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A study of beta-spectra of once-forbidden transitions PDF

94 Pages·6.602 MB·English
by  PriceHenry C
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Preview A study of beta-spectra of once-forbidden transitions

a B fiam o f m m i m n m m % 1# o&wjjr fr&e## J!F# H Smtattte*! to the Wmul&f of the Graduate School in F&rtlml M lfiltoint of tho &eqpl#M£g|&& for the Xtogp#*t Bootor of fhiloeophff to the Department of Indiana IM rerelty* 1961# t®Sr ProQuest Number: 10295258 All rights reserved INFORMATION TO ALL USERS The quality of this reproduction is dependent upon the quality of the copy submitted. In the unlikely event that the author did not send a complete manuscript and there are missing pages, these will be noted. Also, if material had to be removed, a note will indicate the deletion. uest, ProQuest 10295258 Published by ProQuest LLC (2016). Copyright of the Dissertation is held by the Author. All rights reserved. This work is protected against unauthorized copying under Title 17, United States Code Microform Edition © ProQuest LLC. ProQuest LLC. 789 East Eisenhower Parkway P.O. Box 1346 Ann Arbor, Ml 48106 - 1346 ACEHaMBfflBIEWS m fb© author hereby acknowledges the mid and guidance of W mtmmr terrene* H* Xsimge?# who dirested mod participated in the research described In this thesis and whose indefati^ gable energy and wealth of idea# amazed this work to oul-» situation* In addition the author desires to express hie appreciation for the- helpful sdrtee of Professor ML1 if* lomopineki;! especially that concerning certain aapeeta of the theory of befca^decay* He is further indebted to the Oak Ridge tohoratorlea Isotopes Btwteieaa for providing the radioasttre materials# to Dr« i^ t© l f# Jtouey for making the coincidence jse&aurments aM o^oulatiom* to Beatrice hanger and Betty Price for. performing certain other calculations* and to the latter for typing this- thesis* Tm author- is deeply grateful to professor Allan. 0* &* Httohell.|- not only for. generous use of the laboratory but Indeed for stimulation of the author*s original interest in physios as an undergraduate and for friendly emowagement throughout the last nine years* fhis work wm assisted by a grant to Br* banger from, the Frederick 0ardaer Cottrell fund of the. Research Corporation and by the Joint progrsii of the §HR and ABC*.. ABSffiAS? of thm m&t critical of the theory of bet&~ dtoay is th# of its predictions for energy aistri-* bubiema of ferbiMcn bete^brimsitioms to- the appropriate o^porlmtntal. moafwamauta* A aonewtod effort has boom made to find toto*totoflbi<m$ yielding unambiguous distributions not 'oorrospoiidiiig to- the allowed ahapoa by measuring in a mm&*Qiwmlm msi»Mb apootrtootor the bata^apaotoa of the forbidden toanatttontt of T^f Sr8®* X^# He3*86# ^ ?»* »#«* * with thin mw?<am* negligible scattering* ami t able adnntora m& high resolution*. A xmi%xm type of forbidden spectra la found for the first five while the last four yield in^lstinpilaMbla from the allowed shape ap o o tra in the rogiona meaawM* Interpretation of those spectra offers evidence for the reliability of mclear shell models* im the validity of MS. mtmileal rules* and for the dominance of the tensor md/m ttia l vector typo interactions in those beta**tramsit £ons which yield uni-quo ona«*ftobtdd*ft shapes* Sad points found aw (la Jfev)* 1,337 * o,007j 3r09, 1 ,« 3 * 0*005i f®©, 2,180 * 0.007} Cs1&7, 0*51 t 0,01} SblS4f s*,a91-'S 0,003, X.S9 1 0,01, 0,95 1 0,03 and lower groups; Au198, 0,956 r 0,005} He186, 1,063 1 0,006} ?3S, 1.(589 ± Q.Olf P#«?# 0*208® * 0,0005, oommm *43X8 of 4 1 t | A b stract 2 444 fable of dombsntt 8 I f 3 I* SAOM OltB* MSSBMKSf Of fllB PROBLEM 7 if# «nBOB«fiOA$, pxsensaiOT xx A*. Ifltocduotim IX 8* iergsiib M ft feluee IX 0# Fermi FormuXatica 12 l>* Other FomfiUtieiie 13 I# AppMatiia&bleme 17 % I# tow Appfes&mebieii 17 8* tow Energy Approximation 18 $# High i Approadbiatlon IS 4* Other Apm^oxlmiiom 10 P.* Screening Correction 10 III* fmoa s fii« W ii£ ifimiiOE so A* Spectral Shapes 20 B# Angular CtaweXetloae 20 X# El eetroiaMasetr iaao Correlation in BetaHdeeay 20 2* Bete^gamt Angular Correlation 22 8* G«aa^ga«a Oojprelefclon 23 8# Internal Bre»atF ahlung 24 O* Pooltron-oleofcron Capture Ratios 25 I* Decay SttosiC*# Lltetla*** and CMP ItiXejfr 25 m if* a rE ii« M * WHO0 A* The Speetreasieter 27 Sowee and Backing Prepar at ion 27 8*. X* Frepareticp of thin Films 27 2*. Source Definition and Conductivity 30 8* preparation #£ the Source Proper 31 0* Detection 32 f* SSSULTS 35 A* Yttrium 91 35 8* Strontium 8f and Yttrium 90 40 0*. Cesium 187 44 I>* Antimony 184 49 S« Rhenium 186 and Geld 198 55 P* Phosphorus 52 and Promethium 147 55 -«* 3 *► m 4 '■# f t# Q M H rn x tm a id m m m n m w fo r p tm h h r work as A* miMfcjr ©f the m m i Models as B* Information About Spin and Parity Changes 64 6 * Hvldeme for the feneor or AadeX fetter-' X$fcbtr«bi» S3 ©* InformtitB F r« Forbidiitn^Trmaition S tra ig h t I£ m IMS n e t t #6 B* F^tlw Smbstantietita ©£ the <MP Stlttbioa Rule® 68 fix* J&m&LX 70 A# lucloar Shell struotmii ifp?sli®abl« to Studied 70 B, Bit simtegr at ion Sthemt ^ ft #*,. pp *» 1 £*ft for frantltitM Studied 78 ©* More lta«b studies of FtrMddto Bttm fraueititut ft I* Chtadtbry 88 fill* EEFEIMOBa 87 LIST OS' FIOTRES glass, iSSS. ■% 30 Conventional P**E plot for taE lit determined independ­ ently by danger and Soapy* 2 $7 GoOTcgtion&X F-E plot for the Y** beta^opooWttm# 3 39 Forbidden P-K plot for the ywl bota^epootrum *. 4 41 Conventional P-K plot for the spectra of 3r®® and S3pw in secular equilib­ rium with $ 49 Forbidden M plot for the spectrum., 6 43 Fo||idden P-E plot for the St*®® spectrum Obtained after correcting for the Y®° contribution* 7 45 Conventional and forbidden F--E plots for data obtained with a scum of 3r®^ from which the It®® had been chemically ©acts?acted * & 40 Conventional arid forbidden F-& plota for data obtained from a thick j0>7 ing/emj*) ehemlcftlly^extracted Y*' so u rce* 0 47 Conventional and forbidden P-E plots for the spectrum of Oe * 10 50 Momentum distribution of th e S b l^ hot arrays* £1 ** 0 m Urn®, u #1 SonyontiqhaX F**E plot of the 66*®* be ta** distribution In the high energy region* m 5$ Forbidden F**K plot© of the ■sbr2* be t&^ distribution at high. energy* 54 Conventional and ones*»for« 15 M M fn W*& p lo ts o f tb s Sbi®4 data*. 14 S6 Conventional P»1 plot for t&* spsetvm of m 6 f C onventional F*K p lo t fo r tbs spectrum of Aul&B* 16 50 C onventional F*K p lo t fo r tbs spectrum of Pw# i f $1 C onventional FwK pj tbs spectrum of recorded with a bsktromSh grid counter -* fa Conventtonal P<*£ plot for 10 the spectrum of Wz¥*®* with recorded a tantalum grid counter*: frobSbl$r the Most aigmlf leant cheek on b$t.a<*decsy theory it m m xm m m t and analysis of the energy .distributions resulting from, forbidden For brevity ti-ie author chooses to. designate smoh spectre resulting from forbidden transitions by the tew forbidion^tf^t spectre (or forbidden spectra) If they are different from- th e.speetw of allowed transitions! otherwise* by the torn. aIlow«d*fcype spectra* The characteristic energy distribution for allowed transitions follows from almost any theory cs^ltlnimg the ea&eeian of two- light particles* For forbidden trmneititns^., different m rngf distributions may arise ■from each of the fits relatl vl $tieally invariant inter actions whlb& transform as scalar* polar' vector* tensor* axial vector,* and pmm^mmAm- respectively* (IK* IF) Far a threats, invariant theory* the transformation properties of the product of the wav© functions &S$#©imb#I with the em itted electron and neu trin o* h e re a fte r c a lle d th e .interaction*. e » * a t moat* be a lin e a r ee& M na& lm o f th e above fiv e b a sis in te ra c tio n s* (2E) Ferm i (21?) original if developed the theory In analogy with the polar vector interaction of e l r a d i a t i o n theory* Orlte&fteld and Wigner (10 J consider be % a*4i si nt cgr at ion as a simultaneous creation of* four- particle# (for mmple* a proton# an electron* and a neutrino in positive energy states and an tmobaerwable neutron in a. negative state) loading to the anti symmetrical m 0 3 m- 4 y (scalar' ■«* axial vector * pseudo sc alar)* /* A meson tre.#ta#nt# on tim other hand* proceed# in two steps and sen rake other Xin&w combination® | e « more natural# tt© theory m m m t 'decide among the various interactions nor can it really offer absolute ^e'TO^imcc that all five basic .interactions do hot enter with varying ©oeffioietifc# governed by yet unknown ami*# in such & fashion that on# interaction* say the tensor* is dominant in a given b«tm»fcrm&ttIon while other# or a combination of other# beoew dominant in other transition#* (If) S w w # the sspsrisgent&l result# for allowed spectra do exclude wy 11 m m mmblmx^lons involving; both '? and a or both f and A* |W# M) liofiH## ms&sursMxtft# and proper analysis of b#bi*#poebra of forbidden transition* shsmld yield ®mm distinction among the -possible Interactions# at least establishing a trend#, and perhaps ellmi&a&ittgs certain of the five ’basic interactions and certain of linear combination# as serious contenders#. ■Thai# five infceraofcio®# determ ine two a cts o f se le c tio n ' rule# concerning angular, momentum and parity# the Farad and the O&mow^feXXer (M S) r u lm * {16* ,21* 20) The polar' v ecto r and the scalar Infractions im wall as the pseudosc&lar Interaction# sxdfspt fo r o p p o site p a rity ) lead to n early th e mm» Feri&i ru les* shil# the 6WP rules# which permit a spin change of one gftcs&er than the Pmmn1 rules in all orders of forbldd#ni*#ssf ar© obeyed by the- tensor and eaam tlally also by the axial vector and the S ■# 4 •** F interactions * Information from forbidden spectra helps

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