Advances inthe criteria fordividing thinsuperconducting filmsinto narrow andwide films V. M. Dmitriev,1,2 I. V. Zolochevskii,1,∗ and E. V. Bezuglyi1 1B.VerkinInstituteforLow Temperature Physics and Engineering, Kharkov 61103, Ukraine 2International LaboratoryofHighMagneticFieldsandLowTemperatures, Wroclaw53-421, Poland Theresultsofexperimentalinvestigationsofthecriticalcurrentsandcertainnonequilibriumphenomenain thinSnfilmsofdifferentwidthwareanalyzed.Usually,thinsuperconductingfilmsaredividedintotwogroups: narrowchannelsw<l ⊥andwidefilmsw>l ⊥.Awidetransitionalregionwheretheconditionw>l ⊥holds 1 withalargemarginandatthesametimecannotbeexplainedfromthestandpointofthetheoryoftheappearance 1 ofavortexstatehasbeenfound.Thisshowsthatthegenerallyacceptedcriterionw∼l ⊥fordividingfilmsinto 0 wideandnarrowdoesnotwork. Thetransitionintoawide-filmregime,describedbytheexistingtheoryofthe 2 vortexstate,isfullycompletedonlyforw/l ⊥(T)>10−20. n a PACSnumbers:74.40+k J 0 Itisnowgenerallyacceptedthatthinsuperconductingfilms 1.0 ] 1 cwaindthbewdainvdidtehdickinnteossndararroewsmaanldlerwtihdaenfithlmeps.eneFtrilamtiosnwdheopsthe GLI/Icc0.8 n l ⊥(T) of a magnetic field and the coherence length x (T), 0.6 o which ensures a uniform distribution of the current over the c 1 2 0.4 - film width and absence of vortex resistivity, are said to be r narrowchannels. Phase-slipcenters(PSCs) appearwhenthe p 0.2 u current, exceeding the critical current IGL(T) for Ginzburg- 0 10 20 30 40 50 60 70 c s Landau (GL) depairing, flows in a narrow channel. These w/l t. centersconsistofthe coresof size ∼x (T) and the diffusion ^ ma tailsonbothsidesofthecore,havingthelengthofthepene- sFaImGp.l1e:sRSendWuc5ed(Nc)r,itSicnaWlc6u(r•re)n,tSdneWnsi8ty(HIc)/,IScGnLWv9er(s(cid:7)us),wS/nlW⊥1f0or((cid:4)th)e; trationdepthofalongitudinalelectricfieldintothesupercon- curve2–ALtheoreticalcurve. Theparametersofthefilmscanbe - d ductor. The order parameterD and the superconductingcur- foundinRef.4. n rentI inthecoreofaPSCoscillate,andatcertainmoments s o D and Is vanish and the phase changes abruptly by 2p . The AL. Itturnedout[4] thatthe vortexresistivity arises only in c [ frequencyof the oscillations is determinedby the Josephson afilmofsufficientwidth,w>4l ⊥,whileforI>Im thefilm ratio fJ =2eV/h. passesnotintoanormalstatebutrathertoavortex-freestate 1 v Films whose width w>l ⊥(T),x (T) are said to be wide withphase-sliplines(PSLs)–thetwo-dimensionalanalogues 4 [1]. In such films, due to the Meissner screeningof the cur- of PSCs. Even more unexpected, and prompting us to raise 1 rent-inducedmagnetic field, the currentdistribution overthe thequestionofthetruecriterionfora“widefilm”,wasthebe- 9 width is nonuniform and exhibits sharp peaks at the edges. havior of the temperaturedependenceof the critical current, 1 AccordingtotheAslamazov-Lempitskiy(AL)theory[2],the shown in Fig. 1 for several samples as a dependence of the . 1 resistive transition of a wide film is due to the instability of reducedcurrentI/IcGL on theparameterw/l ⊥, whichis pro- 0 thecurrentstatewhentheedgecurrentdensityreachesavalue portionalto1−T/Tc.AccordingtotheALtheory,forw>l ⊥ 1 closetothecriticalcurrentdensity jGLintheGLtheory.This this dependenceshould be described by a universalfunction 1 c : instability results in the creation of vortices, whose motion ofw/l ⊥,IcAL/IcGL=1.5(pl ⊥/w)1/2 (curve2). Intheexperi- v generatesvoltageatthe endsof thefilm. Thecorresponding ment,asseenfromFig.1, thisuniversalitydoesindeedexist Xi criticalcurrentIcALissmallcomparedtoIcGL,sincethecurrent butonlyforverylargevaluesofw/l ⊥∼10−20,whichthere- densityinthebulkofthefilmisfarfromthecriticalvalue.On foreshouldserveastherealcriterionforatransitionintothe r a accountofthemotionandannihilationofthevortices,asec- wide-filmregime. ond sharp peak in the current density forms at the center of For smaller values of w/l ⊥, the behavior of the critical thefilm. ForcertainvalueIm ofthecurrent,themagnitudeof current is very peculiar. According to Ref. 4, samples with this peak reachesa criticalvalue jcGL, whichresults in insta- w/l ⊥ <4 are narrow channels (in Fig. 1 the region to the bilityofthestationaryflowofthevortices. IntheALtheory, left of the vertical straight line 1). In the interval between itwassupposedthatforI >Im a film exhibitstransitioninto the vertical straight line 1 and the curve 2, there is a tran- thenormalstate. sitional region where the film is “quasi-wide” (a vortex sec- The experimental investigations of resistive transitions in tionis presentinthe current-voltagecharacteristic(IVC) but wide films, although qualitatively confirmingthe above-des- the AL theory “does not work” yet). For the SnW10 film cribed picture of a nonuniform distribution of the current in (w=7m m)theexperimentalcurrentIc forw/l ⊥<4equals subcriticalandvortexstates [3, 4], haveatthe sametime re- the computed value of IGL. As temperature decreases, i.e. c sultedinconsiderablerefinementofthemainassumptionsof w/l ⊥ increases, vortexresistivity arisesandIc dropsrapidly 2 than the Josephson frequency, also point to the inapplicabil- ity of the widely accepted criterion w≈l ⊥(T) for a “wide film”. This phenomenon, called non-Josephson generation [5, 6], arises when a certain current density j is reached, g andthisgenerationcurrentdensityfornarrowtin films(w≈ x ≈ 1 m m) is 2.7 times higher than for wide samples with w>20m matthesamereducedtemperatureT/T =0.99[6]. c Thus,forfilmwidthintherange1−20m m,asmoothtransi- tioncanoccurfromhightolowgenerationcurrentdensities. FIG.2: GenerationcurrentdensityversusSnfilmwidthatT/Tc= To check this assumption, a film obtained in one deposition 0.99. operation was used to prepare a series of samples with dif- ferentwidth. The results of measurementsof the generation toasmallervalue,whichnonethelessrevealsthetemperature currentdensity jg versusthewidthwoftinfilmsattempera- dependenceclosetoIc(T)thatcontinuesrightuptoatransi- tureT =0.99Tc [6]arepresentedinFig. 2. Itisevidentthat tionintoregimedescribedbytheALtheory.Thisdecreaseof the center of the transition from a narrow to a wide channel I isevenmorerapidfortheSnW6film(w=17m m),asare- correspondstow≈12m m.Thus,fromthestandpointofnon- c sultofwhichtheregionofthetransitionaltemperaturedepen- Josephson generation, tin films with width up to w≈5 m m dence I (cid:181) (1−T/T)3/2 expands considerably. Finally, for canbetreatedasnarrowchannels,whiletheybecome“wide” c c thewidestfilmsSnW8(w=25m m)andSnW5(w=42m m), onlyforw>20m m. whereanarrow-channelregimeisnotobservedbecauseofthe A similar conclusion concerningthe inapplicability of the extremeproximityofthecorrespondingtemperatureregionto widelyacceptedcriterionw≈l ⊥(T)[1]fordeterminingthe Tc,thedependenciesofIc/IcGLonw/l ⊥arecompletelyidenti- boundarybetween narrowand wide films can also be drawn cal,andthewidthofthetransitionalregionreachessaturation. on the basis of an analysis of changes in the dependence of It should be noted that the observed wide transitional re- thecriticalcurrentIconthepowerPofanexternalmicrowave gion, where the conditionw>l ⊥ holdswith a large margin field for films with differentwidth [7]. Figure 3a shows the andatthesametimethedependenceIc(T)isidenticaltothe functionIc(P)inrelativeunitsfortinfilmsofdifferentwidth behaviorofIGL(T), cannotbeexplainedfromthestandpoint underidenticalexperimentalconditions. Thedescendingsec- c of the AL theoryof the mechanismof the appearanceof the tions of the curves Ic(P)/Ic(0) in Fig. 3a can be fit by the vortexstate. Acharacteristicfeatureofthisregionisa sharp functionIc(cid:181) (1−P/Pc)a .ForthesampleSnW10(w=7m m), transitionofIc(cid:181) (1−T/Tc)3/2toIcAL(T)(cid:181) 1−T/Tc.Ournu- whichatT/Tc=0.99isanarrowchannel[4],thedependence merical solution of the London integral equation [2] for the Ic(P)/Ic(0)isconvexand,correspondingly,a =0.53<1.For currentdistributionoverthefilmwidthforarbitraryvaluesof thesampleSnW6(w=17m m)thisdependencebecomescon- w/l ⊥ also shows the absence of a wide transitional region caveanda =1.4islargerthan1,whilefortheobviouslywide betweenIGL(T)andIAL(T)providedthecriticalcurrentden- filmSnW5(w=42m m)a =2.9. Thedependenceoftheex- c c sity jGL is reachedat the edge of the film at the pointof the ponent of the fitting functions of the critical current versus c transition. This could signify that the condition for the ap- thesample width, presentedinFig. 3b, showsthatthevalue pearance of vortices for w/l ⊥ < 10−20 weakens because a =1canbeexpectedforafilmofwidthw≈12m m,andthe of the existence of a competing mechanism for the penetra- descendingsectionofthefunctionIc(P)isa straightline. In tion of vortices into the film when the edge current density otherwords, as the film width increases, the sign of the cur- reachessomevalue j (T)smallerthan jGL(T). Toexplainthe vatureofthedescendingsectionsofthecurveschanges,anda c c observedconstancyofthe valueof Ic/IGL in the transitional filmwithw≈12m misaboundarybetweenquasi-narrowand c region,it mustbe assumedthatas thetemperaturedecreases quasi-widesamples,asinthecasedisplayedinFig. 2. thequantity jc(T)increasesmorerapidlythan jcGL(T),andis In summary, the result of the investigationsof the critical proportionalto(1−T/Tc)2. Atthepointwheretheybecome currentsanddifferentnonequilibriumphenomenainthinfilms equal,atransitionoccursintotheALregime,whichexplains ofdifferentwidthmakeitpossibletoconcludethatthewidely thesharpnessofthecrossovertothelineartemperaturedepen- acceptedcriterionw∼l ⊥fordividingfilmsintowideandnar- denceofIAL(T)seeninFig.1.Inprinciple,suchamechanism rowdoesnotwork. Thetransitionintothewide-filmregime, c can be associated with edge microdefects, which have virtu- describedbytheexistingtheoryofthevortexstate, fullyoc- allynoeffectontheGLdepairingcurrentinthenarrow-film curs only for w/l ⊥ >10−20. It can be supposed that the regime,buttheyareasourceofvorticesinawidefilm.Atthe simplecriterionw>l ⊥ doesnotworkinpracticebecauseof same time the excellent quantitative agreement between the the structural particularities of a Pearl vortex in a thin film, critical currents Ic(T), Im(T) and the predictions of the AL which is not a truly localized formation [8]: in contrast to theoryfor large valuesof w/l ⊥ casts doubton this supposi- an Abrikosov vortex in a bulk superconductor, its fields de- tion. creasewithincreasingdistancenotexponentiallybutratherin Other nonequilibrium phenomena, for example, the gen- a power-lawfashion. Specifically, Kogan[9] hasshown that eration of electromagnetic oscillations with frequencylower the magnetic flux trapped by a single vortex in a thin film, 3 even at a distance 24l ⊥ from the vortex core, is 90% of the (a) fluxquantum.Theratiobetweenthefilmwidthandthepene- 1.5 3 0) trationdepthofanelectricfield,whichforw/l ⊥∼10isclose I(c to1,canalsoplayacertainrole.The“anomalous”vortexstate / ) (transitionalregion)whichwediscoveredandwhicharisesin P I(c the interval 4<w/l ⊥ <10−20 for the computed value of 1.0 theedgecurrentdensity(cid:181) (1−T/T)2muchsmallerthanthe c 2 depairing current density jGL(T) draws attention also. The c mechanismofthepenetrationofvorticesintoafilmforsuch small edge currentsand the reason why it vanishesfor large 0.5 valuesofw/l ⊥arenotdescribedbyexistingtheoriesandhave noexplanationatthepresenttime. 1 0.0 0.0 0.5 1.0 ∗ Electronicaddress:[email protected] P /P [1] I.M.Dmitrenko, Fiz.Nizk.Temp.22, 849(1996)[LowTemp. c Phys.22,845(1996)]. 3 [2] L.G.AslamazovandS.V.Lempitskiˇi,Zh.Eksp.Teor.Fiz.84, 2216(1983)[Sov.Phys.JETP57,1291(1983)]. [3] A. G. Sivakov, A. P. Zhuravel, O. G. Turutanov, and I. M. Dmitrenko,Czech.J.Phys.46,877(1996). (b) [4] V.M.DmitrievandI.V.Zolochevskii,Supercond.Sci.Technol. 19,342(2006). [5] G.E.Churilov,V.M.Dmitriev,andA.P.Beskorsyˇi,PismaZh. 2 Eksp.Teor.Fiz.10,231(1969). [6] G. E. Churidov, V. N. Svetlov, and V. M. Dmitriev, Fiz. Nizk. Temp.12,425(1986)[Sov.J.LowTemp.Phys.12,242(1986)]. a [7] V. M. Dmitriev, I. V. Zolochevskiˇi, T. V. Salenkova, and E. V. Khristenko,Fiz.Nizk.Temp.31,1258(2005)[LowTemp.Phys. 31,957(2005)]. [8] J.Pearl,Appl.Phys.Lett.5,65(1964). 1 [9] V.G.Kogan,Phys.Rev.B49,15874(1994) 0 0 10 20 30 40 w, m m FIG. 3: Relative critical current Ic(P)/Ic(0) versus the reduced•ir- radiationpowerP/Pc fordifferenttinfilms: SnW5(N),SnW6( ), andSnW10((cid:4))(a)andtheexponentofitsfittingfunctionversusthe widthwofthesampleat9.2GHzatT/Tc≈0.99(b).