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Air Pollution Modeling and Its Application XII PDF

739 Pages·1998·31.386 MB·English
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Air Pollution Modeling and Its Application XII NATO. Challenges of Modern Society A series of volumes comprising multifaceted studies of contemporary problems facing our society, assembled in cooperation with NATO Committee on the Challenges of Modern Society. Recent volumes in this series: Volume 6 REMOTE SENSING FOR THE CONTROL OF MARINE POLLUTION Edited by Jean-Marie Massin Volume 7 AIR POLLUTION MODELING AND ITS APPLICATION IV Edited by C. De Wispelaere Volume 8 CONTAMINATED LAND: Reclamation and Treatment Edited by Michael A. Smith Volume 9 INTERREGIONAL AIR POLLUTION MODELING: The State of the Art Edited by S. Zwerver and J. van Ham Volume 10 AIR POLLUTION MODELING AND ITS APPLICATION V Edited by C. De Wispelaere, Francis A. Schiermeier, and Noor V. Gillani Volume 11 AIR POLLUTION MODELING AND ITS APPLICATION VI Edited by Han van Dop Volume 12 RISK MANAGEMENT OF CHEMICALS IN THE ENVIRONMENT Edited by Hans M. Seip and Anders B. Heiberg Volume 13 AIR POLLUTION MODELING AND ITS APPLICATION VII Edited by Han van Dop Volume 14 HEALTH AND MEDICAL ASPECTS OF DISASTER PREPAREDNESS Edited by John C. Duffy Volume 15 AIR POLLUTION MODELING AND ITS APPLICATION VIII Edited by Han van Dop and Douw G. Steyn Volume 16 DIOXIN PERSPECTIVES: A Pilot Study on International Information Exchange on Dioxins and Related Compounds Edited by Erich W. Bretthauer, Heinrich W. Kraus, and Alessandro di Domenico Volume 17 AIR POLLUTION MODELING AND ITS APPLICATION IX Edited by Han van Dop and George Kallos Volume 18 AIR POLLUTION MODELING AND ITS APPLICATION X Edited by Sven-Erik Gryning and Millan M. Millan Volume 19 METHODS OF PESTICIDE EXPOSURE ASSESSMENT Edited by Patricia B. Curry, Sesh Iyengar, Pamela A. Maloney, and Marco Maroni Volume 20 PLANNING ESTUARIES Cees-Jan van Westen and Reinier Jan Scheele Volume 21 AIR POLLUTION MODELING AND ITS APPLICATION XI Edited by Sven-Erik Gryning and Francis A. Schiermeier Volume 22 AIR POLLUTION MODELING AND ITS APPLICATION XII Edited by Sven-Erik Gryning and Nadine Chaumerliac Air Pollution Modeling and Its Application XII Edited by Sven-Brik Gryning RiS0 National Laboratory Roskilde, Denmark and Nadine Chaumerliac Universite Blaise Pascal-CNRS Clermont-Ferrand, France Published in cooperation with NATO Committee on the Challenges of Modern Society Springer Science+Business Media, LLC Library of Congress Cataloging in Publication Data Air pollution modeling and its application XII / edited by Sven-Erik Gryning and Nadine Chaumerliac. p. cm.—(NATO challenges of modern society; v. 22.) "Published in cooperation with NATO Committee on the Challenges of Modern Society." Proceedings of the Twenty-Second NATO/CCMS International Technical Meeting on Air Pollution Modeling and its Application, held June 2-6, 1997, in Clermont-Ferrand, France. Includes bibliographical references and index. 1. Air—Pollution—Mathematical models—Congresses. 2. Atmospheric diffusion—Mathe- matical models—Congresses. I. Gryning, Sven-Erik. II. Chaumerliac, Nadine. III. North At- lantic Treaty Organization. Committee on the Challenges of Modern Society. IV. NATO/ CCMS International Technical Meeting on Air Pollution Modeling and its Application (22nd: 1997: Clermont-Ferrand, France) V. Series. TD881.A47523 1998 628.5' 3' 015118—dc21 98-7493 CIP Proceedings of the Twenty-Second NATO/CCMS International Technical Meeting on Air Pollution Modeling and Its Application, held June 2-6, 1997, in Clermont-Ferrand, France ISBN 978-1-4757-9130-3 ISBN 978-1-4757-9128-0 (eBook) DOI 10.1007/978-1-4757-9128-0 © Springer Science+Business Media New York 1998 Originally published by Plenum Press, New York in 1998 Softcover reprint of the hardcover 1st edition 1998 http://www.plenum.com 10 9 8 7 6 5 4 32 1 All rights reserved Mo part of this book may be reproduced, stored in a retrieval system, or transmitted in any form or by any means, electronic, mechanical, photocopying, microfilming, recording, or otherwise, without written permission from the Publisher PREFACE In 1969 the North Atlantic Treaty Organization (NATO) cstablishcd thc Committee on Challenges of Modern Society (CCMS). The subject of air pollution was from the thc very beginning one of the priority problems umier deliberation within the tJ-amcwork of various pi lot studies undertaken by this committee. The organization of a yearly conference dealing with air pollution modelling and its application has become one of the main activities within thc pilot study rclating to air pollution. Pleasc see the listing on the next page for completed NATO/CCMS Pilot Studies and the International Technical Meetings (ITM) on Air Pollution Modelling and Its Application. This volume contains the papers at the 22ND lTM, being held in Clermont-Ferrand, France during June 2 -6,1997. It was attended by 152 participants representing 33 countries. This lTM wasjointly organized by the Ris0 National Laboratory of Denmark (pilot country): the Laboratoire Associe de Meteorologic Physique, associated with the Centre National de la Recherche Scientifique, the Universite Blaise Pascal. and the Observatoire de Physique du Globe de Clermont-Ferrand, France (host country). We wish to express our gratitude to the sponsors that made this conference possible. In addition to tinancial support from NATO/CCMS, the conference received contributions from Centre National de Recherche Scientitique, Observatoire de Physique du Globe de Clermont-Ferrand, Universite Blaise Pascal, Electricite de France, lnstitut Francais du Pe trole, Conscil Regional d'Auvergne, Conseil General du Puy de DC1I11e, Mairie de Clermont Ferrand, SATCAR Semaine des arts techniques et culture de l'automobile et de la route. European Association for the Sciencies of Air Pollution, Ris0 National Laboratory. and the Danish Environmental Research Programme. On behalfofthe ITM Scientific Committee and the organizers, we express our grati tude to those who worked to make this conference a reality and to the active participants rep resenting numerous countries. Sven-Erik Gryning and Nadine Chaumerliac THE SCIENTIFIC BOARD OF THE 22nd NATO/CCMS INTERNATIONAL TECHNICAL MEETING 01\ AIR POLLUTION MODELING AND ITS APPLICA TIO:\ (i. Sehayes. Helgium D. Anfossi. Italy J. L. Walmsley. Canada T. Iversen. Norway S. L. Gryning (chairman), Denmark C. Borrego. Portugal H. R. Olesen. Denmark M. Millan. Spain W. Klug. Germany S. Ulug. Tyrkey N. Chaumerl iac. France M. L. Williams. United Kingdom G. Kallos. Greeee F. A. Schiermeier. USA R. M. van Aalst. Holland Y. Sehiffmann. USA II. \an Dop. Holland HISTORY OF :\ATO/CCMS AIR POLLUTION PILOT STUDIES Pilot Study on Air Pollution: International Technical Meetings (lTM) on Air Pollution Modeling and Its Application Dates of Completed Pilot Studies 1%9 1974 Air Pollution Pilot Study (United States Pilot Country) 1975 1979 Air Pollution Assessment Methodologies and Modeling (Germany) 19X() 19X4 Air Pollution Control Strategies and Impact Modeling (Germany) Dates and Locations of Pilot Study Follow-ep Meetings Pilot CO/IIII/TUnilcd States rR.A. AfcCormick, I.E. iVicmcl'cr) Feb 1971. Findhovcn. Thc Nctherlands-First Conference on Low Pollution Power Systems Development .lui 1971. Paris. France Second Meeting of the Expert Panel on Air Pollution Modeling All following meetings were entitled NATOICCMS International Technical Mectings ((I'M) on Air Pollution Modeling and Its Application Oet 197'2. Paris. France Third ITM May 1973. Oberursel. Federal Republic of Germany- Fourth ITM Jun 1974. Roskilde. Denmark--Fifth ITM Pi lot COlllltlT C;CI'II/(/II), (Erich ~j;('hcr) Sep 1975. Frankfurt. Federal Republic of Germany-. Sixth ITM Sep 1976. Airlie House. Virginia. USA--Seventh ITM Sep 1977. L.ouvain-La-Meuve. Belgium---Eighth ITM Aug I97X. Toronto. Ontario. Canada-Ninth ITM Oet 1979. ROllle. Italy--Tenth ITM \ 11 Pilot Country-Belgium (c. De Wispelaere) Nov 1980, Amsterdam, The Netherlands--Eleventh ITM Aug 1981, Menlo Park, California, USA-Twelfth ITM Sep 1982, Ile des Embiez, France-Thirteenth ITM Sep 1983, Copenhagen, Denmark-Fourteenth ITM Apr 1985, St. Louis, Missouri, USA-Fifteenth ITM Pilot Country-The Netherlands (Han van Dop) Apr 1987, Lindau, Federal Republic of Germany-Sixteenth ITM Sep 1988, Cambridge, United Kingdom-Seventeenth ITM May 1990, Vancouver, British Columbia, Canada-Eighteenth ITM Sep 1991, Ierapetra, Crete, Greece-Nineteenth ITM Pilot Country--Denmark (Sven-Erik Gryning) Nov 1993, Valencia, Spain-Twentieth ITM Nov 1995, Baltimore, Maryland, USA-Twenty-first ITM lun 1997, Clermont-Ferrand, France-Twenty-second ITM \ III CONTENTS INTEGRATED REGIONAL MODELLDIG Modeling of a Saharan Dust Event ...................................... . G. Cautener, B. Marticorena. and G. Bergametti Temporal and Spatial Scales for Transport and Transformation Processes in the Eastern Mediterranean .......................................... 15 G. Kallos. G. V. Kotroni. K. Lagouvardos. A. Papadopoulos. M. Varinou. O. Kakaliagou. M. Luria. M. Peleg. A. Wanger. and M. Uliasz Assimilation of Satellite Data in Regional Air Quality Models . . . . . . . . . . . .. 25 R. McNider. W. B. Norris. and D. M. Casey Evaluation of an Aerosol Model: Responses to Meteorology and Emission Scenari os . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. 37 S. C. Pryor. and R. J. Barthelmie Mesoscale Flow and Pollutants Transport Modeling in North-East Sicily ........... 43 P. Grossi. G. Graziani. and C. Cerutti Mesoscale Modeling of Transport and Deposition of Heavy Metals in Southern Poland. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .. 53 M. Uliasz. K. Olendrzynski. and 1. Bartnicki Biomass Burning: Local and Regional Redistribution. . . . . . . . . . . . . . . . . . . . . . . . . .. 63 J. Edy and S. Cautenet High Resolution. Long-Period Modelling of Photochemical Oxidants over Europe 71 J. Langner. C. Persson. and L. Robertson Application of the Urban Airshed Model in the Fraser Valley of British Columbia. Canada and Implications to Local Ozone Control Strategies ................. 71) J. Pottier Estimates of Sensitivities of Photochemical Grid Models to Uncertainties in Input Parameters. as Applied to UAM-IV on the New York Domain. . . . . . . . . . . . . RI) S. R. Hanna. J. C. Chang. M. E. Fernau. and D. A. Hansen IX Effects of Initial and Boundary Values of Reactive Nitrogen Compounds and Hydrocarbons on the Ozone Concentration in the Free Troposphere ........... 97 B. Schell, H. Feldmann, M. Memmesheimer, and A. Ebel Fast Sensitivity Analysis of Three-Dimensional Photochemical Models ............ 107 Y-J. Yang, J. G. Wilkinson, and A. G. Russell Integrating Observations and Modeling in Ozone Management Efforts . . . . . . . . . . . .. 115 S. T. Rao, E. Zalewsky, I. G. Zurbenko, P. S. Porter, G. Sistla, W. Hao, N. Zhou, J.-Y Ku, G. Kallos, and D. A. Hansen Study of the Role of a Stratiform Cloud Layer on the Redistribution of Hydrogen Peroxide .......................................................... 125 N. Audiffren, E. Buisson, and N. Chaumerliac Influence of the Resolution of Emissions and Topography on the Air Pollution . Distribution in a Mesoscale Area ....................................... 133 K. Nester, H.-1. Panitz, F. Fiedler, and W. Wilms A Comparison of CALPUFF Modeling Results with 1977 !nel Field Data Results .... 143 J. S. Irwin GLOBAL AND LONG-RANGE TRANSPORT Atmospheric Transport-Chemistry Modelling-Some Ideas for the Future .......... 157 P. Builtjes A Model for Airborne Poli-Dispersive Particle Transport and Deposition ........... 167 M. Galperin and D. Syrakov Numerical Study of Regional Air Pollution Transport and Photochemistry in Greece .. 177 I. Ziomas, P. Tzoumaka, D. Balis, D. Melas, D. Asimakopoulos, G. Sanida, P. Simeonidis, I. Kioutsioukis, and C. Zerefos Simulated Acidic Aerosol Long-Range Transport and Deposition over East Asia-Role of Synoptic Scale Weather System. . . . . . . . . . . . . . . . . . . . . . . . . . .. 185 1. Uno, T. Ohara, and K. Murano Long-Range Transport of Lead and Cadmium in Europe. Results of the Model Simulation for the 1985-1995 Period .................................... 195 J. Bartnicki, K. Olendrzynski, and M. Uliasz Long Range Transport of NO x' NOy' 03 and SOx over East Asia and the Western Pacific Ocean in Winter Season-a Numerical Analysis ..................... 205 T. Kitada, M. Nishizawa, and Y Kondo The Transport of Dust and SOx in East Asia during the PEM -B Experiment ......... 217 H. Xiao, G. R. Carmichael, and 1. Durchenwald A Simulation of Long-Range Transport ofCFCs in the Troposphere Using a 3-D Global Lagrangian Model with 6-Hourly Meteorological Fields .............. 227 W. 1. Collins, D. S. Stevenson, C. E. Johnson, and R. G. Derwent x

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