry L. Willard Richards G.L. Hutchinson, W.X. Yang Overcoming humidity dependence of the chromium trioxide and C.E. Andre converter used in luminol-based nitric oxide detection Technical Note C. Dimitroulopoulou and The influence of the photolysis rates on modelled ozone con- H.M. ApSimon centrations Short Communication T.P. DeFelice Chemical composition of fresh snowfalls at Palmer Station, Antarctica ©. Gustaffsson and Hydrophobic organic compound partitioning from bulk water P.M. Gschwend to the water/air interface New Directions S.F. Watts and C.N. Roberts Hydrogen sulfide from car catalytic converters News and Opinions Introduction Calendar List of Forthcoming Papers Preparation of Papers Contents of Volume 33 Number 2 B.R.T. Simoneit, J.J. Schauer, 173 Levoglucosan, a tracer for cellulose in biomass burning and C.G. Nolte, D.R. Oros, atmospheric particles V.O. Elias, M.P. Fraser, W.F. Rogge and G.R. Cass A. El-Hussein, A.M ohammed 183 Radon exhalation and ultrafine fraction of radon progeny in and A.A. Ahmed closed room air P.-L. Leung and R.M. Harrison 191 Roadside and in-vehicle concentrations of monoaromatic hydrocarbons N.V. Heeb, A.-M. Forss 205 Fast and quantitative measurement of benzene, toluene and C,- and C. Bach benzenes in automotive exhaust during transient engine opera- tion with and without catalytic exhaust gas treatment T.G.M. Demmers, L.R. Burgess, 217 Ammonia emissions from two mechanically ventilated UK J.L. Short, V.R. Phillips, livestock buildings J.A. Clark and C.M. Wathes F. Sauer, C. Schafer, P. Neeb, 229 Formation of hydrogen peroxide in the ozonolysis of isoprene O. Horie and G.K. Moortgat and simple alkenes under humid conditions D. Blaha, K. Bartlett, P. Czepiel, 243 Natural and anthropogenic methane sources in New England R. Harriss and P. Crill Y.F. Li, Y.J. Zhang, G.L. Cao, 257 Distribution of seasonal SO, emissions from fuel combustion J.H. Liu and L.A. Barrie and industrial activities in Shanxi province, China, with 1/6° x 1/4° longitude/latitude resolution R.A. Hashmonay, M.G. Yost 267 Computed tomography of air pollutants using radial scanning and C.-F. Wu path-integrated optical remote sensing P.N. Price 275 Pollutant tomography using integrated concentration data from non-intersecting optical paths A. Maurizi and F. Tampieri 281 Velocity probability density functions in Lagrangian dispersion models for inhomogeneous turbulence B.L. Duffy, P.F. Nelson, Y. Ye 291 Speciated hydrocarbon profiles and calculated reactivities of and I.A. Weeks exhaust and evaporative emissions from 82 in-use light-duty Australian vehicles R.M. Harrison, M. Jones 309 Measurements of the physical properties of particles in the and G. Collins urban atmosphere D.R. Hastie, J. Narayan, 323 Observational evidence for the impact of the lake breeze circu- C. Schiller, H. Niki, P.B. Shepson, lation on ozone concentrations in Southern Ontario D.M.L. Sills, P.A. Taylor, Wm. J. Moroz, J.W. Drummond, N. Reid, R. Taylor, P.B. Roussel and O.T. Melo Technical Note _L. Thoni, F. Krieg 337 Testing the Bergerhoff method to determine the bulk depo- and U. Siewers sition loads of 49 elements News and Opinions Introduction Calendar List of Forthcoming Papers Preparation of Papers Contents of Volume 33 INS Number 3 R.M. Koerner, D.A. Fisher and 347 A 100 year record of ion chemistry from Agassiz Ice Cap, K. Goto-Azuma Northern Ellesmere Island NWT, CANADA A. Rodrigo, A. Avila and 359 Trace metal contents in Parmelia caperata (L.) Ach. compared A. Gomez-Bolea to bulk deposition, throughfall and leaf-wash fluxes in two holm oak forests in Montseny (NE Spain) C.L. Blanchard, F.W. Lurmann, 369 The use of ambient data to corroborate analyses of ozone P.M. Roth, H.E. Jeffries control strategies and M. Korc R.S. Gabruk, R.I. Sykes, C. Seigneur, 383 Evaluation of the reactive and optics model of emissions P. Pai, P. Gillespie, R.W. Bergstrom (ROME) and P. Saxena D. Wang, S.R. Yates, J. Gan and 401 Atmospheric volatilization of methyl bromide, 1,3-dichloro- J.A. Knuteson propene, and propargyl bromide through two plastic films: transfer coefficient and temperature effect W.-K. Jo and K.-H. Park 409 Commuter exposure to volatile organic compounds under different driving conditions A. Samecka-Cymerman 419 Bioindication of heavy metals in the town Wroctaw (Poland) and A.J. Kempers with evergreen plants D.A. Winner and G.R. Cass 431 Modeling the long-term frequency distribution of regional ozone concentrations W.J. Massman 453 Molecular diffusivities of Hg vapor in air, O02 and N2 near STP and the kinematic viscosity and thermal diffusivity of air near STP M. Jang and R.M. Kamens 459 Newly characterized products and composition of secondary aerosols from the reaction of «-pinene with ozone C.F. Clement and I.J. Ford 475 Gas-to-particle conversion in the atmosphere: I. Evidence from empirical atmospheric aerosols C.F. Clement and I.J. Ford 489 Gas-to-particle conversion in the atmosphere: II. Analytical models of nucleation bursts C. Duefas, M.C. Fernandez, 501 ?22Rn concentrations, natural flow rate and the radiation expo- S. Canete, J. Carretero and E. Liger sure levels in the Nerja Cave News and Opinions Introduction Calendar List of Forthcoming Papers Preparation of Papers Number 4 M.R. Heal, M.A. O’Donoghue and 513 Overestimation of urban nitrogen dioxide by passive diffusion J.N. Cape tubes: a comparative exposure and model study T. Etzkorn, B. Klotz, S. S@rensen, 525 Gas-phase absorption cross sections of 24 monocyclic aromatic I.V. Patroescu, I. Barnes, K.H. Becker hydrocarbons in the UV and IR spectral ranges and U. Platt IN6 Contents of Volume 33 C.J. Halsall, B. Gevao, M. Howsam, 541 Temperature dependence of PCBs in the UK atmosphere R.G.M. Lee, W.A. Ockenden and K.C. Jones G. Buzorius, K. Hameri, J. Pekkanen 553 Spatial variation of aerosol number concentration in Helsinki and M. Kulmala city K. von Salzen and K.H. Schliinzen 567 A prognostic physico-chemical model of secondary and marine inorganic multicomponent aerosols I. Model description B. Hall, C. Claiborn and D. Baldocchi 577 Measurement and modeling of the dry deposition of peroxides S.M. Aschmann and R. Atkinson 591 Atmospheric chemistry of 1-methyl-2-pyrrolidinone I. Mori, Y. lwasaka, K. Matsunaga, 601 Chemical characteristics of free tropospheric aerosols over the M. Hayashi and M. Nishikawa Japan Sea coast: aircraft-borne measurements B. Lighthart 611 An hypothesis describing the general temporal and spatial distribution of alfresco bacteria in the earth’s atmospheric surface layer G.M. Lovett, A.W. Thompson, 617 Elevational patterns of sulfur deposition at a site in the Catskill J.B. Anderson and J.J. Bowser Mountains, New York D.L. MacTaggart, S.O. Farwell 625 A continuous monitor-sulfur chemiluminescence detector (CM- J.R. Burdge, Z.-T. Cai, T.J. Haakenson SCD) system for the measurement of total gaseous sulfur spe- and W.L. Bamesberger cies in air J.A. van Aardenne, G.R. Carmichael, 633 Anthropogenic NO, emissions in Asia in the period 1990-2020 H. Levy HI, D. Streets, L. Hordijk J.P. Putaud, B.M. Davison, 647 Dimethylsulfide and its oxidation products at two sites in S.F. Watts, N. Mihalopoulos, Brittany (France) B.C. Nguyen and C.N. Hewitt A. Scaperdas and R.N. Colvile 661 Assessing the representativeness of monitoring data from an urban intersection site in central London, UK Technical Note P.C.S. Lee, R.A. Zaveri, R.C. Easter 675 On the parallelization of a global climate-chemistry modeling and L.K. Peters system New Directions S. Elliott, D.R. Blake and 683 Rapid industrialization in developing countries: the challenge F.S. Rowland to earth system research for the new millennium News and Opinions Introduction Calendar List of Forthcoming Papers Preparation of Papers EAC ’99 Announcement Number 5 D.J. Fish, D.E. Shallcross and The vertical distribution of NO3 in the atmospheric boundary R.L. Jones layer P. Wolkoff, P.A. Clausen, 693 Formation of strong airway irritants in a model mixture of C.K. Wilkins, K.S. Hougaard ( + )-a-pinene/ozone and G.D. Nielsen Contents of Volume 33 IN7 J. Kildesg, J. Vallarino, J.D. Spengler, 699 Dust built-up on surfaces in the indoor environment H.S. Brightman and T. Schneider M.W. Gardner and S.R. Dorling 709 Neural network modelling and prediction of hourly NO, and NO, concentrations in urban air in London E.D. Pellizzari, C.A. Clayton, 721 Particulate matter and manganese exposure in Toronto, C.E. Rodes, R.E. Mason, Canada L.L. Piper, B. Fort, G. Pfeifer and D. Lynam R.A. Hashmonay, M.G. Yost, 735 Emission rate apportionment from fugitive sources using open- Y. Mamane and Y. Benayahu path FTIR and mathematical inversion A.S. Ansari and S.N. Pandis 745 Prediction of multicomponent inorganic atmospheric aerosol behavior E.J. Highwood, K.P. Shine, 759 Estimation of direct radiative forcing due to non-methane hy- M.D. Hurley and T.J. Wallington drocarbons P.E. Padgett, E.B. Allen, 769 Changes in soil inorganic nitrogen as related to atmospheric A. Bytnerowicz and R.A. Minich nitrogenous pollutants in southern California M. Fang, M. Zheng, F. Wang, 783 The solvent-extractable organic compounds in the Indonesia K.L. To, A.B. Jaafar and S.L. Tong biomass burning aerosols - characterization studies W.O. Siegl, R.H. Hammerle, 797 Organic emissions profile for a light-duty diesel vehicle H.M. Herrmann, B.W. Wenclawiak and B. Luers-Jongen J.D. Shannon 807 Regional trends in wet deposition of sulfate in the United States and SO, emissions from 1980 through 1995 G.A. Allen, J. Lawrence and 817 Field validation of a semi-continuous method for aerosol black P. Koutrakis carbon (aethalometer) and temporal patterns of summertime hourly black carbon measurements in southwestern PA J.A. Lind and G.L. Kok 825 Emission strengths for primary pollutant as _ esti- mated from an aircraft study of Hong Kong air quality S.E. Cornell and T.D. Jickells 833 Water-soluble organic nitrogen in atmospheric aerosol: a com- parision of UV and persulfate oxidation methods News and Opinions Introduction Calendar List of Forthcoming Papers Preparation of Papers Number 6 H. Zhuang, C.K. Chan, M. Fang and 843 Size distributions of particulate sulfate, nitrate, and ammonium A.S. Wexler at a coastal site in Hong Kong J.P. Greenberg, A. Guenther, 855 Tethered balloon measurements of biogenic VOCs in the atmo- P. Zimmerman, W. Baugh, spheric boundary layer C. Geron, K. Davis, D. Helmig and L.F. Klinger IN8 Contents of Volume 33 M.D. Moulik and J.B. Milford 869 Factors influencing ozone chemistry in subsonic aircraft plumes T.C.W. Tung, C.Y.H. Chao and 881 A methodology to investigate the particulate penetration coef- J. Burnett ficient through building shell A. Kasper-Giebl, M.F. Kalina and 895 Scavenging ratios for sulfate, ammonium and nitrate deter- H. Puxbaum mined at Mt. Sonnblick (3106 m a.s.l.) L.W.A. van Hove, M.E. Bossen, 907 The uptake of O; by poplar leaves: the impact of a long-term F.A.M. de Bok and C.A.M. Hooijmaijers exposure to low O3-concentrations E.G. Pavelin, C.E. Johnson, S. Rughooputh 919 Evaluation of pre-industrial surface ozone measurements made and R. Toumi using Schonbein’s method P.A. Ariya, H. Niki, G.W. Harris, 931 Polar sunrise experiment 1995: hydrocarbon measurements K.G. Anlauf and D.E.J. Worthy and tropospheric Cl and Br-atoms chemistry I. Mavroidis, R.F. Griffiths, C.D. Jones 939 Experimental investigation of the residence of contaminants in and C.A. Biltoft the wake of an obstacle under different stability conditions S. Parat, A. Perdrix, S. Mann and 951 Contribution of particle counting in assessment of exposure to P. Baconnier airborne microorganisms J.S. Fuglestvedt, T.K. Bernsten, 961 Climatic forcing of nitrogen oxides through changes in tropo- I.S.A. Isaksen, H. Mao, X.-Z. Liang spheric ozone and methane; global 3D model studies and W.-C. Wang E. Dupont, L. Menut, B. Carissimo, 979 Comparison between the atmospheric boundary layer in Paris J. Pelon and P. Flamant and its rural suburbs during the ECLAP experiment U. Kuhn, C. Ammann, A. Wolf, 995 Carbonyl sulfide exchange on an ecosystem scale: soil repres- F.X. Meixner, M.O. Andreae and ents a dominant sink for atmospheric COS J. Kesselmeier Technical Note X. Li-Jones, C.M cCormick and 1009 Zero offset in computer-recorded analog data in measuring H.B. Maring aerosol scattering coefficient: a “threshold” or a “blank”? News and Opinions Introduction Calendar List of Forthcoming Papers Preparation of Papers Number 7 A.T. Buckland and 1017 Nomograms for calculating pollution within street canyons D.R. Middleton R.M. Harrison, J.P. Shi and 1037 Continuous measurements of aerosol physical properties in the M.R. Jones urban atmosphere J.G. Vasiliou, D. Sorensen 1049 Sampling at controlled relative humidity with a cascade impac- and P.H. McMurry tor R.D. Saylor, W.L. Chameides 1057 Demonstrating attainment in Atlanta using urban airshed and M.E. Chang model simulations: impact of boundary conditions and alternative forms of the NAAQS Contents of Volume 33 INQ B. Eklund 1065 Comparison of line- and point-source releases of tracer gases D.J. Luecken, G.S. Tonnesen 1073 Differences in NO, speciation predicted by three photochemi- and J.E. Sickles, II cal mechanisms M. Khan, Y.J. Yang and 1085 Photochemical reactivities of common solvents: comparison A.G. Russell between urban and regional domains A. Venkatram, D. Fitz, 1093 Using a dispersion model to estimate emission rates of partic- K. Bumiller, S. Du, M. Boeck ulate matter from paved roads and C. Ganguly C. Trevino and 1103 Simplified model for the prediction of ozone generation F. Méndez in polluted urban areas with continuous precursor species emissions Y. Andersson-Sk6éld and D. Simpson 1111 Comparison of the chemical schemes of the EMEP MSC-W and IVL photochemical trajectory models C. Zellweger, M. Ammann, 1131 NO, speciation with a combined wet effluent diffusion de- P. Hofer and U. Baltensperger nuder-aerosol collector coupled to ion chromatography I.J. Simpson, G.C. Edwards and Variations in methane and nitrous oxide mixing ratios at the G.W. Thurtell southern boundary of a Canadian boreal forest M.A.K. Khalil and R.A. Rasmussen Atmospheric chloroform C.M. Mitic, W.J. Massman, Structural analysis and flux associations of CO,, H,O, heat P.H. Schuepp and J.L. Collett Jr and ozone over cotton and grape canopies News and Opinions Introduction Calendar List of Forthcoming Papers Preparation of Papers Roomvent 2000 Announcement Number 8 M. Glasius, M.F. Carlsen, Measurements of nitrogen dioxide on Funen using diffusion T.S. Hansen and C. Lohse tubes D.J. Hall, S. Walker and 1187 Dispersion from courtyards and other enclosed spaces A.M. Spanton Z. Guo, J.C.S. Chang, L.E. Sparks 1205 Estimation of the rate of VOC emissions from solvent-based and R.C. Fortmann indoor coating materials based on product formulation H.N. Knudsen, U.D. Kjaer, 1217 Sensory and chemical characterization of VOC emissions from P.A. Nielsen and P. Wolkoff building products: impact of concentration and air velocity A. Feilberg, R.M. Kamens, 1231 Modeling the formation, decay, and partitioning of semivolatile M.R. Strommen and T. Nielsen nitro-polycyclic aromatic hydrocarbons (nitronaphthalenes) in the atmosphere J.M.F. Diaz, M.A.R. Brana, 1245 Difficulties inherent to the use of analytic solution of the con- B.A. Garcia, C.G.-P. Muniz densation-evaporation equation for multicomponent aerosols and P.J.G. Nieto L. Morawska, S. Thomas, 1261 A study of the horizontal and vertical profile of submicrometer D. Gilbert, C. Greenaway and particles in relation to a busy road E. Rijnders IN10 Contents of Volume 33 M.E. Jenkin and G.D. Hayman 1275 Photochemical ozone creation potentials for oxygenated volatile organic compounds: sensitivity to variations in kinetic and mechanistic parameters E. Smet, H.V. Langenhove and 1295 The emission of volatile compounds during the aerobic and the I.D. Bo combined anaerobic/aerobic composting of biowaste M.A.K. Khalil and R.A. Rasmussen 1305 Atmospheric methyl chloride Technical Note A. Kasper-Giebl and H. Puxbaum 1323 Deposition of particulate matter in diffusion tube samplers for the determination of NO, and SO, M. Sharan, A.K. Yadav, 1327 Accounting for the source strength in the solution of the diffu- M.P. Singh and S. Gupta sion equation: alternative mathematical formulations News and Opinions Introduction Calendar List of Forthcoming Papers Preparation of Papers Number 9 R. von Glasow and A. Bott 1333 Interaction of radiation fog with tall vegetation R. Gabriel, L. Schafer, C. Gerlach, 1347 Factors controlling the emissions of volatile organic acids from T. Rausch and J. Kesselmeier leaves of Quercus ilex L. (Holm oak) R. Leuning, S.K. Baker, I.M. Jamie, 1357 Methane emission from free-ranging sheep: a comparison of C.H. Hsu, L. Klein, O.T. Denmead two measurement methods and D.W.T. Griffith H.V. Andersen, M.F. Hovmand, 1367 Measurements of ammonia concentrations, fluxes and dry de- P. Hummelshgj and N.O. Jensen position velocities to a spruce forest 1991-1995 M. Vakeva, K. Hameri, 1385 Street level versus rooftop concentrations of submicron aerosol M. Kulmala, R. Lahdes, particles and gaseous pollutants in an urban street canyon J. Ruuskanen and T. Laitinen G. Aberg, D.E. Stijfhoorn, K. Iden 1399 Carbon isotope exchange during calcite sulphation and R. Lofvendahl A.N. Thakur, H.B. Singh, 1403 Distribution of reactive nitrogen species in the remote free P. Mariani, Y. Chen, Y. Wang, troposphere: data and model comparisons D.J. Jacob, G. Brasseur, J.-F. Miller and M. Lawrence A. Calogirou, B.R. Larsen and 1423 Gas-phase terpene oxidation products: a review D. Kotzias K.A. Rahn 1441 A graphical technique for determining major components in a mixed aerosol. I. Descriptive aspects M. Ikegawa, M. Kimura, 1457 Geographical variations of major and trace elements in East K. Honda, I. Akabane, K. Makita, Antarctica H. Motoyama, Y. Fujii and Y. Itokawa Y. Deng and Y. Zuo 1469 Factors affecting the levels of hydrogen peroxide in rainwater F. Sunny, T.N. Mahadevan and 1479 Estimation of actinic flux and photolysis rate constant of NO, V. Sitaraman from aerosol size data